Photons with high generation rate is one of the essential resources for quantum communication, quantum computing and quantum metrology. Due to the naturally memory-built-in feature, the memory-based photon source is a promising route towards large-scale quantum information processing. However, such photon sources are mostly implemented in extremely low-temperature ensembles or isolated systems, limiting its physical scalability. Here we realize a single-photon source based on a far off-resonance Duan-Lukin-Cirac-Zoller quantum memory at broadband and room-temperature regime. By harnessing high-speed feedback control and repeat-until-success write process, the photon generation rate obtains considerable enhancement up to tenfold. Such a memory-enhanced single-photon source, based on the broadband room-temperature quantum memory, suggests a promising way for establishing large-scale quantum memory-enabled network at ambient condition.
Photons with high generation rate is one of the essential resources for quantum communication, quantum computing and quantum metrology. Due to the naturally memory-built-in feature, the memory-based photon source is a promising route towards large-scale quantum information processing. However, such photon sources are mostly implemented in extremely low-temperature ensembles or isolated systems, limiting its physical scalability. Here we realize a single-photon source based on a far off-resonance Duan-Lukin-Cirac-Zoller quantum memory at broadband and room-temperature regime. By harnessing high-speed feedback control and repeat-until-success write process, the photon generation rate obtains considerable enhancement up to tenfold. Such a memory-enhanced single-photon source, based on the broadband room-temperature quantum memory, suggests a promising way for establishing large-scale quantum memory-enabled network at ambient condition.
Abstract Quantum memory capable of stopping flying photons and storing their quantum coherence is essential for scalable quantum technologies. A room-temperature broadband quantum memory will enable the implementation of large-scale quantum systems for real-life applications. Due to either intrinsic high noises or short lifetime, it is still challenging to find a room-temperature broadband quantum memory beyond conceptual demonstration. Here, we present a far off-resonance Duan–Lukin–Cirac–Zoller (FORD) protocol and demonstrate the broadband quantum memory in room-temperature atoms. We observe a low unconditional noise level of 10−4 and a cross-correlation up to 28. A strong violation of Cauchy–Schwarz inequality indicates high-fidelity generation and preservation of non-classical correlation. Furthermore, the achieved cross-correlation in room-temperature atoms exceeds the key boundary of 6, above which quantum correlation is able to violate Bell’s inequality. Our results open up the door to an entirely new realm of memory-enabled quantum applications at ambient conditions.
Quantum technologies, for example, quantum communication and quantum computation, promise spectacular quantum enhanced advantages beyond what can be done classically. However, quantum states, as the element of quantum technologies, are very fragile and easily get lost to the environment, and meanwhile, their generation and quantum operations are mostly probabilistic. These problems make it exponentially hard to build long-distance quantum channels for quantum communication and large quantum systems for quantum computing. Quantum memory allows quantum states to be stored and retrieved in a programmable fashion, therefore providing an elegant solution to the probabilistic nature and associated limitation by coordinating asynchronous events. In the past decades, enormous advances in quantum memory have been made by developing various storage protocols and their physical implementations, and the quantum memory has gradually evolved from the initial conceptual demonstration to a nearly practical one. Aiming at being practicable for efficient synchronisation and physical scalability, an ideal quantum memory should meet several key features known as high efficiency, low noise level, large time bandwidth product (lifetime divided by pulse duration) and operating at room temperature. Here, we present the research status and development trends of this field by introducing some typical storage protocols. Among these protocols, a room-temperature broadband quantum memory is the most attractive due to its simplicity and practicability. However, at room temperature, noise becomes dominant and is a bottleneck problem that has impeded the realization of a real room-temperature broadband quantum memory in the last decades. Recently, the noise problem has been solved in two memory protocols, i.e. FORD (far off-resonance Duan-Lukin-Cirac-Zoller) protocol and ORCA (off-resonant cascaded absorption) protocol. In this paper, the working principles, the merits and demerits of various quantum memory protocols are illustrated. Furthermore, the approaches to eliminating noise and the applications of quantum memory are summarized.
To realize a large-scale quantum network, both quantum memory and the interference of retrieved indistinguishable photons are essentially required to perform multi-photon synchronization and quantum-interference-mediated entanglement swapping. Significant progress has been achieved in low-temperature and well-isolated systems. However, linking independent quantum memories at room temperature remain challenging. Here, we present an experimental demonstration of Hong–Ou–Mandel interference between single photons from two independent room-temperature quantum memories. We manage to simultaneously operate two such quantum memories and individually obtain a memory-built-in quantum correlation of Stokes and anti-Stokes photons by a far-off-resonance Duan–Lukin–Cirac–Zoller protocol. We also successfully enhance the Hong–Ou–Mandel interference rate up to about 15 times by increasing each photon rate, which is achieved by coordinating two quantum memories with a repeat-until-success fashion. We observe the visibility of quantum interference up to 75.0% without reduction of any background noise, well exceeding the classical limit of 50%. Our results, together with its straightforward, broadband, and room-temperature features, open up a promising way towards realizing large-scale quantum networks at ambient conditions.
