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APL Photonics

Quantum structured light in high dimensions

Isaac M. Nape, Bereneice Sephton, Pedro Ornelas, Chané Moodley, Andrew Forbes

Published May 1, 2023• 103 citations
PDF (CC BY)Publisher

Abstract

Structured light has become topical of late, where controlling light in all its degrees of freedom has offered novel states of light long predicted, enhanced functionality in applications, and a modern toolbox for probing fundamental science. Structuring light as single photons and entangled states allows the spatial modes of light to be used to encode a large alphabet, accessing high dimensional Hilbert spaces for fundamental tests of quantum mechanics and improved quantum information processing tasks. In this tutorial, we outline the basic concepts of high dimensional quantum states expressed in a basis of spatial modes (structured light) and explain how to create, control, and detect such quantum states in the laboratory with a focus on transverse spatial modes such as the orbital angular momentum and pixel (position) modes. Finally, we highlight some example applications of such quantum structured light, from communications to imaging.

DOI
10.1063/5.0138224

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Experimental measurements in the transverse position of the image carried by the photon before and after storage are presented in (d) and (e), respectively; (f) shows the simplified experimental setup for storage of a superposition of OAM. Interference patterns taken at different angle settings of the half-wave plate are shown in (g). The left column represents the experimental angle settings of the half-wave and the quarter-wave plates, the middle column gives the experimental results, and the right column gives results from theoretical simulations; (h) and (i) present the interference patterns of the input signal photon and the retrieved signal with plate angle, respectively. This is a significant breakthrough towards the realization of a quantum internet and, potentially, quantum computing. This work addresses the ability to generate, store, retrieve on demand an arbitrary single-photon-level photonic state encoded in OAM space. It signifies an important step in the development of practical quantum-enabled technologies, opens up the possibility for realizing high-dimensional quantum memories based on this degree of freedom of light, and will have a large impact in a broad physical community, especially in the quantum information and quantum optics communities. The Technology Review website of MIT comments on their work very positively with an article entitled ‘First Quantum Memory That Records the Shape of a Single Photon Unveiled in China’. Further, Nature Photonics selected this work as a research highlight. Clearly, memory that can preserve the spatial structure of photons will make the internet far more flexible and capable. Of course, there are still many basic problems remaining that need to be solved to build the future quantum internet, one of which is the construction of quantum memory exploiting entanglement. 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National Science Review•Aug 20, 2014•2 citations
Structured light has become topical of late, where controlling light in all its degrees of freedom has offered novel states of light long predicted, enhanced functionality in applications, and a modern toolbox for probing fundamental science. Structuring light as single photons and entangled states allows the spatial modes of light to be used to encode a large alphabet, accessing high dimensional Hilbert spaces for fundamental tests of quantum mechanics and improved quantum information processing tasks. In this tutorial, we outline the basic concepts of high dimensional quantum states expressed in a basis of spatial modes (structured light) and explain how to create, control, and detect such quantum states in the laboratory with a focus on transverse spatial modes such as the orbital angular momentum and pixel (position) modes. Finally, we highlight some example applications of such quantum structured light, from communications to imaging.
Quantum mechanics is now a mature topic dating back more than a century. During its scientific development, it fostered many technological advances that now are integrated into our everyday lives. More recently, over the past few decades, the authors have seen the emergence of a second quantum revolution, ushering in control of quantum states. Here, the spatial modes of light, “patterns of light,” hold tremendous potential: light is weakly interacting and so an attractive avenue for exploring entanglement preservation in open systems, while spatial modes of light offer a route to high dimensional Hilbert spaces for larger encoding alphabets, promising higher information capacity per photon, better security, and enhanced robustness to noise. Yet, progress in harnessing high dimensional spatial mode entanglement remains in its infancy. Here, the authors review the recent progress in this regard, outlining the core concepts in a tutorial manner before delving into the advances made in creation, manipulation, and detection of such quantum states. The authors cover advances in using orbital angular momentum as well as vectorial states that are hybrid entangled, combining spatial modes with polarization to form an infinite set of two-dimensional spaces: multidimensional entanglement. The authors highlight the exciting work in pushing the boundaries in both the dimension and the photon number, before finally summarizing the open challenges, and the questions that remain unanswered.
