Bound quantum states such as atoms can be torn apart by strong oscillating fields. A natural expectation is that stronger fields lead to more certain destruction. In contradiction to this intuition, some theories predict a striking reversal: that as the field intensity is raised above some threshold, bound state wavefunctions can spatially bifurcate and become increasingly stable with increasing field intensity. This ``strong field stabilization'' was predicted decades ago in the context of atoms in pulsed laser fields, but has resisted experimental observation due to extreme laser intensity requirements and theoretical controversy. We report the experimental observation of strong-field stabilization of a ground state, using trapped neutral atoms to emulate the dynamics of atomic electrons in an extremely strong laser field. We directly image the predicted wavepacket bifurcation, measure an ionization rate non-monotonic in field amplitude, and map out the regime of stabilization as a function of laser pulse parameters. We observe that stabilization persists down to surprisingly low drive frequencies, near and below the scale of the lowest-energy excitations of the bound state. These results confirm and extend a long-standing prediction of extreme quantum dynamics, and showcase a complementary tool for probing strong-field phenomena near and beyond the frontier of current laser technology.
Rydberg-state excitation of atoms in strong infrared laser fields provides a new complementary aspect of the perspective of atom--strong field interactions. In this article, we perform an experimental and theoretical study on the corresponding process of diatomic molecules,
N2 and
O2. We show that neutral molecules can also survive strong 800-nm laser fields in high Rydberg states, while their behavior is remarkably different in comparison with their companion atoms, Ar and Xe. The Rydberg excitation of
N2 generally behaves similarly to Ar, while that of
O2 is more significantly suppressed than the ionization compared to Xe in a high intensity region, which can be understood in the frame of a semiclassical picture, together with their different structures of molecular orbitals. However, distinct quantum features in the Rydberg excitation processes that are apparently beyond the semiclassical picture have been identified, i.e., the less suppressed probability of
O2 at low intensity and the oscillation behavior of the ratio between
N2 and Ar, indicating that our understanding of the relevant physics is still far from complete.
This book presents and describes a series of unusual and striking strong-field phenomena concerning atoms and free electrons. Some of these phenomena are: multiphoton stimulated bremsstrahlung, free-electron lasers, wave-packet physics, above-threshold ionization, and strong-field stabilization in Rydberg atoms. The theoretical foundations and causes of the phenomena are described in detail, with all the approximations and derivations discussed. All the known and relevant experiments are described too, and their results are compared with those of the existing theoretical models.An extensive ge
Excitation and photoionization of Rydberg wave packets are described. Interference of bound-free transitions from many coherently populated Rydberg levels is shown to affect the dependence of the photoionization probability on the duration of interaction. Strong-field interference effects in such a system are described also. The most important of these is the field-induced interference stabilization of Rydberg atoms in a strong ionizing field. The intensity range in which this effect can exist is determined. The results derived are used for a qualitative model describing supercontinuum emission in the process of multiphoton ionization.
We describe a detailed account of an experiment demonstrating light-induced stabilization against photoionization. The choice of initial state and atom is discussed in relation to the laser wavelength and laser pulse duration. In combination with a 100-fs, 620-nm probe pulse, the optimum choice is the circular 5g state in neon. A picosecond pump laser was used to prepare this Rydberg state. Initially, the population in this state was probed with a nanosecond laser pulse. Subsequently, the nanosecond probe pulse was replaced by an intense, (sub)picosecond pulse and the photoionization signal was studied. When the probe intensity is several times
1013 W/
cm2 a decrease in yield with respect to a less intense pulse with the same fluence is observed, which indicates stabilization. The results are in accordance with recent theoretical predictions.