Abstract Non-classical photon sources are a crucial resource for distributed quantum networks. Photons generated from matter systems with memory capability are particularly promising, as they can be integrated into a network where each source is used on-demand. Among all kinds of solid state and atomic quantum memories, room-temperature atomic vapours are especially attractive due to their robustness and potential scalability. To-date room-temperature photon sources have been limited either in their memory time or the purity of the photonic state. Here we demonstrate a single-photon source based on room-temperature memory. Following heralded loading of the memory, a single photon is retrieved from it after a variable storage time. The single-photon character of the retrieved field is validated by the strong suppression of the two-photon component with antibunching as low as gRR∣W=1(2)=0.20±0.07 g RR∣W=1 ( 2 ) = 0.20 ± 0.07 . Non-classical correlations between the heralding and the retrieved photons are maintained for up to τNCR=(0.68±0.08)ms τ NC R = ( 0.68 ± 0.08 ) ms , more than two orders of magnitude longer than previously demonstrated with other room-temperature systems. Correlations sufficient for violating Bell inequalities exist for up to τBI = (0.15 ± 0.03) ms.
With the accelerating developments in the field of quantum communication, there will be a need for sources of highly quantum single-photons. In addition to communication applications, the purity, brightness, and fidelity of a given single-photon source are intrinsically linked to the success rate and scalability of a range of photonic technologies in quantum computing, metrology, memory, and cryptography. Further, quantum repeater architectures for maintaining quantum information over long distances will become crucial. In these schemes, end-to-end entanglement is generated by establishing entanglement between the ends of several elementary segments, followed by successive entanglement-swapping operations to increase the entanglement distance until it spans the transmission channel. The most widely studied proposal for the practical implementation of a quantum repeater is the Duan-Lukin-Cirac-Zoller (DLCZ) protocol. This consists of off-resonant Raman excitation by a write pulse, which induces a spin-wave excitation in an atomic ensemble and emits a Stokes photon. At a later time, this spin-wave may be read with a high-power resonant pulse, resulting in the emission of an anti-Stokes photon into a well-defined spatial mode. The Stokes photon may be used for entanglement with another ensemble, while the anti-Stokes may be read out for an entanglement-swapping operation. Notably, in the DLCZ protocol, the atomic ensemble serves as both the quantum memory and a heralded single-photon source. Using atomic ensembles for single-photon sources enables the production of highly pure, indistinguishable photons with minimal spectral broadening; however, the generation rate remains a challenge. In the case of DLCZ, the Raman-scattering step is highly probabilistic, reducing the anti-Stokes generation rate considerably. Furthermore, DLCZ requires operation in the low-excitation-probability regime to avoid multiphoton noise contributions. Additionally, the profile of the induced spin wave is suboptimal for readout. To compensate for these drawbacks, in this thesis we report the experimental realization of a variant of DLCZ that leverages collectively enhanced superradiant (SR) emission. Superradiant emission is characterized by intense bursts of photons emitted in a shorter amount of time than independent atomic state decay. By switching to a resonant excitation and optimizing the write profile, the induced spin-wave is primed for readout, thus increasing retrieval efficiency and the level of quantum correlation. We report data for both the DLCZ and SR schemes under similar optical conditions and compare the two. At high write power, the SR protocol exhibits conditional readout probabilities as high as $\sim$1.2\%, compared to $\sim$0.6\% for the DLCZ protocol under the same conditions. We also analyze the temporal distribution of anti-Stokes emission and find a degree of maintenance of the spin-wave profile, even in the anti-Stokes direction.
Entanglement distribution through existing telecommunication infrastructure is crucial for realizing large-scale quantum networks. However, distance limitations imposed by photon losses and the no-cloning theorem present significant challenges. Quantum repeaters based on entangled telecom wavelength photons and quantum memories offer a promising solution to overcome these limitations. In this work, we report an important milestone in quantum repeater architecture by demonstrating entanglement between a telecom-wavelength (1324 nm) photon and a room-temperature quantum memory with a fidelity up to 90.2%, using simple rubidium systems for both photon generation and storage. Furthermore, we achieve high-rate photon-memory entanglement generation of up to 1,200 Bell pairs per second with 80% fidelity. The technical simplicity and robustness of our room-temperature systems paves the way towards deploying quantum networks at scale in realistic settings.