The ability to prepare, control, and detect high-dimensional photonic quantum states is a key capability in modern quantum science. Spatially structured single- and bi-photon states provide access to large Hilbert spaces, enabling both fundamental studies and practical advances across quantum technologies. Precise control of these states is essential to characterising quantum light sources and to using spatial degrees of freedom for information encoding, with applications ranging from quantum imaging and simulation to high-capacity, noise-resilient quantum communication. In this talk, I will review recent experimental and theoretical progress in structured-light quantum information processing. I will discuss high-dimensional QKD with structured photons, strategies based on adaptive optics and tailored measurements to counter channel distortions, and protocols that exploit spatial mode structure. I will also describe how structured photonic states can be used to simulate linear and cyclic quantum systems, illustrating their potential as scalable platforms for high-dimensional quantum information processing.
The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.
Structured light refers to the arbitrarily tailoring of optical fields in all their degrees of freedom (DoFs), from spatial to temporal. Although orbital angular momentum (OAM) is perhaps the most topical example, and celebrating 30 years since its connection to the spatial structure of light, control over other DoFs is slowly gaining traction, promising access to higher-dimensional forms of structured light. Nevertheless, harnessing these new DoFs in quantum and classical states remains challenging, with the toolkit still in its infancy. In this perspective, we discuss methods, challenges, and opportunities for the creation, detection, and control of multiple DoFs for higher-dimensional structured light. We present a roadmap for future development trends, from fundamental research to applications, concentrating on the potential for larger-capacity, higher-security information processing and communication, and beyond.
Quantum structured light offers a roadmap to high-dimensional and multi-dimensional quantum states by exploiting all of light’s many degrees of freedom at the quantum level. In this talk, I will review the recent progress in quantum entanglement of photons in their spatial degree of freedom: quantum structured light. I will explain how to create high-dimensional quantum states in the laboratory, how to measure them, and review the present state of the art in the field. I will show how the patterns can be abstracted, mixing degrees of freedom to produce quantum topologies in light, introducing new paradigms for quantum state observables and classification. Finally, I will outline the advantages and disadvantages of using such single photon and entangled states in real-world applications, offering a perspective on the present challenges and exciting opportunities in the field.
Quantum memory is a key component of quantum networks. A successful development in enabling the distribution of quantum information requires the storage of single-photon light. Usually quantum information is encoded using a 2D space, spanned, for example, by the orthogonal polarization states of a photon. In this case, each photon carries a quantum bit of information. If the photon could be encoded in a high-dimensional space instead, the information carried by each photon could be increased from a bit to |log⁡2d\log {}_2dlog2​d| bits, where d is the dimension of the Hilbert space in which the photon is described. The channel capacity of the network and the transmission efficiency would then be greatly enlarged [1]. Moreover, storing high-dimensional states in quantum memory can reduce its sensitivity to memory coherence time [2], leading to significant improvements in storage capacity [3]. It is thus no surprise that many research groups are actively working on different physical systems for storing light encoded using a high-dimensional space. The degrees of freedom for position, linear momentum, time-bin or orbital angular momentum (OAM) of a photon can all be considered as a high-dimensional space for encoding. The photon's OAM has the most potential for encoding [4]. Electromagnetic waves have both spin and OAM. Spin angular momentum produces polarization. Photons with OAM can be regarded as helices with left and right handedness twisted to varying degrees (Fig. 1). Information is encoded using this handedness and the amount of twist. Because of the inherent infinite degrees of freedom for