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Annual Meeting Optical Society of America

Measurement of the instability threshold in Brillouin enhanced four-wave mixing

David E. Watkins, A. M. Scott, Kevin D. Ridley

Published Jan 1, 1989• 0 citations

Abstract

Four-wave mixing mediated by Brillouin scattering in the transient regime exhibits an instability which results in large phase conjugate reflectivities [A. M. Scott and K. D. Ridley, IEEE J Quantum Electron. QE-25, 438 (1989)]. In this paper we compare measurements of the threshold for the instability both as a function of the ratio of the second pump beam to the first pump beam and as a function of the phase mismatch. Phase conjugation in Brillouin enhanced four-wave mixing occurs through the interaction of a signal with two counterpropagating pump beams. In our experiments, the frequencies of all three input beams are different, and a small phase mismatch results. The magnitude of this mismatch was varied both by changing one of the input frequencies and the interaction length. The frequency of the second pump beam was changed by using stimulated Brillouin scattering in various mixtures. Thus we were able to vary the phase mismatch from four to thirteen resulting in a 50% change in the threshold intensity, in agreement with theoretical models. The ratio of the backward-to-forward pump beam intensities also affects the threshold, and measurements of this agree with the model.

DOI: 10.1364/oam.1989.tua2

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Four-wave mixing mediated by Brillouin scattering in the transient regime exhibits an instability which results in large phase conjugate reflectivities [A. M. Scott and K. D. Ridley, IEEE J Quantum Electron. QE-25, 438 (1989)]. In this paper we compare measurements of the threshold for the instability both as a function of the ratio of the second pump beam to the first pump beam and as a function of the phase mismatch. Phase conjugation in Brillouin enhanced four-wave mixing occurs through the interaction of a signal with two counterpropagating pump beams. In our experiments, the frequencies of all three input beams are different, and a small phase mismatch results. The magnitude of this mismatch was varied both by changing one of the input frequencies and the interaction length. The frequency of the second pump beam was changed by using stimulated Brillouin scattering in various mixtures. Thus we were able to vary the phase mismatch from four to thirteen resulting in a 50% change in the threshold intensity, in agreement with theoretical models. The ratio of the backward-to-forward pump beam intensities also affects the threshold, and measurements of this agree with the model.

We report on a theoretical and modeling study of self-pumped four-wave mixing in a Brillouin medium. A theoretical analysis gives expressions for the threshold intensity and for the steady-state reflectivity at small input intensities. Operation over a range of input intensities is also investigated by using a computer model that predicts that, for high input intensities, the conjugate can become unstable and oscillate chaotically in time. Experimentally we observe phase conjugation with an input threshold 25 times less than that required for phase conjugation by stimulated Brillouin scattering.

It has previously been shown that Brillouin enhanced four-wave mixing can lead to large phase conjugate reflectivities for moderate laser powers.1,2 However, in the geometry considered by previous workers the pumps have equal frequency and hence the conjugate signal is shifted in frequency with respect to the probe. We have conducted an experimental and theoretical study of Brillouin-enhanced four-wave mixing for the different case in which the two pump waves differ in frequency by twice the Brillouin frequency of the four-wave mixing medium, and in which the probe wave frequency is halfway between those of the pump waves. In this case, the phase conjugate wave has the same frequency as the probe. Reflectivities > 100 % have been measured. Experimental results are compared to those of a theory that includes the effects of phase mismatch, pump depletion, and the finite response time of the medium.

We report on an investigation of Brillouin-enhanced four-wave mixing which provides phase conjugate reflectivities greater than 104. Theoretical modeling shows that the phase conjugate intensity grows with time until limited by pump depletion, and the main effect of varying the signal power is to increase the time delay before the conjugate beam reaches peak intensity. This is confirmed experimentally, and the maximum peak reflectivity is limited by the length of the laser pulses used in the experiment.

The results of an experimental investigation of a new geometry for producing phase conjugation by Brillouin-enhanced four-wave mixing are presented. In this geometry, the four-wave mixing medium is carbon disulfide, and the backward-going pump wave is created from the transmitted forward-going pump wave by stimulated Brillouin scattering (SBS) in glycerol. The two pump waves are hence phase conjugates of each other, and the quality of the phase-conjugation process is not degraded even by the use of an aberrated pump wave. The probe wave is created by SBS in carbon disulfide, which has a Brillouin frequency half that of glycerol, and the conjugate wave is therefore generated at the same frequency as the probe. Since the pump and signal waves differ in frequency by the Brillouin frequency of the carbon disulfide four-wave mixing medium, high reflectivities (approximately 2000%) are obtained as a result of Brillouin resonance enhancement.

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