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Optical Materials

Temperature-modulated superradiance near phase transition material

Yuying Liu, Tongbiao Wang, Jianrong Yang, Tianbao Yu, Qinghua Liao

Published Feb 14, 2023• 1 citation
Publisher
DOI
10.1016/j.optmat.2023.113568

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We study magnetic materials whose low energy physics can be effectively described by a Dicke model, which we term Dicke materials. We show how a Dicke model emerges in such materials due to a coexistence of fast-dispersing and slow-dispersing spins, which are strongly coupled. Analogous to the paradigmatic Dicke model describing light-matter interactions, these materials also exhibit signatures of a superradiant phase transition. The ground state near the superradiant phase transition is expected to be squeezed, making Dicke materials a resource for quantum metrology and witnessing entanglement in solid-state systems. However, as an entanglement measure, squeezing can be sensitive to perturbations that are otherwise irrelevant for usual correlation functions and order parameters. Motivated by the prospect of observing squeezing in such Dicke materials, we study the robustness of ground state squeezing under ubiquitous imperfections such as finite temperature, disorder, and local interactions. Using analytical and numerical techniques, we show that the squeezing obtained is perturbatively stable against these imperfections and quantitatively evaluate regimes promising for experimental observation.
In the present work we propose a novel quantum material concept, which enables super- and/or ultrastrong interaction of two-level systems with the photonic field in a complex network. Within the mean field approximation we examine phase transition to superradiance that results in two excitation (polariton) branches and is accompanied by the appearance of non-zero macroscopic polarization of two-level systems. We characterize the statistical properties of networks by the first, ⟨k⟩{\langle}k{\rangle}⟨k⟩, and second normalized, ζ≡⟨k2⟩/⟨k⟩ζ\equiv{\langle}k^2{\rangle}/{\langle}k{\rangle}ζ≡⟨k2⟩/⟨k⟩, moments for node degree distribution. We have shown that the Rabi frequency is essentially enhanced due to the topology of the network within the anomalous domain where ⟨k⟩{\langle}k{\rangle}⟨k⟩ and ζζζ sufficiently grow. The multichannel (multimode) structure of matter-field interaction leads superstrong coupling that provides primary behavior of the high temperature phase transition. The results obtained pave the way to design new photonic and polaritonic circuits, quantum networks for efficient processing quantum information at high (room) temperatures.