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International Meeting on Instabilities and Dynamics of Lasers and Nonlinear Optical Systems

Large Signal Analysis of Phase Variations and Bistability in Degenerate Four-Wave Mixing

Kazuhito Tajima, Hsiung Hsu

Published Jan 1, 1985• 0 citations
Publisher

Abstract

Large signal analyses for degenerate four-wave mixing (DFWM) have been reported for sometime(1-3). It was nevertheless not obvious why, in specific examples(1,2). DFWM exhibits hysteresis and bistability characteristics, whereas in the case of ideal phase conjugation(3), there is no such instability. The objective of this paper is to show that hysteresis and bistability are caused by phase variations in the interaction. These phase variations are detrimental to phase conjugation and may Indeed up-set the basic characteristies of phase conjugation.

DOI
10.1364/idlnos.1985.wd28

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Large signal analyses for degenerate four-wave mixing (DFWM) have been reported for sometime(1-3). It was nevertheless not obvious why, in specific examples(1,2). DFWM exhibits hysteresis and bistability characteristics, whereas in the case of ideal phase conjugation(3), there is no such instability. The objective of this paper is to show that hysteresis and bistability are caused by phase variations in the interaction. These phase variations are detrimental to phase conjugation and may Indeed up-set the basic characteristies of phase conjugation.
A large-signal theory of noncollinear degenerate four-wave mixing (DFWM) is presented, taking into account the pump depletion and the full nonlinear polarization density appropriate for the noncollinear geometry. Phases of all of the interacting fields, as well as the amplitudes, are obtained as functions of the spatial coordinate. Owing to the completeness of the set of analytic solutions, considerable physical insights into the physics of DFWM are obtained. The DFWM exhibits a variety of rich behaviors, including hysteresis and bistability, multistability, and multiple isolated branches. The authors show that all of these behaviors can be explained in a unified way, that is, in terms of mode hopping characteristics.>
A general formalism is developed to study intracavity phase conjugation through resonant degenerate four-wave mixing. The effects of spatial hole burning, arising from interference of the counterpropagating pump waves, are fully incorporated. The analysis is applied to discuss intracavity phase conjugation in nonlinear media that can be modeled using either a two-level system or a Λ-type three-level system. In both cases, the phase-conjugate reflectivity exhibits bistability for an appropriate choice of the input parameters. For a two-level system, the tuning characteristics of the Fabry–Perot cavity significantly affect the phase-conjugate spectrum that displays hysteresis when the cavity is detuned from the applied laser frequency.
Degenerate four-wave mixing (DFWM) spectroscopy is a potentially powerful technique for quantitative measurement of minor species in gas-phase media [1-3]. In this paper we compare the DFWM signal levels and lineshapes obtained using two different phase-matching geometries: the phase-conjugate geometry and the forward phase-matched geometry. DFWM signal levels are calculated by solving the time-dependent density matrix equations using direct numerical integration (DNI) [4, 5] for a two-level system interacting with three laser beams. This numerical analysis includes the effects of molecular motion, intermolecular collisions, and high laser intensities, all of which have been shown to affect the DFWM signal level.
The exact theory of degenerate four-wave mixing in a Kerr-like medium in the Bragg scattering regime is used to study the reflectivity of phase-conjugate mirrors pumped by intense laser beams. The analysis takes into account pump depletion, nonlinear phase modulation and the relaxation time of the nonlinearity. The steady-state response exhibits multivalued reflectivity, hysteresis and potential bistability; however, the transient response shows that at most one value of the phase-conjugate reflectivity is stable. Periodic or chaotic pulsations are predicted beyond threshold values of pump intensity. The onset of a natural oscillation in the Kerr-like medium is also predicted in the absence of a continuous probe beam; the resulting field amplitude is stable and weakly sensitive upon the presence of external noise.