Abstract Spin-polarized atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that are continuously optically pumped and probed. Due to the collective scattering of photons at large optical depth, the steady state of atoms does not correspond to an uncorrelated tensor-product state, as is usually assumed. We introduce a self-consistent method to approximate the steady state including the pair correlations, taking into account the multilevel structure of atoms. We find and characterize regimes of Raman lasing, akin to the model of a superradiant laser. We determine the spectrum of the collectively scattered photons, which also characterizes the coherence time of the collective spin excitations on top of the stationary correlated mean-field state, as relevant for applications in metrology and quantum information.
Abstract Spin-polarized atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that are continuously optically pumped and probed. Due to the collective scattering of photons at large optical depth, the steady state of atoms does not correspond to an uncorrelated tensor-product state, as is usually assumed. We introduce a self-consistent method to approximate the steady state including the pair correlations, taking into account the multilevel structure of atoms. We find and characterize regimes of Raman lasing, akin to the model of a superradiant laser. We determine the spectrum of the collectively scattered photons, which also characterizes the coherence time of the collective spin excitations on top of the stationary correlated mean-field state, as relevant for applications in metrology and quantum information.
Spin-polarised atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that are continuously optically pumped and probed. Due to the collective scattering of photons at large optical depth, the steady state of atoms does not correspond to an uncorrelated tensor-product state, as is usually assumed. We introduce a self-consistent method to approximate the steady state including the pair correlations, taking into account the multilevel structure of atoms. We find and characterize regimes of Raman lasing, akin to the model of a superradiant laser. We determine the spectrum of the collectively scattered photons, which also characterises the coherence time of the collective spin excitations on top of the stationary correlated mean-field state, as relevant for applications in metrology and quantum information.
We study the three-dimensional nature of the quantum interface between an ensemble of cold, trapped atomic spins and a paraxial laser beam, coupled through a dispersive interaction. To achieve strong entanglement between the collective atomic spin and the photons, one must match the spatial mode of the collective radiation of the ensemble with the mode of the laser beam while minimizing the effects of decoherence due to optical pumping. For ensembles coupling to a probe field that varies over the extent of the cloud, the set of atoms that indistinguishably radiates into a desired mode of the field defines an inhomogeneous spin wave. Strong coupling of a spin wave to the probe mode is not characterized by a single parameter, the optical density, but by a collection of different effective atom numbers that characterize the coherence and decoherence of the system. To model the dynamics of the system, we develop a full stochastic master equation, including coherent collective scattering into paraxial modes, decoherence by local inhomogeneous diffuse scattering, and backaction due to continuous measurement of the light entangled with the spin waves. This formalism is used to study the squeezing of a spin wave via continuous quantum nondemolition (QND) measurement. We find that the greatest squeezing occurs in parameter regimes where spatial inhomogeneities are significant, far from the limit in which the interface is well approximated by a one-dimensional, homogeneous model.
Optimally extracting information from measurements performed on a physical system requires an accurate model of the measurement interaction. Continuously probing the collective spin of an alkali-metal atom cloud via its interaction with an off-resonant optical probe is an important example of such a measurement where realistic modeling at the quantum level is possible using standard techniques from atomic physics. Typically, however, tutorial descriptions of this technique have neglected the multilevel structure of realistic atoms for the sake of simplification. We account for the full multilevel structure of alkali-metal atoms and derive the irreducible form of the polarizability Hamiltonian describing a typical dispersive quantum measurement. For a specific set of parameters, we then show that semiclassical predictions of the theory are consistent with our experimental observations of polarization scattering by a polarized cloud of laser-cooled cesium atoms. We also derive the signal-to-noise ratio under a single-measurement trial and use this to predict the rate of spin squeezing with multilevel alkali-metal atoms for arbitrary detuning of the probe beam.
Abstract We investigate a hybrid quantum system consisting of two coupled optical cavities, each containing an ensemble of coherently pumped artificial or real two-level atoms. The system is modelled within the dressed-state formalism, accounting for coherent driving and dissipative interactions with independent electromagnetic reservoirs. Focusing on the regime where the Rabi frequency greatly exceeds the collective spontaneous emission and cavity decay rates, respectively, we derive the equations of motion characterizing the system and analyse its steady-state behaviours. Special attention is given to the scenario in which only one cavity contains a pumped multi-atom ensemble, and as a consequence, coherent excitation transfer to the second cavity occurs via cavity–cavity coupling. In this case, the mean photon number in the second cavity mode scales proportional to the squared number of atoms, i.e., N2 from the first cavity. The proposed model offers insight into light–matter interaction in composite systems and suggests viable mechanisms for engineering collective interactions and non-local excitation transport in quantum optical platforms.
Quantum measurement is one of the most important features of quantum theory. Although mathematical predictions have been verified in great detail, practical implementation has lagged behind. Only recently have people begun to take advantage of quantum measurement properties to produce new technologies. This research helps fill that technological gap by experimental examination of a continuous, optical measurement for an ensemble of cold atomic spins. The essential physics reduces to the interaction between an atomic ensemble and a weak optical field, which has many well known results. While this work demonstrates many novel applications of the interaction, it also shows that the whole can be more than the sum of the individual parts. Starting with basic characterization of the measurement system using laser-cooled cæsium atoms, the mean value of a spin component is obtained in real time. In essence, the angular momentum of the atomic spins creates a Faraday-like rotation in the polarization of a laser probe beam. With slight modifications, additional spin components are also observed, and are shown to be in good agreement with predictions. In measuring spin dynamics, it is important to account for effects of the probe on the spin states as well. Capitalizing on this as a resource, the probe-induced ac-Stark shift is used to transform a quasi-classical spin-coherent state into a highly quantum Schrödinger cat type of superposition between two spin states. Finally, this work combines all the previous results to demonstrate how a continuous measurement of the spin with a carefully crafted evolution created in part by the probe, allows for nearly real-time determination of the complete spin density matrix. In a single 1.5 millisecond run, a spin density matrix is determined with fidelities ranging from about 85% to 90% across a wide spectrum of test states.
Calibrating the strength of the light-matter interaction is an important experimental task in quantum information and quantum state engineering protocols. The strength of the off-resonant light-matter interaction in multi-atom spin oscillators can be characterized by the readout rate ΓS. Here we introduce the method named Coherently Induced FAraday Rotation (CIFAR) for determining the readout rate. The method is suited for both continuous and pulsed readout of the spin oscillator, relying only on applying a known polarization modulation to the probe laser beam and detecting a known optical polarization component. Importantly, the method does not require changes to the optical and magnetic fields performing the state preparation and probing. The CIFAR signal is also independent of the probe beam photo-detection quantum efficiency, and allows direct extraction of other parameters of the interaction, such as the tensor coupling ζS, and the damping rate γS. We verify this method in the continuous wave regime, probing a strongly coupled spin oscillator prepared in a warm cesium atomic vapour.