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Scientific Reports

Quantum causality emerging in a delayed-choice quantum Cheshire Cat experiment with neutrons

Richard Wagner, Wenzel Kersten, Hartmut Lemmel, Stephan Sponar, Yuji Hasegawa

Published Mar 8, 2023• 6 citations
Publisher

Abstract

We report an experiment with neutrons in a silicon perfect crystal interferometer, that realizes a quantum Cheshire Cat in a delayed choice setting. In our setup the quantum Cheshire Cat is established by spatially separating the particle and its property (i.e. the neutron and its spin) into the two different paths of the interferometer. The condition for a delayed choice setting is achieved by postponing the choice of path assignment for the quantum Cheshire Cat, i.e. which path is taken by the particle and which by its property, until the point in time when the neutron wave function has already split and entered the interferometer. The results of the experiment suggest not only the fact that the neutrons and its spin are separated and take different paths in the interferometer, but also quantum-mechanical causality is implied, insomuch that the behavior of a quantum system is affected by the choice of the selection at a later point in time.

DOI
10.1038/s41598-023-29970-6

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We report an experiment with neutrons in a silicon perfect crystal interferometer, that realizes a quantum Cheshire Cat in a delayed choice setting. In our setup the quantum Cheshire Cat is established by spatially separating the particle and its property (i.e. the neutron and its spin) into the two different paths of the interferometer. The condition for a delayed choice setting is achieved by postponing the choice of path assignment for the quantum Cheshire Cat, i.e. which path is taken by the particle and which by its property, until the point in time when the neutron wave function has already split and entered the interferometer. The results of the experiment suggest not only the fact that the neutrons and its spin are separated and take different paths in the interferometer, but also quantum-mechanical causality is implied, insomuch that the behavior of a quantum system is affected by the choice of the selection at a later point in time.
From its very beginning, quantum theory has been revealing extraordinary and counter-intuitive phenomena, such as wave-particle duality, Schrödinger cats and quantum non-locality. Another paradoxical phenomenon found within the framework of quantum mechanics is the 'quantum Cheshire Cat': if a quantum system is subject to a certain pre- and postselection, it can behave as if a particle and its property are spatially separated. It has been suggested to employ weak measurements in order to explore the Cheshire Cat's nature. Here we report an experiment in which we send neutrons through a perfect silicon crystal interferometer and perform weak measurements to probe the location of the particle and its magnetic moment. The experimental results suggest that the system behaves as if the neutrons go through one beam path, while their magnetic moment travels along the other.
Abstract Although our every-day experience rejects it, the quantum Cheshire Cat suggests a potential spatial separation between different properties of a single particle in an interferometer. The first experiment with neutrons confirmed the quantum Cheshire Cat effect by using the path and spin degrees of freedom. The locations of each property are determined qualitatively through reactions to locally applied perturbations. Yet, no consensus on the interpretation has been reached. To clarify the origin of the effect, in the present experiment the energy degree of freedom is used as the third property; the three properties of neutrons appear to be separated in different paths in the interferometer. The analysis of the experiment suggests the strong involvement of the inner product between the state vectors, one evolved from the initial state through the perturbation and the other being the final state. The inner product results in amplitudes from two sub-beams which contribute to the intensity. The cross-term between amplitudes gives rise to the quantum Cheshire Cat.
Quantum theory provides us with the best account of microscopic components of matter as well as of radiation. It was introduced in the twentieth century and has experienced a wide range of success. Although the theory’s probabilistic predictions of final experimental outcomes is found to be correct with high precision, there is no general consensus regarding what is actually going on with a quantum system “en route”, or rather the perceivable intermediate behavior of a quantum system, e.g., the particle’s behavior in the double-slit experiment. Neutron interferometry using single silicon perfect crystals is established as a versatile tool to test fundamental phenomena in quantum mechanics, where an incident neutron beam is coherently split in two or three beam paths with macroscopic separation of several centimeters. Here, we present quantum optical experiments with these matter-wave interferometers, studying the effect of the quantum Cheshire Cat in some variants, the neutron’s presence in the paths of the interferometer as well as the direct test of a commutation relation. To reduce disturbances induced by the measurement, the interaction strength is lessened and so-called weak interactions are exploited by employing pre- and post-selection procedures. All results of the experiments confirm the predictions of quantum theory; the observed behaviors of the neutron between the pre- and post-selection in space and time emphasize striking and counter-intuitive aspects of quantum theory.
