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Nature Communications

Quantum decoherence of dark pulses in optical microresonators

Chenghao Lao, Xing Jin, Lin Chang, Heming Wang, Zhe Lv, Weiqiang Xie, Haowen Shu, Xingjun Wang, John Edward Bowers, Qi‐Fan Yang

Published Mar 31, 2023• 34 citations
Publisher

Abstract

Abstract Quantum fluctuations disrupt the cyclic motions of dissipative Kerr solitons (DKSs) in nonlinear optical microresonators and consequently cause timing jitter of the emitted pulse trains. This problem is translated to the performance of several applications that employ DKSs as compact frequency comb sources. Recently, device manufacturing and noise reduction technologies have advanced to unveil the quantum properties of DKSs. Here we investigate the quantum decoherence of DKSs existing in normal-dispersion microresonators known as dark pulses. By virtue of the very large material nonlinearity, we directly observe the quantum decoherence of dark pulses in an AlGaAs-on-insulator microresonator, and the underlying dynamical processes are resolved by injecting stochastic photons into the microresonators. Moreover, phase correlation measurements show that the uniformity of comb spacing of quantum-limited dark pulses is better than 1.2 × 10 −16 and 2.5 × 10 −13 when normalized to the optical carrier frequencies and repetition frequencies, respectively. Comparing DKSs generated in different material platforms explicitly confirms the advantages of dark pulses over bright solitons in terms of quantum-limited coherence. Our work establishes a critical performance assessment of DKSs, providing guidelines for coherence engineering of chip-scale optical frequency combs.

