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Annual Meeting Optical Society of America

Quantum beats from separated atoms excited by correlated photons

Mark P. Silverman

Published Jan 1, 1990• 0 citations
Publisher

Abstract

Entangled multiparticle quantum states cannot be expressed as a product of singleparticle states; they can give rise to correlations between separated particles unaccountable within the framework of classical physics and are of considerable interest to those concerned with the foundations of quantum mechanics. Two separated identical atoms having, for example, two excited levels with energy interval h12 are brought into an entangled linear superposition of excited states by absorption of two correlated photons. The quantum description of either atom alone shows incoherently populated excited states; the single-atom emission probability shows no quantum interference. However, the joint probability for fluorescent emission manifests, as a function of the time interval between radiative decay of both atoms, quantum beats1 at frequency 12. This quantum interference is insensitive to atomic motion and atomic density, and it can be engendered by photons whose spectral widths are smaller than the beat frequency.

DOI
10.1364/oam.1990.tuv6

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Entangled multiparticle quantum states cannot be expressed as a product of singleparticle states; they can give rise to correlations between separated particles unaccountable within the framework of classical physics and are of considerable interest to those concerned with the foundations of quantum mechanics. Two separated identical atoms having, for example, two excited levels with energy interval h12 are brought into an entangled linear superposition of excited states by absorption of two correlated photons. The quantum description of either atom alone shows incoherently populated excited states; the single-atom emission probability shows no quantum interference. However, the joint probability for fluorescent emission manifests, as a function of the time interval between radiative decay of both atoms, quantum beats1 at frequency 12. This quantum interference is insensitive to atomic motion and atomic density, and it can be engendered by photons whose spectral widths are smaller than the beat frequency.
The appearance of quantum beats in a two-time second-order correlation function is discussed for the case of spontaneous emission from two nonidentical atoms. The atoms are separated by distances comparable with the resonance wavelength and have different transition frequencies and natural line widths. It is shown that quantum beats appear for nonidentical and identical atoms. In the latter case the dipole–dipole interaction between the atoms is a necessary condition for the appearance of quantum beats. Two mechanisms lead to quantum beats in the case of nonidentical atoms and such beats may appear even for independent atoms. The effect is similar to that of interference between independent beams.
The interference of two single photons impinging on a beam splitter is measured in a time-resolved manner. Using long photons of different frequencies emitted from an atom-cavity system, a quantum beat with a visibility close to 100% is observed in the correlation between the photodetections at the output ports of the beam splitter. The time dependence of the beat amplitude reflects the coherence properties of the photons. Most remarkably, simultaneous photodetections are never observed, so that a temporal filter allows one to obtain perfect two-photon coalescence even for nonperfect photons.
In photodissociation of a homonuclear diatomic molecule, conservation of linear and angular momenta requires that each atomic fragment follow identical but oppositely directed trajectories with respect to the molecular center of mass. For certain values of the incident photon energy, one of the atoms will be electronically excited while the other will be in its ground state. When a detector records the undispersed fluorescence from the decay of the excited atom it cannot distinguish which trajectory the excited atom followed and hence whether the photon possesses a blue or red Doppler shift corresponding to recoil towards or away from the detector. According to the principle of superposition in quantum mechanics, the wave function of the photon must be a sum over two paths corresponding to emission from an excited atom in either of the two recoil directions. Detection of such photons gives rise to an interference between the probability amplitudes for the two paths that is manifested in the output from the photodetector as a beat frequency. Since photodissociation of an ensemble of molecules gives rise to a distribution of recoil directions relative to the electric vector of the incident radiation, a range of beat frequencies must be present in the detected signal. This paper gives a calculation of expected output voltage waveforms from a photodetector viewing atomic fluorescence excited by molecular photodissociation. Expressions are given for partial Fourier transforms of the photodetector signals. The results show that the shape of the voltage waveforms depends strongly on the asymmetry parameter for recoil of the photofragments and on whether or not the magnetic sublevels of the excited atomic state are created in a coherent superposition.
Optical response of an active medium can substantially be modified when coherent superpositions of states are excited, that is, when systems display quantum coherence and interference. This has led to fascinating applications in atomic and molecular systems. Examples include coherent population trapping, lasing without inversion, electromagnetically induced transparency, cooperative spontaneous emission, and quantum entanglement. \n \nWe study quantum coherence effects in several quantum optical systems and find interesting applications. We show that quantum coherence can lead to transient Raman lasing and lasing without inversion in short wavelength spectral regions--extreme ultraviolet and x-ray--without the requirement of incoherent pumping. For example, we demonstrate transient Raman lasing at 58.4 nm in Helium atom and transient lasing without inversion at 6.1 nm in Helium-like Boron (triply-ionized Boron). We also investigate dynamical properties of a collective superradiant state prepared by absorption of a single photon when the size of the sample is larger than the radiation wavelength. We show that for large number of atoms such a state, to a good approximation, decays exponentially with a rate proportional to the number of atoms. We also find that the collective frequency shift resulting from repeated emission and reabsorption of short-lived virtual photons is proportional to the number of species in the sample. Furthermore, we examine how a position-dependent excitation phase affects the evolution of entanglement between two dipole-coupled qubits. It turns out that the coherence induced by position-dependent excitation phase slows down the otherwise fast decay of the two-qubit entanglement. We also show that it is possible to entangle two spatially separated and uncoupled qubits via interaction with correlated photons in a cavity quantum electrodynamics setup. Finally, we analyze how quantum coherence can be used to generate continuous-variable entanglement in quantum-beat lasers in steady state and propose possible implementation in quantum lithography.
Entanglement can be understood as an extraordinary degree of correlation between states of quantum systems – a correlation that cannot be given an explanation in terms of something like a common cause. Entanglement can occur between two or more quantum systems, and the most interesting case is when these correlations occur between systems that are space-like separated, meaning that changes made to one system are immediately correlated with changes in a distant system even though there is no time for a signal to travel between them. In this case one says that quantum entanglement leads to non-local correlations, or non-locality. More precisely, entanglement can be defined in the following way. Consider two particles, A and B, whose (pure) states can be represented by the state vectors ψA and ψB. Instead of representing the state of each particle individually, one can represent the composite two-particle system by another wavefunction, Ψ AB. If the two particles are unentangled , then the composite state is just the tensor product of the states of the components: Ψ AB = ψ A ⊗ ψ B; the state is then said to be factorable (or separable). If the particles are entangled, however, then the state of the composite system cannot be written as such a product of a definite state for A and a definite state for B. This is how an entangled state is defined for pure states: a state is entangled if and only if it cannot be factored: Ψ AB ≠ ψ A ⊗ ψ B.
We investigate the excitation of a three-level ladder-type atom by a unidirectional field with a pair of indistinguishable photons. Starting from an analytical expression for the two-photon absorption probability, we determine the two-photon state that maximizes the population of the upper atomic state at a chosen time and show that in the limit of an infinitely long pulse, perfect excitation is possible. The optimal state is identified as the time-reversed counterpart of the two-photon state emitted in spontaneous cascade decay. We then compare this ideal excitation strategy with experimentally accessible families of states, including symmetrized Gaussian product states, temporally correlated Gaussian states, and coherent pulses. We analyze how the optimal excitation conditions depend on the ratio of atomic decay rates and on the separation of the atomic transition frequencies. For indistinguishable photons, quantum interference may shift the maxima of the marginal spectral distribution away from the atomic resonances and qualitatively modify the optimal excitation strategy. Our results clarify the role of indistinguishability and correlations in two-photon absorption and provide guidance for designing realistic excitation schemes in quantum-optical light-matter interfaces.