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Optical trapping of SrOH molecules for dark matter and T -violation searches

Hiromitsu Sawaoka, Abdullah Nasir, Annika Lunstad +4 more

We report an optical dipole trap of strontium monohydroxide (SrOH) with 1400(300) trapped molecules. Through optical pumping, we access vibrational states that are proposed for improved probes of the electron’s electric dipole moment (eEDM) and ultralight dark matter (UDM). For each of these states, the lifetime of trapped molecules is measured and found to be consistent with spontaneous radiative decay and blackbody excitation limits, making this platform viable for these eEDM and UDM searches.We report an optical dipole trap of strontium monohydroxide (SrOH) with 1400(300) trapped molecules. Through optical pumping, we access vibrational states that are proposed for improved probes of the electron’s electric dipole moment (eEDM) and ultralight dark matter (UDM). For each of these states, the lifetime of trapped molecules is measured and found to be consistent with spontaneous radiative decay and blackbody excitation limits, making this platform viable for these eEDM and UDM searches.

arXiv:2509.01618Physical Review ResearchDec 17, 20258 citations

Optical Dipole Traps for Neutral Atoms

Rudolf Grimm, Matthias Weidemüller, Yuri B. Ovchinnikov

Advances in atomic, molecular, and optical physicsJan 1, 20001,549 citations

Characterizing single atom optical dipole traps

Chung-Yu Shih, Michael J. Gibbons, Michael Chapman

Bulletin of the American Physical SocietyJun 7, 20122 citations

Zeeman frequency shifts in an optical dipole trap used to search for an electric-dipole moment

Michael V. Romalis, E. Norval Fortson

We calculate the Zeeman frequency shifts due to interactions with the light in a far-off-resonance optical dipole trap. These shifts are important for potential use of such a trap to search for an atomic permanent electric-dipole moment (EDM). We present numerical results for Cs and Hg, as examples of paramagnetic and diamagnetic atoms. The vector and tensor light shifts are calculated for a large range of trap optical frequencies, for both red-detuned and blue-detuned traps. We also consider frequency shifts resulting from magnetic dipole and electric quadrupole transitions mixed in by a static electric field. These shifts are particularly important for EDM experiments since they are linear in the electric field. The Zeeman frequency shifts represent a substantial problem for EDM experiments in a dipole trap and must be controlled with care to achieve theoretical sensitivity.We calculate the Zeeman frequency shifts due to interactions with the light in a far-off-resonance optical dipole trap. These shifts are important for potential use of such a trap to search for an atomic permanent electric-dipole moment (EDM). We present numerical results for Cs and Hg, as examples of paramagnetic and diamagnetic atoms. The vector and tensor light shifts are calculated for a large range of trap optical frequencies, for both red-detuned and blue-detuned traps. We also consider frequency shifts resulting from magnetic dipole and electric quadrupole transitions mixed in by a static electric field. These shifts are particularly important for EDM experiments since they are linear in the electric field. The Zeeman frequency shifts represent a substantial problem for EDM experiments in a dipole trap and must be controlled with care to achieve theoretical sensitivity.

Physical Review AJun 1, 199969 citations

Optical Dipole Trap

Galina A. Nemova

SPIE eBooksNov 6, 20190 citations

Ultracold mercury–alkali-metal molecules for electron-electric-dipole-moment searches

Ayaki Sunaga, V. S. Prasannaa, Minori Abe +2 more

Heavy polar diatomic molecules are the leading candidates in searches for the permanent electric-dipole moment of the electron (eEDM). Next-generation eEDM search experiments ideally require extremely large coherence times, in large ensembles of trapped molecules that have a high sensitivity to the eEDM. We consider a family of molecules, mercury--alkali-metal diatomics, that can be feasibly produced from ultracold atoms. We present calculations of the effective electric fields experienced by the electron in these molecules. The combination of reasonably large effective electric fields, and the possibility of obtaining trapped ultracold samples, leads us to identify these molecules as favorable candidates for eEDM search experiments.Heavy polar diatomic molecules are the leading candidates in searches for the permanent electric-dipole moment of the electron (eEDM). Next-generation eEDM search experiments ideally require extremely large coherence times, in large ensembles of trapped molecules that have a high sensitivity to the eEDM. We consider a family of molecules, mercury--alkali-metal diatomics, that can be feasibly produced from ultracold atoms. We present calculations of the effective electric fields experienced by the electron in these molecules. The combination of reasonably large effective electric fields, and the possibility of obtaining trapped ultracold samples, leads us to identify these molecules as favorable candidates for eEDM search experiments.

arXiv:1810.10177Physical Review AApr 5, 201918 citations

Development of an Optical Dipole Trap System for the Electron Electric Dipole Moment Search

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