Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Annual Meeting Optical Society of America

Polarization properties of degenerate four-wave mixing in a medium of rigidly held dye molecules

Wayne R. Tompkin, Michelle S. Malcuit, Robert W. Boyd

Published Jan 1, 1989• 0 citations
Publisher

Abstract

Rigidly held molecules display nonlinear optical properties which differ substantially from the properties of isotropic absorbers.1 In particular, the absorption of a collection of randomly oriented, rigidly held molecules saturates differently for different polarization states. We show that the polarization properties of degenerate four-wave mixing in such a medium are dramatically modified by this polarization-dependent saturation. We predict theoretically that for linearly polarized pump waves and for an input intensity near the saturation intensity, degenerate four-wave mixing in this material system can lead directly to vector phase conjugation; that is, to the simultaneous reversal of the optical wavefront and conjugation of the polarization state of the incident optical field.2 We confirm these theoretical predictions through phase conjugation experiments using fluorescein doped boric acid glass as the material system, and we find that degenerate four-wave mixing leads to nearly perfect vector phase conjugation when pumped by linearly polarized pump waves for field strengths near the saturation intensity.

DOI
10.1364/oam.1989.tua5

Related papers

Polarization properties of phase conjugation by degenerate four-wave mixing in a medium of rigidly held dye molecules

Wayne R. Tompkin, John E. Sipe, Michelle S. Malcuit +1 more

The saturation properties of dye molecules that are rigidly held in a solid host are qualitatively different from those of molecules that are free to rotate. We have found that these unique saturation characteristics can be exploited to achieve nearly perfect vector phase conjugation for field strengths near the saturation intensity. We have studied these properties experimentally by using fluorescein-doped boric acid glass as the nonlinear-optical material.

Journal of the Optical Society of America B•Apr 1, 1989•34 citations

Polarization-dependent phase-conjugate reflectivity in randomly oriented saturable absorbers

Shigeki Miyanaga, Kazuo Nakagawa, Hirofumi Fujiwara

Polarization dependence of phase-conjugate reflectivity by degenerate four-wave mixing is clarified theoretically and experimentally in a saturable-dye-doped polymer film. 1. _INTRODUCTLON A dyedoped film in which optically anisotropic saturable dye molecules are rigidly fixed and are randomly oriented has been used as a nonlinear material which can generate a phase-conjugate (PC) wave by degenerate four-wave mixing13 (DFWM). Such a film can generate a PC wave which has the same polarization state as the probe wave even for a probe wave orthogonally polarized to two pump waves. Tompkin et. al. 4 showed that in such a phase conjugator the nearly perfect vectorial phase conjugation can be obtained at the pump intensity near the saturation intensity of the phase conjugator. In this work following the analysis of Tompkin et. al. 4 closed-form solutions for the PC reflectivities in the dye-doped film are derived for two states of the polarization: the probe wave is polarized parallel and perpendicular to the pump waves. Some experimental results are also demonstrated in an eosin-Y-doped poly-vinyl alcohol (PVA) film and are compared with the theoretical results. 2. POLARIZATION DEPENDENT PC REFLECTIVITIES Dye molecules are modeled as dipoles which are randomly and uniformly oriented and are rigidly fixed in a solid matrix. We assume that each dye molecule has only one component of transition dipole moments at a wavelength considered5. An induced dipole moment of each dye molecule by

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jul 1, 1990•5 citations

Polarization dependence of phase-conjugate reflectivities in solid films containing randomly oriented saturable dyes

T. Sato, Shigeki Miyanaga

The properties of polarization-dependent phase-conjugate (PC) reflectivities by degenerate four-wave mixing in saturable-dye-doped films are investigated on the basis of a four-level model including an excited-state absorption. Numerical calculations are carried out by taking account of the effect of molecular orientation as well as of pump propagation under the assumption that optically anisotropic dye molecules are rigidly fixed in a solid matrix without any positional and orientational order, in which a PC wave can be generated even in the case of a probe wave perpendicularly polarized to pump waves. Two cases of the polarization state are employed, where the polarization direction of the probe wave is either parallel or perpendicular to that of the parallel linearly polarized pump waves. Numerically calculating the PC reflectivities as a function of the pump intensity, we show how the polarization properties of the PC-reflectivity curves depend on saturation parameters, and clarify the influences of the molecular orientational and the pump propagation effect. The numerical results are compared with the experimental results obtained by using eosin-Y-doped polyvinyl alcohol films as saturable absorbers.

IEEE Journal of Quantum Electronics•Jan 1, 1999•3 citations

Polarization Properties Of Phase Conjugation By Degenerate Four-Wave Mixing In Saturable Absorbers

Robert W. Boyd, Daniel J. Gauthier, Martti Olavi Kauranen +2 more

Dye molecules held rigidly in solid hosts display unusual polarization properties that can be exploited to produce nearly perfect vector phase conjugation with high sensitivity.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Aug 8, 1989•1 citation

Vector phase conjugation by two-photon-resonant degenerate four-wave mixing

Michelle S. Malcuit, Daniel J. Gauthier, Robert W. Boyd

We have studied the polarization properties of phase conjugation by degenerate four-wave mixing resonantly enhanced by the sodium 3S1/2 → 6S1/2 two-photon-allowed transition. As predicted by third-order theories, this interaction leads to simultaneous conjugation of the optical wave front and state of polarization (vector phase conjugation) when the pump intensities are sufficiently weak. However, qualitatively different polarization behavior is observed for pump intensities near or above the two-photon saturation intensity.

