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Physical Review Applied

Polarization Entanglement from Parametric Down-conversion with an LED Pump

Wuhong Zhang, Diefei Xu, Lixiang Chen

Published May 24, 2023• 13 citations
Publisher

Abstract

Spontaneous parametric down-conversion (SPDC) is a reliable platform for entanglement generation. Routinely, a coherent laser beam is an essential prerequisite for pumping the nonlinear crystal. Here we break this barrier to generate polarization-entangled photon pairs by using a commercial light-emitting diode (LED) source to serve as the pump beam. This effect is counterintuitive, as the LED source is of extremely low spatial coherence, which is transferred during the down-conversion process to the biphoton wave function. However, the type-II phase matching condition naturally filters the specific frequency and wavelength of LED light exclusively to participate in SPDC such that localized polarization Bell states can be generated, regardless of the global incoherence over the full transverse plane. In our experiment, we characterize the degree of LED light-induced polarization entanglement in the standard framework of the violation of Bell's inequality. We achieve the Bell value $S=2.33\ifmmode\pm\else\textpm\fi{}0.097$, obviously surpassing the classical bound $S=2$ and thus witnessing the quantum entanglement. Our work can be extended to prepare polarization entanglement by using other natural light sources, such as sunlight and biolight, which holds promise for electricity-free quantum communications in outer space.

DOI
10.1103/physrevapplied.19.054079

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Polarization Entanglement from Parametric Down-Conversion with a LED Pump

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Spontaneous parametric down-conversion (SPDC) is a reliable platform for entanglement generation. Routinely, a coherent laser beam is an essential prerequisite for pumping the nonlinear crystal. Here we break this barrier to generate polarization entangled photon pairs by using a commercial light-emitting diode (LED) source to serve as the pump beam. This effect is counterintuitive, as the LED source is of extremely low spatial coherence, which is transferred during the down-conversion process to the biphoton wavefunction. However, the type-II phase-matching condition naturally filters the specific frequency and wavelength of LED light exclusively to participate in SPDC such that localized polarization Bell states can be generated, regardless of the global incoherence over the full transverse plane. In our experiment, we characterize the degree of LED light-induced polarization entanglement in the standard framework of the violation of Bell inequality. We have achieved the Bell value $S=2.33\pm 0.097$, obviously surpassing the classical bound $S=2$ and thus witnessing the quantum entanglement. Our work can be extended to prepare polarization entanglement by using other natural light sources, such as sunlight and bio-light, which holds promise for electricity-free quantum communications in outer space.

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We report a bright source of polarization-entangled photon pairs using spontaneous parametric down-conversion (SPDC) in a 10 mm long type-II PPKTP crystal pumped by a broadband multi-mode diode laser with the coherence length of 330 μm. Ordinarily, the huge mismatch between the pump coherence length and the PPKTP length would degrade the polarization entanglement completely. By employing the universal Bell-state synthesizer scheme, we remove the spectral/temporal distinguishability of the biphoton amplitudes entirely to recover high-visibility and high-fidelity two-photon polarization entanglement. The pair detection rates are 7,000 pairs/mW via single-mode fibers (with 99.2% fidelity) and 90,900 pairs/mW via multi-mode fibers (with 96.8% fidelity). We also analyze the scheme theoretically to show the effect of broadband multi-mode pumping on the phase matching condition of the type-II PPKTP.

