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Optics Express

Efficient room-temperature molecular single-photon sources for quantum key distribution

Ghülam Murtaza, Maja Colautti, Michael Hilke, Pietro Lombardi, F. S. Cataliotti, Alessandro Zavatta, Davide Bacco, Costanza Toninelli

Published Dec 12, 2022• 46 citations
Publisher

Abstract

Quantum key distribution (QKD) allows the distribution of cryptographic keys between multiple users in an information-theoretic secure way, exploiting quantum physics. While current QKD systems are mainly based on attenuated laser pulses, deterministic single-photon sources could give concrete advantages in terms of secret key rate (SKR) and security owing to the negligible probability of multi-photon events. Here, we introduce and demonstrate a proof-of-concept QKD system exploiting a molecule-based single-photon source operating at room temperature and emitting at 785 nm. With an estimated maximum SKR of 0.5 Mbps, our solution paves the way for room-temperature single-photon sources for quantum communication protocols.

DOI
10.1364/oe.476440

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Quantum key distribution (QKD) allows the distribution of cryptographic keys between multiple users in an information-theoretic secure way, exploiting quantum physics. While current QKD systems are mainly based on attenuated laser pulses, deterministic single-photon sources could give concrete advantages in terms of secret key rate (SKR) and security owing to the negligible probability of multi-photon events. Here, we introduce and demonstrate a proof-of-concept QKD system exploiting a molecule-based single-photon source operating at room temperature and emitting at 785 nm. With an estimated maximum SKR of 0.5 Mbps, our solution paves the way for room-temperature single-photon sources for quantum communication protocols.
Quantum Key Distribution (QKD) allows the distribution of cryptographic keys between multiple users in an information-theoretic secure way, exploiting quantum physics. While current QKD systems are mainly based on attenuated laser pulses, deterministic single-photon sources could give concrete advantages in terms of secret key rate (SKR) and security owing to the negligible probability of multi-photon events. Here, we introduce and demonstrate a proof-of-concept QKD system exploiting a molecule-based single-photon source operating at room temperature and emitting at 785nm. With an estimated SKR of 0.5 Mbps, our solution paves the way for room-temperature single-photon sources for quantum communication protocols.
Quantum key distribution (QKD) offers a secure means of communication based on the laws of quantum physics. Despite its remarkable advancements, the current reliance of QKD on attenuated coherent (laser) light sources has imposed a fundamental limit on the secure key rate (SKR) per channel use. This constraint stems from the scarcity of single-photon components within coherent light, inherently bounded by a maximum of 1/e. Here, we report comprehensive demonstrations of single-photon-source-based high-rate QKD, surpassing the fundamental SKR limit imposed by the weak coherent light. By employing an on-demand, bright single-photon source with an efficiency of 0.71(2), coupled with narrow-bandwidth filtering and random polarization modulation, we demonstrated a field QKD trial over a 14.6(1.1) dB-loss free-space urban channel, achieving a SKR of 1.08×10^{-3} bits per pulse. This SKR surpasses the practical limit of weak coherent-light-based QKD by 79%. These findings unequivocally demonstrate the superior performance of single-photon sources over weak coherent light for QKD applications, marking a pivotal stride towards realizing a global quantum internet.
Abstract In quantum cryptography, fundamental laws of quantum physics are exploited to enhance the security of cryptographic tasks. Quantum key distribution (QKD) is by far the most studied protocol to date, enabling the establishment of a secret key between trusted parties. Many practical use-cases in communication networks, however, involve parties who do not trust each other. The most fundamental quantum cryptographic building block in such a distrustful setting is quantum coin flipping, which has been studied only in few experimental studies to date, all of which used probabilistic quantum light sources facing fundamental limitations. Here, we experimentally implement a quantum strong coin flipping protocol using single-photon states and demonstrate an advantage compared to both classical realizations and implementations using faint laser pulses. We achieve this by employing a state-of-the-art deterministic single-photon source based on the Purcell-enhanced emission of a semiconductor quantum dot in combination with fast polarization-state encoding with sufficiently low quantum bit error ratio. The reduced multi-photon emission of the single-photon source yields a smaller bias of the coin flipping protocol compared to an attenuated laser implementation, both in simulations and in the experiment. By demonstrating a single-photon quantum advantage in a cryptographic primitive beyond QKD, our work represents a major advance towards the implementation of complex cryptographic tasks in a future quantum internet.
Single-photon sources are essential for quantum networks, enabling applications ranging from quantum key distribution (QKD) to the burgeoning quantum internet. Despite the remarkable advancements, the current reliance of QKD on attenuated coherent (laser) light sources has imposed a fundamental limit on the secret key rate (SKR). This constraint is primarily attributable to the scarcity of single-photon components within coherent light, confined by an inherent upper bound of 1/e. Here, we report high-rate QKD using a high-efficiency single-photon source, enabling an SKR transcending the fundamental rate limit of coherent light. We developed an on-demand, bright semiconductor quantum-dot single-photon source with an efficiency of 0.71(2), exceeding the inherent bound of coherent light by approximately 2.87 dB. Implementing narrow-bandwidth filtering and random polarization modulation, we conducted a field QKD trial over a 14.6(1.1)-dB-loss free-space urban channel, achieving an SKR of 0.00108 bits per pulse. This surpasses the practical limit of coherent-light-based QKD by 2.53 dB. Our findings conclusively demonstrate the superior performance of nanotechnology-based single-photon sources over coherent light for QKD applications, marking a pivotal stride towards the realization of a global quantum internet.
Single-photon sources (SPSs) hold the potential to enhance the performance of quantum key distribution (QKD). QKD systems using SPS often require cryogenic cooling, while recent QKD attempts using SPS operating at room temperature have failed to achieve long-distance transmission due to the SPS not operating at telecommunication wavelength. In this work, we have successfully demonstrated QKD using a room-temperature SPS at telecommunication wavelength. The SPS used in this work is based on point defects hosted by gallium nitride (GaN\mathrm{Ga}\mathrm{N}GaN) thin films grown on sapphire substrates. We employed a time-bin and phase-encoding scheme to perform the BB84 and reference-frame-independent QKD protocols over a 33-km fiber spool, achieving a secure key rate of $7.58\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}7}$ per pulse. Moreover, we also implemented a metropolitan QKD experiment over a 30-km deployed fiber, achieving a secure key rate of $6.06\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}$ per pulse. These results broaden the prospects for future use of SPS in commercial QKD applications.