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Topical Meeting on Optical Bistability (OB)

Optical Bistability with Two-State Atoms: Steady States and Dynamical Instabilities

Harry J. Kimble, Albert T. Rosenberger, Luis A. Orozco, M. S. Raizen

Published Jan 1, 1985• 1 citation
Publisher

Abstract

Beams of homogeneously broadened two-state sodium atoms in a confocal ring resonator have been employed to investigate the steady-state characteristics of absorptive [1] and dispersive optical bistability. Also studied in the same system is the dynamical behavior due to the intrinsic single-longitudinal-mode instability [2] originating in the alteration of the atomic absorption profile by a strong field as in the Lorenz-type instability in the homogeneously broadened laser. All experimental parameters are carefully measured and corrected for transit broadening, finite absorption, and residual Doppler broadening in order to be able to make an absolute comparison with the single-Gaussian-transverse-mode theory [3-6]. Despite the frequency degeneracy of the transverse modes of the resonator, the agreement with this theory for absorptive bistability is remarkably good. The dispersive bistability data are more difficult to interpret, but they seem to be in reasonable agreement with the theory; the same can be said of the results for the domain and oscillation frequency of the instability, at least within a certain region of parameter space. Outside this region, multiple unstable states appear for various intracavity intensities; recent observations suggest that these may be due in part to instabilities involving higher-order transverse modes of the resonator.

DOI
10.1364/obi.1985.we2

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Beams of homogeneously broadened two-state sodium atoms in a confocal ring resonator have been employed to investigate the steady-state characteristics of absorptive [1] and dispersive optical bistability. Also studied in the same system is the dynamical behavior due to the intrinsic single-longitudinal-mode instability [2] originating in the alteration of the atomic absorption profile by a strong field as in the Lorenz-type instability in the homogeneously broadened laser. All experimental parameters are carefully measured and corrected for transit broadening, finite absorption, and residual Doppler broadening in order to be able to make an absolute comparison with the single-Gaussian-transverse-mode theory [3-6]. Despite the frequency degeneracy of the transverse modes of the resonator, the agreement with this theory for absorptive bistability is remarkably good. The dispersive bistability data are more difficult to interpret, but they seem to be in reasonable agreement with the theory; the same can be said of the results for the domain and oscillation frequency of the instability, at least within a certain region of parameter space. Outside this region, multiple unstable states appear for various intracavity intensities; recent observations suggest that these may be due in part to instabilities involving higher-order transverse modes of the resonator.
Absolute quantitative comparisons between experiment and theory are reported for the steady-state characteristics of optical bistability with two-state atoms in ring and in standing-wave resonators. The case treated here is the absorptive one, with both atoms and cavity resonant with the field. The experiment is designed to realize as closely as possible a standard theoretical model of two-state atoms interacting with a single mode of the electromagnetic field in a resonator and is described in detail. A detailed explanation is also given of the extensions to the standard theory that are needed to account for unavoidable experimental limitations such as transit broadening and the nonideal nature of the resonator. The good agreement observed between experiment and theory provides a foundation for quantitative investigation of nonlinear dynamics and quantum phenomena in this nonequilibrium optical system.
In this paper we analyze the steady-state and stability properties of bistable optical systems, lasers with an injected signal, and ordinary free-running lasers. The starting point of our study is a unified model of a ring cavity containing a finite-size cylindrical sample of homogeneously broadened two-level atoms, and capable of supporting a single field mode with a Gaussian transverse profile. After solving the equations of motion in the steady state, we carry out a linear stability analysis of the stationary solutions, identify the domains of unstable operation of each of the three systems, and compare in detail the results of this work with those of earlier plane-wave uniform-field calculations. In the case of the laser with an injected signal, we find a significant enhancement of the instability domain relative to the plane-wave limit. A similar conclusion holds for mixed absorptive and dispersive optical bistability, although the enhancement of the domain of instability is less pronounced. Unstable behavior is predicted to occur for experimentally accessible values of the bistability parameter, and to be favored by the absence of bistability and by the selection of atomic and cavity detunings having opposite signs. This configuration ensures that the instability will be responsible for the emergence of undamped output pulsations of the type that will make the bistable system behave as an optical clock.
In nonlinear optical interactions, one expects the transverse spatial intensity dependence to be modified. Nonlinear interactions within an optical resonator, in the absence of a mode-selective element such as an aperture, will thus in general couple the energy into various transverse modes of the resonator. One attractive analytical model incorporating transverse effects into optical bistability assumes, in spite of the observations above, that the transverse intensity profile remains a single-Gaussian (TEM00) mode. This model seems to be supported by experimental results for bistability with two-level sodium atoms in a confocal ring resonator. To test the generality of the single-Gaussian mode model, we have performed bistability experiments with two-level atoms in standing-wave resonators. Two resonators, differing only in length, were used. The confocal resonator is transverse-mode-degenerate and will support a combination of modes, as would the ring; the slightly longer resonator will allow only a single-transverse mode to be excited. Preliminary results indicate that there may be a difference in the two cases; although the behavior near the critical onset of bistability seems to be the same in the two cases, there seems to be a difference in the evolution of hysteresis with increasing cooperativity parameter. Further results, including a quantitative comparison with the single-Gaussian mode theory for standing-wave resonators, are presented.
Observations of steady-state hysteresis in absorptive bistability are reported for well-collimated atomic beams of sodium within a traveling-wave interferometer. The atomic medium approximates a system of homogeneously broadened "two-level" atoms, and effects due to standing waves are eliminated. The experiment thus represents the first demonstration of optical bistability under conditions that have been widely employed in theoretical models. Absolute measurements of switching intensities versus atomic cooperativity CCC are reported, and a preliminary comparison with Gaussian-beam theory is made.
This paper gives a detailed description of the plane-wave Gaussian models of optical bistability and of the experimental investigations of the single-mode instability induced on a beam of sodium atoms in a cavity by an external driving field. Our goal is to provide a careful comparison of the theoretical and experimental results. We focus on the shape of the instability domain, the nature and behavior of the spontaneous output oscillations produced by the instability, and their frequency dependence on the control parameters. We carry out this comparison using both the plane-wave and Gaussian models. Our analysis shows that the latter is in good quantitative agreement with the experimental results. We investigate in detail the main assumption of the Gaussian model, namely, that the internal cavity field retains the same radial profile as the input field.