The domain of the third-order theory of the single-mode laser is usually defined by the condition nB/A ≪ 1, where n is the photon number in the cavity, and A and B are the gain and saturation coefficients. When the laser cavity is detuned from line center by Δω ≡ ηγ, where γ is the natural linewidth of the atomic transition, A and B change in the prescribed manner given by the Lamb theory, and it is usually taken for granted that the theory is valid both for small and large detunings η. By examining the relationships between various parameters we show that the limits on the domain of the third-order laser theory effectively limit the allowed detuning in many common lasers to one natural linewidth (η ≈ 1).
The domain of the third-order theory of the single-mode laser is usually defined by the condition nB/A ≪ 1, where n is the photon number in the cavity, and A and B are the gain and saturation coefficients. When the laser cavity is detuned from line center by Δω ≡ ηγ, where γ is the natural linewidth of the atomic transition, A and B change in the prescribed manner given by the Lamb theory, and it is usually taken for granted that the theory is valid both for small and large detunings η. By examining the relationships between various parameters we show that the limits on the domain of the third-order laser theory effectively limit the allowed detuning in many common lasers to one natural linewidth (η ≈ 1).
Essentially closed-form formulae are given for the linewidth of inhomogeneously broadened lasers, with arbitrary cavity detuning and pumping statistics (Poissonian or quiet pumps). The so-called `bad-cavity' mode of operation is treated. The general formula is obtained from a semiclassical theory first derived from a linearized symmetrically ordered quantum theory in the limit of a large number of atoms. This semiclassical theory is most easily explained in terms of independent quantum jumps performed by emitting and absorbing atoms. The effect of inhomogeneous broadening on linewidth is found to be negligible for some pumping schemes, but when the atoms are independently pumped the linewidth is proportional (at some constant power level) to the gain-medium spectral width. We consider, in particular, an intermediate situation in which the rate at which atoms are promoted from the lower to the upper level (pump rate) is proportional to the lower-state population for each atom class. For that particular model, pump fluctuations do not affect the linewidth, even when the cavity is detuned from the centre of the atomic transition frequency distribution.
It is very important to understand the characteristics of gain saturation for homogeneously broadened laser medium. Assuming a Lorentzian lineshape function with a linewidth of ΔνH, we have derived the analytical functions of the gain coefficient under three different conditions: 1) a small and 2) a large signal incident on the medium respectively, and 3) a small signal accompanied by a large signal simultaneously incident on the medium. We have found that the bandwidth Δν of the gain coefficient is equal to the linewidth ΔνH for condition 1) and 3) while it is Δ ν = 1 + I ν 1 / I s Δ ν H for condition 2). Here, I v 1 and Is are the intensity of the large signal and the saturation intensity at the center frequency Vo, respectively. The reasons are also presented for such results. For condition 2), gain saturation effect is strongly dependent on the frequency of the large signal: the more the frequency deviates from the center frequency, the weaker the gain saturation effect. This results an increase of the bandwidth. For condition 3), the intensity of the large signal only changes the distribution of populations on the upper and lower energy levels. Hence, the shape of the gain coefficient does not change with the gain reduction of the small signal, thus, its bandwidth remains the same.
The quantum theory of a laser developed by Scully and Lamb (1967) is reformulated to include the effects of atomic motion and detuning. The equations are solved to fourth order in the atom-field coupling constant. An approximate treatment of the mode structure is shown to reproduce the results of Lamb's semi-classical theory in the Doppler limit. In addition the photon distribution may be studied as a function of the detuning. The width of the photon distribution is found to increase monotonically with increasing detuning.
It is very important to understand the characteristics of gain saturation for homogeneously broadened laser medium. Assuming a Lorentzian lineshape function with a linewidth of ΔνH, we have derived the analytical functions of the gain coefficient under three different conditions: 1) a small and 2) a large signal incident on the medium respectively, and 3) a small signal accompanied by a large signal simultaneously incident on the medium. We have found that the bandwidth Δν of the gain coefficient is equal to the linewidth ΔνH for condition 1) and 3) while it is Δν = √1+Iν1 / IsΔνH for condition 2). Here, Iν1 and Is are the intensity of the large signal and the saturation intensity at the center frequency ν0, respectively. The reasons are also presented for such results. For condition 2), gain saturation effect is strongly dependent on the frequency of the large signal: the more the frequency deviates from the center frequency, the weaker the gain saturation effect. This results an increase of the bandwidth. For condition 3), the intensity of the large signal only changes the distribution of populations on the upper and lower energy levels. Hence, the shape of the gain coefficient does not change with the gain reduction of the small signal, thus, its bandwidth remains the same.
Up to this point we have always assumed that all the atoms which interact with the radiation field have the same atomic transition frequency, with an atomic linewidth given by γ ⊥ . This configuration is called homogeneous broadening. However, in the great majority of lasers the linewidth is inhomogeneously broadened , because the atomic frequency follows a distribution. For example, in solid-state lasers such as the ruby laser and fiber lasers the inhomogeneity is due to the imperfections in the crystalline structure of the material. In gas lasers, where the atoms or molecules are free to move, the inhomogeneous broadening is due to the Doppler effect, for which a molecule moving with velocity v in a field of frequency ω and wave vector k experiences an effective frequency ω ′ = ω − k · v [8]. Since what matters is the difference between the atomic transition frequency and the field frequency, we can keep the field frequency fixed and imagine that the field interacts with different groups of atoms that move with different velocities and therefore have different transition frequencies. The realistic velocity distribution is a Gaussian, for which the corresponding distribution for the modulus of the velocity is Maxwellian. However, in the following we will mainly analyze the case of a Lorentzian distribution for the atomic transition frequency, because this allows an analytical treatment. Again for the sake of simplicity, we will limit our analysis to the case of a ring cavity. In Section 15.1 we will generalize to the inhomogeneous-broadening configuration the modal equations for the case of homogeneous broadening, which were formulated in Chapter 12. In Section 15.2 we will specialize to the single-mode model and discuss its stationary solutions for the laser case. Multimode dynamical equations The atomic transition frequency of the generic group of atoms is given by ω a + δ D , where ω a is the central atomic frequency and δ D takes positive and negative values. We call ω c the frequency of the cavity mode nearest to ω a and denote by δ ac the difference ω a − ω c .
The Lamb theory of the optical maser is extended to fifth and higher orders in the perturbation by the time-dependent iteration method, and by a rate-constant approach obtained by removing the time dependence in the Hamiltonian with a unitary transformation. The third- and fifth-order Fourier projections of the atomic polarization are integrated exactly over the atomic velocity distribution, assumed Maxwellian, and the results are then valid for any ratio of natural linewidth, or cavity detuning, to the Doppler width. Dominant fifth-order terms occur whose variation with cavity detuning depends only on the natural line-width of the transition. These produce an increase in laser intensity versus cavity detuning, including a reduction of the dip phenomena, and are effective at low levels of laser excitation. In addition, third-order and numerous fifth-order terms occur which involve sharper resonances near line center because of Doppler interference effects. Such terms involve the individual decay constants of the states in a complicated way. Owing to cancellation effects, the totality of such terms is in general small compared with the usual saturation term and the dominant fifth-order contributions. This considerably simplifies the deduction of higher-order perturbation terms. Collision processes would also reduce their effect as a result of their higher-order atomic response functions, but the theory is reasonably consistent with present experimental characteristics even without this possibility. The rate-constant approach facilitates the deduction of the various higher-order perturbation results and would be of even greater utility in discussing the Zeeman laser, particularly for axial magnetic fields and complicated transitions.