The quantum Cheshire cat effect is an important phenomenon in quantum mechanics that reveals the separability of physical properties from their carriers. This effect transcends the classical framework whose attributes must be inherently attached to objects, providing new perspectives for quantum information and precision measurement. According to the quantum Cheshire cat effect, we prepare a pre-selected state of a spin-1/2 atomic system composed of two particles through a pre-selection process. We conduct quantum weak measurements on the spins and positions of these two atoms and extract weak values by using the method of imaginary time evolution (ITE). Subsequently, we perform post-selection on these two atoms and design two distinct post-selected states. Initially, we calculate analytical solutions when both atoms encounter these two different post-selected states separately. Then, during the stage of obtaining weak values via ITE, we first discuss the scenario with only one post-selected state. In this case, our experimental goal is to achieve spin exchange between the two atoms. We use ITE to obtain normalized coincidence rate for the system. By linearly fitting these normalized coincidence rate, we derive numerical solutions for the weak values of the system. The comparison between the analytical solutions and numerical results indicates that they are in close agreement, demonstrating that our method promotes spin exchange between the two atoms. Next, we examine scenarios involving both post-selected states in the post-selection process. After completing weak measurements on particles, delayed-choice allows them to evolve along different paths ultimately leading to distinct post-selected states. One particular post-selected state that results in final measurement outcomes indicates that the spin exchange occurs between both particles with amplification. Conversely, the other post-selected state ensures that even after undergoing weak measurement and delayed-choice, the states of the two particles remain consistent with their pre-measurement conditions. We also compare the analytical and numerical solutions of the experiment involving delayed choice and find that they are very consistent with each other. This consistency indicates that delayed-choice indeed has a significant influence on whether the final exchange occurs. Our research theoretically confirms the feasibility of fermionic systems within bipartite quantum Cheshire cat effects and illustrates how delayed-choice influences quantum Cheshire cat effects in spin-1/2 atomic systems.
The so-called quantum Cheshire Cat is a scenario where a photon, identified with a cat, and a component of its polarization, identified with the grin of that cat, are separated. We observe that the same techniques can be used to separate two orthogonal components of polarization of a photon, on an average. We identify these polarization components of the photon as the grin and snarl of the cat for ease of comprehension. A gedanken experiment is presented in which we simultaneously tune the input polarizations of the photon in the two arms of a Mach-Zehnder interferometer. It is noted that for two particular choices of photon polarization, the presence of the two components gets reversed in the two arms. This reversal of the grin and the snarl occurs before the polarization components even interact with the tuners, i.e., before the choice of which arm each should be in is made.
Fundamental phenomena in quantum mechanics are investigated by the use of matter-wave optics: in the studies neutron polarimeter and interferometer are exploited. Successive measurements of 1/2-spin of the neutron are carried out to test the error-disturbance uncertainty relation. The experimental results confirm the violation of Heisenberg's original reciprocal relation for measurement error and disturbance, and the validity of the reformulated generally valid relation. In addition, as an example of a counterfactual phenomenon of quantum mechanics, interferometric experiment is performed to observe the so-called quantum Cheshire-Cat: a particle and its magnetic moment travel through the interferometer along different beam paths. The results of our experiment suggest that, with suitable pre- and post-selections, neutrons travel along one of the arms of the interferometer, while their spin is located in the other arm.