DOI
10.1038/s41467-023-37475-z

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Abstract Quantum fluctuations disrupt the cyclic motions of dissipative Kerr solitons (DKSs) in nonlinear optical microresonators and consequently cause timing jitter of the emitted pulse trains. This problem is translated to the performance of several applications that employ DKSs as compact frequency comb sources. Recently, device manufacturing and noise reduction technologies have advanced to unveil the quantum properties of DKSs. Here we investigate the quantum decoherence of DKSs existing in normal-dispersion microresonators known as dark pulses. By virtue of the very large material nonlinearity, we directly observe the quantum decoherence of dark pulses in an AlGaAs-on-insulator microresonator, and the underlying dynamical processes are resolved by injecting stochastic photons into the microresonators. Moreover, phase correlation measurements show that the uniformity of comb spacing of quantum-limited dark pulses is better than 1.2 × 10 −16 and 2.5 × 10 −13 when normalized to the optical carrier frequencies and repetition frequencies, respectively. Comparing DKSs generated in different material platforms explicitly confirms the advantages of dark pulses over bright solitons in terms of quantum-limited coherence. Our work establishes a critical performance assessment of DKSs, providing guidelines for coherence engineering of chip-scale optical frequency combs.
Temporal cavity solitons generated in monochromatically driven dispersive Kerr resonators offer an attractive avenue for on-chip optical frequency comb generation. Key to many of their applications is to understand how noise -- both technical and quantum -- affects the soliton states, which has accordingly been extensively investigated. Here, we report on a comprehensive theoretical study that elucidates how technical and quantum fluctuations impact a new type of soliton structure that has very recently been predicted and observed in dispersive Kerr resonators under conditions of bichromatic driving: the pure-Kerr parametrically driven cavity soliton (PDCS). We examine how classical laser phase noise transfers from the two pump fields onto the soliton frequency comb, and we calculate the solitons' fundamental quantum-limited timing jitter and two-mode squeezing spectra. In each case, we find that PDCSs can out-perform conventional cavity solitons with comparable characteristics, even when driven by two uncorrelated lasers. Our results demonstrate that pure-Kerr PDCSs can offer unprecedented performance in noise-sensitive photonic applications and as a quantum resource
Dissipative Kerr solitons in optical microresonators underpin chip-scale frequency combs with applications ranging from coherent telecommunications to precision spectroscopy. Yet the characterization of their intrinsic femtosecond temporal structure remains challenging, as the low pulse energy and broad spectral bandwidth necessitate optical amplification and careful dispersion compensation in conventional ultrafast diagnostics, both of which can significantly distort the waveform. Here we demonstrate a quantum-interference metrology of microcomb solitons based on Hong-Ou-Mandel interference. By attenuating the soliton stream to the single-photon level and measuring fourth-order interference, we directly retrieve near transform-limited pulse durations without amplification or dispersion management, remaining accurate even after propagation through 25 km of standard fiber. The same interferogram also provides direct access to the temporal separations in multi-soliton states by converting inter-soliton separations into additional interference dips at corresponding delays, enabling sub-picosecond characterization of their intracavity temporal structure. This quantum-inspired paradigm introduces a fundamentally new metrological approach that is immune to amplification and dispersion distortions, offering a powerful tool for the characterization of complex soliton physics.
While coherently driven Kerr microcavities have rapidly matured as a platform for frequency-comb formation, such microresonators generally possess weak Kerr coefficients; consequently, triggering comb generation requires millions of photons to be circulating inside the cavity. This suppresses the role of quantum fluctuations in the dynamics of the comb. In this paper, we realize a minimal version of coherently driven Kerr-mediated microwave-frequency combs in the circuit quantum electrodynamics (cQED) architecture, where the fluctuations of the quantum vacuum are the primary limitation on comb coherence. We achieve a comb phase coherence of up to 35 $\ensuremath{\mu}\mathrm{s}$, approaching the theoretical device quantum limit of 55 $\ensuremath{\mu}\mathrm{s}$ and vastly longer than the inherent lifetimes of the modes, of 13 ns. The ability within cQED to engineer stronger nonlinearities than optical microresonators, together with operation at cryogenic temperatures, and the excellent agreement of comb dynamics with quantum theory indicates a promising platform for the study of complex dynamics of quantum nonlinear systems.
Abstract In a traveling wave microresonator, the cascaded four‐wave mixing (FWM) between optical modes allows the generation of frequency combs, including intriguing dissipative Kerr solitons (DKS). This study explores the quantum fluctuations of frequency combs and reveal the continuous‐variable quantum entanglement between different comb lines of the DKS states. The entanglement of DKS exhibits two distinct characteristics. For modes located at the spectral edge with a small number of excitations, different comb modes with multiple colors become entangled due to photon‐pair generation and coherent photon conversion stimulated by the FWM. Notably, a sudden disappearance of quantum entanglement in the center of the DKS spectrum is observed, which is attributed to the self‐locking phenomena in the FWM network. These findings demonstrate the prominent quantum nature of DKS, which is of fundamental significance in quantum optics and has the potential to be utilized in quantum networking and distributed quantum sensing applications.
Soliton microcombs are self-organized pulses of light sustained in driven Kerr microresonators, intensively studied for applications in integrated photonic technologies and for their rich nonlinear dynamics. In this work, we theoretically study the collective dynamics of the quantum fluctuations of soliton microcombs. We find that the mean field of a dissipative Kerr soliton crystal is accompanied by pulses of squeezed multimode vacuum and derives its operational stability from the strong detuning of the below-threshold parametric process. We present a photonic architecture that enables independent control of the above- and below-threshold states and achieves a high degree of squeezing (>15dB) in the output waveguide with realistic losses. Our work elucidates the quantum dynamics of formation and annihilation in dissipative Kerr soliton systems, and establishes a pathway for the realization of a practical integrated source of multimode squeezed light.
Temporal cavity solitons, or dissipative Kerr solitons (DKSs) in integrated microresonators, are essential for deployable metrology technologies. Such applications favor the lowest noise state, typically the single-DKS state where one soliton is in the resonator. Other multi-DKS states can also be reached, offering better conversion efficiency and thermal stability, potentially simplifying DKS-based technologies. Yet they exhibit more noise due to relative soliton jitter and are usually not compatible with targeted applications. We demonstrate that Kerr-induced synchronization, an all-optical trapping technique, can azimuthally pin the multi-DKS state to a common reference field. This method ensures repetition rate noise is independent of the number of solitons, making a multi-DKS state indistinguishable from a single-DKS state in that regard, akin to trapped-soliton molecule behavior. Supported by theoretical analysis and experimental demonstration in an integrated microresonator, this approach provides metrological capacity regardless of the number of cavity solitons, benefiting numerous DKS-based metrology applications.