Reversible Tuning of Nanowire Quantum Dot to Cesium D1 line
Rubayet Al Maruf, Sreesh Venuturumilli, Divya Bharadwaj, Paul Anderson, Jiawei Qiu, Mohd Zeeshan, Behrooz Semnani, Philip J. Poole, Dan Dalacu, Michael E. Reimer, Michal Bajcsy
We report local reversible tuning of nanowire quantum dot emission to cesium D1 line (~ 894.6 nm) and demonstrate slow light and resonant absorption of single photons in hot cesium vapor.
Quantum dots embedded in semiconductor photonic nanowires (NW-QDs) can deterministically produce single-photons and entangled photon pairs at high repetition rates. These photons can be efficiently coupled from the photonic nanowire into free space or optical fibers thanks to the sharp tip of the nanowire, which provides impedance matching. However, precise control of the NW-QD emission frequency in a way that is reversible, does not degrade the properties of the emitted photons, and can be used independently for individual NW-QDs on the same chip has so far remained a challenge. Resolving this issue is crucial for applications when interfacing the photons with quantum systems that require MHz to sub-GHz precision, such as atomic ensembles acting as memories in a quantum network. Here, we demonstrate a reversible tuning method that can tune the emission frequency of a NW-QD by more than 300 GHz with sub-GHz precision. We achieve this through gas condensation that is then partially reversed with localized laser ablation. This process finely adjusts stress applied to the quantum dots, thereby tuning their emission frequency. We validate the precision and stability of this method by tuning the frequency of the emitted single-photons across an atomic resonance to probe its absorption and dispersion. We observed up to 80\% absorption of the single-photons from NW-QD in hot caesium vapour at the D1-line resonances and a 75-fold decrease in group velocity associated with the hyperfine transitions of the D1-line ground states. We observed no discernible effects in the second-order autocorrelation function, lifetime, or linewidth of the NW-QD emission for up to 300 GHz of tuning and we saw minimal effects on the fine structure splitting of the NW-QD when tuning up to 100 GHz.
High Resolution Image Download MS PowerPoint Slide Quantum dots embedded in semiconductor photonic nanowires (NW-QDs) can deterministically produce single-photons and entangled photon pairs at high repetition rates. These photons can be efficiently coupled from the photonic nanowire into free space or optical fibers thanks to the sharp tip of the nanowire, which provides impedance matching. However, precise control of the NW-QD emission frequency in a way that is reversible, does not degrade the properties of the emitted photons, and can be used independently for individual NW-QDs on the same chip has so far remained a challenge. Resolving this issue is crucial for applications when interfacing the photons with quantum systems that require MHz to sub-GHz precision, such as atomic ensembles acting as memories in a quantum network. Here, we demonstrate a reversible tuning method that can tune the emission frequency of a NW-QD by more than 300 GHz with sub-GHz precision. We achieve this through gas condensation that is then partially reversed with localized laser ablation. This process finely adjusts stress applied to the quantum dots, thereby tuning their emission frequency. We validate the precision and stability of this method by tuning the frequency of the emitted single-photons across an atomic resonance to probe its absorption and dispersion. We observed up to 80% absorption of the single-photons from NW-QD in hot cesium vapor at the D 1 -line resonances and a 75-fold decrease in group velocity associated with the hyperfine transitions of the D 1 -line ground states. We observed no discernible effects in the second-order autocorrelation function, lifetime, or linewidth of the NW-QD emission for up to 300 GHz of tuning and we saw minimal effects on the fine structure splitting of the NW-QD when tuning up to 100 GHz.
We describe the development and applications of a single-photon source based on a quantum dot embedded in a semiconductor nanowire, which can be precision-tuned to emit ∼1ns long photons at wavelengths that match the transitions of caesium D1 line. We discuss interfacing such single-photon source with atomic ensembles and present our experimental results demonstrating a new method of tuning the emission of the quantum dot by condensing inert gas (N2) on the nanowire. Next, we describe how these single photons at ∼895nm can be efficiently converted to wavelength suitable for satellite QKD links (∼794 nm) and optical fiber links (∼1469 nm) using a laser-cooled atomic ensemble that is loaded and confined inside a hollow-core optical fiber. Lastly, we inroduce our proposal of integrating the semiconductor nanowire with a lensed fiber to create a compact single-photon source with improved photon-collection efficiency compared to conventional setups.
Abstract Hybrid quantum technologies aim to combine diverse quantum systems, mirroring classical computers' integration of electronic, photonic, magnetic, and mechanical components. Quantum dots in semiconductor nanowires emit high-purity, deterministic single photons with high repetition, while atomic ensembles offer photon storage and strong optical nonlinearities controllable by single photons. To interface quantum dots with atomic ensembles successfully, precise optical frequency matching of these two platforms is crucial. We demonstrate a simple, precise, reversible, broad-range, and local method for controlling the emission frequency of individual quantum dots embedded in tapered semiconductor nanowires. We then interface the quantum dots with an atomic ensemble via single-photons matched to hyperfine transitions and slow-light regions of the cesium D1-line. Our approach allows linking atomic and solid-state quantum systems and can potentially also be applied to other types of nanowire-embedded solid-state emitters, as well as for creating devices based on multiple solid-state emitters tuned to produce indistinguishable photons.
In forthcoming quantum networks various quantum systems might be involved to accomplish individual tasks, including storage of quantum states, quantum logic operations, error correction, or entanglement distillation. An interface between a single photon emitter and a potential photon storage could provide one fundamental building block of such a hybrid quantum system. Semiconductor quantum dots (QD) and atomic vapors have already been brought together by single photon spectroscopy of cesium and rubidium [1,2], narrow filtering of QD resonance fluorescence in cesium [3], slowing down QD photons by dispersion between the 6.8 GHz hyperfine-split rubidium D2transitions [4] and in the middle of the four cesium D1 transitions [5] (at around 5.0 GHz in Fig. 1 b).In our experiment the neutrally charged excitonic transition of a strain-tunable InGaAs QD is pumped either resonantly or non-resonantly by a pulsed laser. The QD emission is set between two cesium D1 transitions at 894 nm, which are hyperfine-split only by 1.2 GHz, with a very strong dispersion compared to preceding studies [4,5]. This allows for delay times of a few nanoseconds even at low optical densities, resulting in a propagation velocity at the order of 1/20 of the vacuum speed of light. Such a single photon - atom interface might lay the foundations for a low-loss quantum memory in a future hybrid quantum network.
A bright source of on-demand entangled photons is needed for quantum networks. A single quantum dot in a site-selected nanowire waveguide is a promising candidate for realizing such sources. However, such sources are associated with poor single-photon indistinguishability, limiting their applicability in quantum networks. A common approach for enhancing the single-photon indistinguishability in quantum dot-based entangled photon sources is to implement a broadband optical cavity. Achieving a high-Purcell cavity while retaining the advantages of the nanowire, such as directional emission, a broad operational bandwidth, and high light extraction efficiency, has been a significant challenge. Here, we propose a nanowire cavity based on quasi-bound states in the continuum formed by the strong coupling of two resonant optical modes. We numerically predict this design to support a cavity mode with 4 nm bandwidth and a Purcell enhancement of $\sim$17. This cavity mode enables a directional far-field emission profile (88% overlap with a Gaussian) with a light extraction efficiency of $\sim$74%. Our solution opens up a route for generating entangled photon pairs with enhanced extraction efficiency and single-photon indistinguishability for the practical realization of quantum networks.