OAM, a photon can in principle carry an arbitrarily large amount of information, and hence the eagerness to store light encoded in OAM space. Although some work on this has been reported for different physical systems, what is lacking is a way of storing and releasing at some later time a true single photon, including its shape and structure [5–7]. Constructing this basic element of quantum memory has been a major challenge. The wavefront of an OAM light is a helical structure (left and center), with an optical vortex at its center in the intensity distribution of light (right). The vortex of light can carry non-zero OAM of any order m. OAM states of a different order are orthogonal. A group at the Key Laboratory of Quantum Information, Chinese Academy of Science, at the University of Science and Technology of China finally resolved this problem [8]. They reported on the first experimental realization of a true single-photon-carrying OAM stored via electromagnetically induced transparency (EIT) in a cold atomic ensemble (Fig. 2). With such a suitable candidate, this work indicates a means of constructing high-dimensional quantum memory. After this, similar results were reported by Laurat's group at Laboratoire Kastler Brossel, at Université Pierre et Marie Curie in France [9], where an extremely weak laser at single-photon level carrying OAM was also stored via EIT in a cold atomic ensemble. Ding et al. [8] first prepared two cold 85Rb atomic clouds in two magnetic-optical traps (MOT) using laser cooling and trapping techniques. They generated non-classical correlated photon pairs using spontaneous four-wave mixing in an atomic cloud. One photon of each pair was used as a trigger; the other mapped and stored in a second atomic cloud via EIT. Each photon to be stored carried one OAM unit. After a programed storage time, the photon was retrieved. What they achieved during storage included (1) proof that the non-classical correlation between the trigger photon and the retrieved photon is retained by demonstrating a strong violation of the Cauchy–Schwarz inequality, (2) a demonstration that the single-photon property of the signal photon is maintained by performing the Hanbury–Brown and Twiss experiment on the trigger photon, (3) proof that the spatial structure of the photon is also very well preserved by showing a high similarity between input and output, and (4) evidence, gathered by Sagnac interferometry, that the coherence of a single photon is also preserved. A heralded single photon is generated through spontaneous four-wave mixing in MOT 1 (a); this single photon carrying OAM is then stored through EIT in MOT 2 (b); (c) shows an image of the photon carrying OAM. Experimental measurements in the transverse position of the image carried by the photon before and after storage are presented in (d) and (e), respectively; (f) shows the simplified experimental setup for storage of a superposition of OAM. Interference patterns taken at different angle settings of the half-wave plate are shown in (g). The left column represents the experimental angle settings of the half-wave and the quarter-wave plates, the middle column gives the experimental results, and the right column gives results from theoretical simulations; (h) and (i) present the interference patterns of the input signal photon and the retrieved signal with plate angle, respectively. This is a significant breakthrough towards the realization of a quantum internet and, potentially, quantum computing. This work addresses the ability to generate, store, retrieve on demand an arbitrary single-photon-level photonic state encoded in OAM space. It signifies an important step in the development of practical quantum-enabled technologies, opens up the possibility for realizing high-dimensional quantum memories based on this degree of freedom of light, and will have a large impact in a broad physical community, especially in the quantum information and quantum optics communities. The Technology Review website of MIT comments on their work very positively with an article entitled ‘First Quantum Memory That Records the Shape of a Single Photon Unveiled in China’. Further, Nature Photonics selected this work as a research highlight. Clearly, memory that can preserve the spatial structure of photons will make the internet far more flexible and capable. Of course, there are still many basic problems remaining that need to be solved to build the future quantum internet, one of which is the construction of quantum memory exploiting entanglement. This derives from the fact that a quantum network needs the distribution of quantum-entangled photons over channels between different nodes [10]. A high-dimensional quantum internet needs to store OAM-entangled states and perform entanglement swapping to efficiently extend the achievable communication distances. While Ding et al. [8] reported the storage of light with OAM at the single-photon level, the photon was, however, still encoded in a 2D space. Therefore, whether it is possible to construct a high-dimensional quantum memory remains an open issue that needs to be investigated further.