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International Laser Science Conference

Steady-state light pulses in stimulated backward scattering

Dilip N. Ghosh Roy, Devulapalli V. G. L. N. Rao

Published Jan 1, 1986• 0 citations
Publisher

Abstract

Characteristics of backward, stimulated light pulses are analyzed in the limit where rate equation approximation breaks down, and fluctuation dynamics (oscillator displacements for Raman and phonon amplitudes for Brillouin) must beconsidered. In this limit, the scattered photon flux N s is N s = a(dN l /dt), (d/dt + γ f )A f = bN l /Af,(d/dt + γ l ) = dN l /Af, where f,/referto fluctuations and pump, respectively; A f the fluctuation intensity, and constants a, b, and d depend on the medium characteristics. An analytical solution to this set of equations has been given by Maier et al.1 in the limit γ f →0 and γ l = 0. With these restrictions removed, analytical solution is difficult. Here, we are considering an analytical solution by reducing the set of equations to that of the cubic Schrodinger equation with real amplitude and by using Backlund transform. Preliminary calculations show that the solitary wave solutions are possible (a purely soliton solution is not admissible2 in the form of hyperbolic secant square).

DOI
10.1364/ils.1986.thc5

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Characteristics of backward, stimulated light pulses are analyzed in the limit where rate equation approximation breaks down, and fluctuation dynamics (oscillator displacements for Raman and phonon amplitudes for Brillouin) must beconsidered. In this limit, the scattered photon flux N s is N s = a(dN l /dt), (d/dt + γ f )A f = bN l /Af,(d/dt + γ l ) = dN l /Af, where f,/referto fluctuations and pump, respectively; A f the fluctuation intensity, and constants a, b, and d depend on the medium characteristics. An analytical solution to this set of equations has been given by Maier et al.1 in the limit γ f →0 and γ l = 0. With these restrictions removed, analytical solution is difficult. Here, we are considering an analytical solution by reducing the set of equations to that of the cubic Schrodinger equation with real amplitude and by using Backlund transform. Preliminary calculations show that the solitary wave solutions are possible (a purely soliton solution is not admissible2 in the form of hyperbolic secant square).
Parametric instability induced by the medium saturation in stimulated Raman scattering is investigated theoretically via a generalized detuning (1) where ω p,s,o are the frequency of the pump, Stokes, and phonon, ϕ ˙ p s is the phase modulation, and the last term is the nonlinear correction of the highly excited anharmonic molecule with an amplitude Q.The steady-state gain and hence the Stokes efficiency, in the presence of the anharmonic term, are governed by a cubic equation of |Q|2which is to be solved from the Bloch and Maxwell equations including the pump depletion. Numerical results are shown for the transition diagram of Stokes efficiency vs input pump intensity at various system conditions at the steady-state. For the transient regime, with pulse duration shorter than the dephasing time, we analyze the temporal profiles of the Stokes and the depleted pump based on a transformed equation which combines Bloch and Maxwell equation as follows: (2) where Tis a nonlinear time, G s is the steady-state gain, l0is the input pump intensity, and Uis the real part of the phonon amplitude Q.For an input pulse intensity given by sech2(t/t p ), Eq. (2) is solved numerically to study the transient pulse profiles in the presence of pump depletion and medium saturation.
The equations describing the transfer of intensity from a pump beam simultaneously to forward and backward stimulated scattered beams in an infinite medium are shown to lead to pulsations similar to relaxation oscillations in the scattered intensities. The period of the pulsations is simply related to the gain length for the forward-scattered beam, and may be much longer than the ordinary transient time (related to the damping of material excitations) usually associated with stimulated scattering. Similar oscillations occur for backward scattering alone (stimulated Brillouin scattering) if the scattering medium is finite. In this case the period equals the photon round-trip time in the medium if the latter exceeds the backward gain length. Both phenomena should be observable in scattering from gases such as N2{\mathrm{N}}_{2}N2​ and H2{\mathrm{H}}_{2}H2​ at high pressure, and may also play a role in determining the temporal structure of light scattered from the region of a self-focus in liquids.
A pencil shaped region of a Raman-active medium forms a source for Stokes-shifted light via stimulated Raman Scattering (SRS) when driven by an intense laser pulse. Stokes photons are scattered spontaneously at first, and then amplified during propagation through the medium. Since the scattering is initiated by quantum noise, the actual number of photons produced in any given pulse will be highly uncertain, even if the pulse energy of the driving laser is constant1. As the Stokes light propagates through such an extended region, it's coherence properties will be changed. The spatial coherence is determined by the size and shape of the region, which may be characterized by its Fresnel number F, defined as F= A/λSL, where A is the cross-sectional area of the interaction region, which has length L, and λS is the Stokes wavelength. The rate at which the microscopic scatterers (atoms or molecules) are dephased by collisions affects the temporal coherence of the Stokes light, characterised by the temporal coherence parameter Γτ /gL, where Γ is the collisional dephasing rate, τ is the laser pulse duration and g is the steady-state Raman gain coefficient.
Acousto-optic soliton generation via stimulated Brillouin self-scattering is predicted for light propagating at the speed of sound under electromagnetically induced transparency conditions. As in stimulated Raman self-scattering, the frequency of the electromagnetic component is gradually Stokes shifted as its intensity increases; the acoustic component has no carrier frequency. This phenomenon is explained by the possibility of forward stimulated Brillouin scattering, which is forbidden in nondispersive media. In contrast to stimulated Raman self-scattering, the Stokes shift of the electromagnetic component approaches a constant limit after the pulse has propagated to a certain distance. It is shown that the predicted soliton generation does not involve any threshold condition and can occur at extremely low input pulse intensities.
A semiclassical model of nonstationary stimulated Raman scattering with account of forward and backward waves of different frequencies is proposed. Equations for the elements of a collective density matrix and electric-field amplitudes are obtained applying the averaging method. It is shown that forward waves are generated by a united polarization component, whereas each of the backward waves is formed by its own component. The description is based on the approximation of small scattering angles and assumes that the quantities considered do not depend on transverse coordinates. The emission dynamics of forward-backward Stokes pulses is investigated both for the linear case and under the strong depletion of pumping and level populations. The domain of applicability of the model of nonstationary forward stimulated Raman scattering is determined.