Optics Express•Jan 13, 2016•28 citations
Spontaneous parametric down-conversion (SPDC) is a reliable platform for entanglement generation. Routinely, a coherent laser beam is an essential prerequisite for pumping the nonlinear crystal. Here we break this barrier to generate polarization-entangled photon pairs by using a commercial light-emitting diode (LED) source to serve as the pump beam. This effect is counterintuitive, as the LED source is of extremely low spatial coherence, which is transferred during the down-conversion process to the biphoton wave function. However, the type-II phase matching condition naturally filters the specific frequency and wavelength of LED light exclusively to participate in SPDC such that localized polarization Bell states can be generated, regardless of the global incoherence over the full transverse plane. In our experiment, we characterize the degree of LED light-induced polarization entanglement in the standard framework of the violation of Bell's inequality. We achieve the Bell value S=2.33\ifmmode±\else\textpm\fi0.097S=2.33\ifmmode\pm\else\textpm\fi{}0.097S=2.33\ifmmode±\else\textpm\fi0.097, obviously surpassing the classical bound S=2S=2S=2 and thus witnessing the quantum entanglement. Our work can be extended to prepare polarization entanglement by using other natural light sources, such as sunlight and biolight, which holds promise for electricity-free quantum communications in outer space.
Spontaneous parametric down-conversion (SPDC) is a reliable platform for entanglement generation. Routinely, a coherent laser beam is an essential prerequisite for pumping the nonlinear crystal. Here we break this barrier to generate polarization entangled photon pairs by using a commercial light-emitting diode (LED) source to serve as the pump beam. This effect is counterintuitive, as the LED source is of extremely low spatial coherence, which is transferred during the down-conversion process to the biphoton wavefunction. However, the type-II phase-matching condition naturally filters the specific frequency and wavelength of LED light exclusively to participate in SPDC such that localized polarization Bell states can be generated, regardless of the global incoherence over the full transverse plane. In our experiment, we characterize the degree of LED light-induced polarization entanglement in the standard framework of the violation of Bell inequality. We have achieved the Bell value S=2.33±0.097S=2.33\pm 0.097S=2.33±0.097, obviously surpassing the classical bound S=2S=2S=2 and thus witnessing the quantum entanglement. Our work can be extended to prepare polarization entanglement by using other natural light sources, such as sunlight and bio-light, which holds promise for electricity-free quantum communications in outer space.
Spontaneous parametric down-conversion (SPDC) can produce entangled photons from a nonlinear medium driven by a pump beam, and has thus been a key resource in photonic quantum technologies. Historically, the low efficiency of SPDC prompted the use of lasers, which are high-intensity light sources, as pump sources. However, the practical implementation of laser-driven systems faces an imminent energy bottleneck. Lasers typically have suboptimal energy efficiencies due to lasing thresholds and the technical demands of thermal management. As a result, laser-pumped entangled photon sources suffer from significant power overhead, rendering quantum devices less sustainable. Over the past few decades, light-emitting diodes (LEDs) have emerged as inexpensive and energy-efficient alternatives for high-intensity light sources. Since 2010, studies have shown that LEDs can drive SPDC and generate photon pairs. These results suggests the potential to replace lasers with ubiquitous and natural light sources to build environmentally friendly quantum devices. However, replacing lasers with other light sources entails a lack of coherence in all degrees of freedom (DoFs) of the pump beam, including spatial, temporal-spectral, and polarization, which may influence the resulting entanglement generated from SPDC. While earlier studies established that pump coherence in a specific DoF sets an upper bound for entanglement in that same DoF, the cross-influence between different DoFs has not been fully investigated. In this thesis, we study the influence of the pump's spatiotemporal coherence on the polarization entanglement generated from SPDC. First, we experimentally demonstrate that polarization-entangled two-photon states can be generated from SPDC pumped by spatiotemporally incoherent light emitted from an LED. Although the resulting entanglement appears lower than that of laser-pumped SPDC, we theoretically show that spatiotemporal incoherence does not fundamentally constrain polarization entanglement; rather, the reduction arises from a coupling between spatiotemporal and polarization DoFs introduced by the experimental setup. We determined experimentally that this cross-influence acts as a deterministic mapping from the spatial components of the pump to the two-photon polarization state. Because this mapping depends on technical aspects of the setup, we envisioned that it could be either (i) engineered to structure entanglement in higher dimensions, or (ii) compensated to reduce spatial distinguishability. Building on the latter, we show that by placing the nonlinear medium in a phase-compensated interferometric setup, SPDC pumped by spatially incoherent light can produce high polarization entanglement that violates local realism, even without postselecting the SPDC field for a single spatial mode. Finally, as a proof-of-principle demonstration of a truly environmentally friendly quantum light source, we demonstrate the generation of polarization-entangled two-photon states from SPDC pumped by a natural source - sunlight.
Spontaneous parametric down conversion (SPDC)-based sources of photonic entangled states are usually generated using coherent pump fields. For temporal, spatial, and polarization degree of freedom, the down-converted light entanglement is limited by the coherence of the pump in the same degree of freedom. However, the effect of pump coherence on the entanglement in a different degree of freedom remains largely unexplored. Here we experimentally demonstrate the generation of polarization entanglement from SPDC pumped by a light emitting diode (LED), a spatiotemporally incoherent pump. The two-photon state is found to have a concurrence of 0.562 and purity of 0.647.
We experimentally demonstrate a violation of local realism with highly spatially multimode polarization-entangled two-photon states produced by spontaneous parametric down-conversion (SPDC) pumped by a spatially incoherent light source---a light-emitting diode (LED). While existing studies have observed such a violation only by postselecting the LED-pumped SPDC photons into a single spatial detection mode, we achieve a Clauser-Horne-Shimony-Holt inequality violation of $S=2.532\ifmmode\pm\else\textpm\fi{}0.069>2$ using a spatially multimode detection setup that collects nearly 4080 SPDC spatial modes. These results indicate that coherent pump sources, such as lasers, are not required for SPDC-based entanglement generation. Our work could enable novel and practical sources of entangled photons for quantum technologies such as device-independent quantum key distribution and quantum-enhanced sensing.
Quantum computation and quantum communication require sources of entangled photons, especially from low-cost diode lasers. This study considered a polarization entangled photons pulse source produced via a spontaneous parametric down-conversion process in the type-I phase-matching of two nonlinear crystals, incorporating a continuous wave laser diode operating in pulse mode as a pump. The generated photons were measured based on visibility as a function of the pump frequency and collection apertures. A polarization correlation between photon pairs of approximately 93% and a Bell parameter S value of 2.56 ± 0.05 were obtained using the source described here.
We report a bright source of polarization-entangled photon pairs using spontaneous parametric down-conversion (SPDC) in a 10 mm long type-II PPKTP crystal pumped by a broadband multi-mode diode laser with the coherence length of 330 μm. Ordinarily, the huge mismatch between the pump coherence length and the PPKTP length would degrade the polarization entanglement completely. By employing the universal Bell-state synthesizer scheme, we remove the spectral/temporal distinguishability of the biphoton amplitudes entirely to recover high-visibility and high-fidelity two-photon polarization entanglement. The pair detection rates are 7,000 pairs/mW via single-mode fibers (with 99.2% fidelity) and 90,900 pairs/mW via multi-mode fibers (with 96.8% fidelity). We also analyze the scheme theoretically to show the effect of broadband multi-mode pumping on the phase matching condition of the type-II PPKTP.