Optics Letters•Aug 1, 1988•23 citations

Polarization Properties of Nonlinear Optical Materials

Michelle S. Malcuit, Robert W. Boyd, Daniel J. Gauthier +2 more

Nonlinear optical interactions can depend in a complicated manner on the state of polarization of the incident optical waves. For the case of isotropic nonlinear optical materials, the third order nonlinear polarization is expressed in terms of two parameters A and B describing the material system and can be written as1,2 (1) where E → is the total field incident upon the medium. In this paper we present the results of investigations of the polarization properties of phase conjugation by degenerate four-wave mixing (DFWM) in fluorescein-doped boric acid glass and in sodium vapor utilizing the 3S1/2→6S1/2 two-photon allowed transition. We find that these two materials can be used for a vector phase conjugation. Vector phase conjugation (VPC) corrects for both wavefront and polarization distortions upon double pass through an aberrating medium.3

Nonlinear Optical Properties of Materials•Jan 1, 1988•0 citations
Rigidly held molecules display nonlinear optical properties which differ substantially from the properties of isotropic absorbers.1 In particular, the absorption of a collection of randomly oriented, rigidly held molecules saturates differently for different polarization states. We show that the polarization properties of degenerate four-wave mixing in such a medium are dramatically modified by this polarization-dependent saturation. We predict theoretically that for linearly polarized pump waves and for an input intensity near the saturation intensity, degenerate four-wave mixing in this material system can lead directly to vector phase conjugation; that is, to the simultaneous reversal of the optical wavefront and conjugation of the polarization state of the incident optical field.2 We confirm these theoretical predictions through phase conjugation experiments using fluorescein doped boric acid glass as the material system, and we find that degenerate four-wave mixing leads to nearly perfect vector phase conjugation when pumped by linearly polarized pump waves for field strengths near the saturation intensity.
Polarization dependence of phase-conjugate reflectivity by degenerate four-wave mixing is clarified theoretically and experimentally in a saturable-dye-doped polymer film. 1. _INTRODUCTLON A dyedoped film in which optically anisotropic saturable dye molecules are rigidly fixed and are randomly oriented has been used as a nonlinear material which can generate a phase-conjugate (PC) wave by degenerate four-wave mixing13 (DFWM). Such a film can generate a PC wave which has the same polarization state as the probe wave even for a probe wave orthogonally polarized to two pump waves. Tompkin et. al. 4 showed that in such a phase conjugator the nearly perfect vectorial phase conjugation can be obtained at the pump intensity near the saturation intensity of the phase conjugator. In this work following the analysis of Tompkin et. al. 4 closed-form solutions for the PC reflectivities in the dye-doped film are derived for two states of the polarization: the probe wave is polarized parallel and perpendicular to the pump waves. Some experimental results are also demonstrated in an eosin-Y-doped poly-vinyl alcohol (PVA) film and are compared with the theoretical results. 2. POLARIZATION DEPENDENT PC REFLECTIVITIES Dye molecules are modeled as dipoles which are randomly and uniformly oriented and are rigidly fixed in a solid matrix. We assume that each dye molecule has only one component of transition dipole moments at a wavelength considered5. An induced dipole moment of each dye molecule by
The properties of polarization-dependent phase-conjugate (PC) reflectivities by degenerate four-wave mixing in saturable-dye-doped films are investigated on the basis of a four-level model including an excited-state absorption. Numerical calculations are carried out by taking account of the effect of molecular orientation as well as of pump propagation under the assumption that optically anisotropic dye molecules are rigidly fixed in a solid matrix without any positional and orientational order, in which a PC wave can be generated even in the case of a probe wave perpendicularly polarized to pump waves. Two cases of the polarization state are employed, where the polarization direction of the probe wave is either parallel or perpendicular to that of the parallel linearly polarized pump waves. Numerically calculating the PC reflectivities as a function of the pump intensity, we show how the polarization properties of the PC-reflectivity curves depend on saturation parameters, and clarify the influences of the molecular orientational and the pump propagation effect. The numerical results are compared with the experimental results obtained by using eosin-Y-doped polyvinyl alcohol films as saturable absorbers.
We have studied the polarization properties of phase conjugation by degenerate four-wave mixing resonantly enhanced by the sodium 3S1/2 → 6S1/2 two-photon-allowed transition. As predicted by third-order theories, this interaction leads to simultaneous conjugation of the optical wave front and state of polarization (vector phase conjugation) when the pump intensities are sufficiently weak. However, qualitatively different polarization behavior is observed for pump intensities near or above the two-photon saturation intensity.
Nonlinear optical interactions can depend in a complicated manner on the state of polarization of the incident optical waves. For the case of isotropic nonlinear optical materials, the third order nonlinear polarization is expressed in terms of two parameters A and B describing the material system and can be written as1,2 (1) where E → is the total field incident upon the medium. In this paper we present the results of investigations of the polarization properties of phase conjugation by degenerate four-wave mixing (DFWM) in fluorescein-doped boric acid glass and in sodium vapor utilizing the 3S1/2→6S1/2 two-photon allowed transition. We find that these two materials can be used for a vector phase conjugation. Vector phase conjugation (VPC) corrects for both wavefront and polarization distortions upon double pass through an aberrating medium.3