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High Resolution Spectroscopy

Ultra-Narrow Velocity Distributions of Slow Atoms Produced with the Zeeman Tuning Technique

Sérgio Carlos Zílio, Vanderlei Salvador Bagnato

Published Jan 1, 1993• 0 citations
Publisher

Abstract

We report on the use of a stimulated Raman transition in a slowed atomic beam to produce a narrow velocity distribution of atoms in a selected electronic state, which could be used for atomic collisions studies in the low temperature regime(1). The velocity selection is part of the deceleration process and in this sense it is unique. The atomic beam is decelerated by the radiation pressure force exerted on the atoms by a counter- propagating laser beam. The resonance condition is maintained along the deceleration path because the changing Doppler shift is compensated by Zeeman tuning the electronic sublevels(2) with a spatialy inhomogneous magnetic field. At the end of the slowing process, the initial Maxwell-Boltzman distribution is compressed to a narrow velocity distribution (Δv ~ 50 m/s), centered close to v = 0. This velocity bunching(3) increases considerably the number of atoms in each velocity class, allowing the use of velocity selection techniques as a feasible way of studying low velocity collisions.

DOI
10.1364/hrs.1993.thb3

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We report on the use of a stimulated Raman transition in a slowed atomic beam to produce a narrow velocity distribution of atoms in a selected electronic state, which could be used for atomic collisions studies in the low temperature regime(1). The velocity selection is part of the deceleration process and in this sense it is unique. The atomic beam is decelerated by the radiation pressure force exerted on the atoms by a counter- propagating laser beam. The resonance condition is maintained along the deceleration path because the changing Doppler shift is compensated by Zeeman tuning the electronic sublevels(2) with a spatialy inhomogneous magnetic field. At the end of the slowing process, the initial Maxwell-Boltzman distribution is compressed to a narrow velocity distribution (Δv ~ 50 m/s), centered close to v = 0. This velocity bunching(3) increases considerably the number of atoms in each velocity class, allowing the use of velocity selection techniques as a feasible way of studying low velocity collisions.
A production of low velocity and monoenergetic atomic beams would increase the resolution in spectroscopic studies and many other experiments in atomic physics. Laser Cooling uses the radiation pressure to decelerate and cool atoms. The effusing from a glow discharge metastable argon atomic beam is affected by a counterpropagating laser light tuned to the cycling transition in argon. The Zeeman shift caused by a spatially varying magnetic field compensates for the changing Doppler shift that takes the atoms out of resonance as they decelerated. Deceleration and velocity bunching of atoms to a final velocity that depends on the detuning of the laser relative to a frequency of the transition have been observed. Time-of-Flight (TOF) spectroscopy is used to examine the velocity distribution of the cooled atomic beam. These TOF studies of the laser cooled atomic beam demonstrate the utility of laser deceleration for atomic-beam "velocity selection".
We have developed a diagnostic tool for the study of Zeeman-compensated slowing of an alkali-metal atomic beam. Our time-of-flight technique measures the longitudinal velocity distribution of the slowed atoms with a resolution below the Doppler limit. Furthermore, it can map the position and velocity distribution of atoms in either ground hyperfine level inside the solenoid without any devices inside the solenoid. The technique reveals the optical pumping effects and shows in detail how the slowing within the solenoid proceeds. We find for Na that most atoms in the chosen hyperfine state are decelerated in the slowing process. The width of the velocity distribution is determined mainly by inhomogeneities in the slowing laser beam. Using the central most uniform part of an expanded laser beam, the width is reduced to 2.5 m/s, corresponding to 3.2 mK. Finally, we discuss and show a method to produce a beam with two-velocity components for the study of head-tail low-energy collisions.
Metastable argon atoms Ar*(3P2), produced by electron bombardment of a nozzle beam of ground state Ar atoms, are slowed down from their initial thermal velocity of 560 m/s down to a few tens of m/s, using a standard Zeeman slower. In this decelerator, a repulsive force is induced by a counter-propagating σ+- polarized laser beam, locked in frequency on the3P2-3D3closed transition (λ= 811.5 nm) and then detuned by 340 MHz. A special profile of longitudinal magnetic field is adjusted in order to maintain atoms in resonance with light all over the device, by compensating the variable Doppler shift by the convenient Zeeman shift. Low velocities, e.g. 55 m/s, are accessible but due to spontaneous emission randomly distributed recoil momentums enlarge both angular and velocity distributions of the beam. Nevertheless, by placing off axis collimating slits and grating, it is in principle possible to observe transmission and/or diffraction phenomena specific of low velocities.