Certifying whether a photon Fock state is present or not while preserving its quantum state is an important task that proves useful in quantum technologies. The existing methods to perform such task apply to single photons only and consume costly quantum resources. In this paper, we propose a resource-efficient scheme for certification of an arbitrary (nonvacuum) photon Fock state by using second-order nonlinearity. In particular, we utilize the correlations in both photon number and polarization of a stimulated parametric downconversion process to herald the presence and the quantum state of an incoming Fock state. The proposed scheme works excellently with a near perfect certification fidelity even when using nonideal photodetectors. We then compare our scheme with the existing ones taking into account relevant figures of merit for each method. We also present applications of our scheme in overcoming transmission loss of photons in quantum channels as well as in preparation of NOON states, $(|N\ensuremath{\rangle}|0\ensuremath{\rangle}+|0\ensuremath{\rangle}|N\ensuremath{\rangle})/\sqrt{2}$. Our paper introduces to the optical toolbox a practical technique that is beneficial for quantum communication and quantum metrology.
Certifying whether a photon Fock state is present or not while preserving its quantum state is an important task that proves useful in quantum technologies. The existing methods to perform such task apply to single photons only and consume costly quantum resources. In this paper, we propose a resource-efficient scheme for certification of an arbitrary (nonvacuum) photon Fock state by using second-order nonlinearity. In particular, we utilize the correlations in both photon number and polarization of a stimulated parametric downconversion process to herald the presence and the quantum state of an incoming Fock state. The proposed scheme works excellently with a near perfect certification fidelity even when using nonideal photodetectors. We then compare our scheme with the existing ones taking into account relevant figures of merit for each method. We also present applications of our scheme in overcoming transmission loss of photons in quantum channels as well as in preparation of NOON states, (∣N\ensuremath⟩∣0\ensuremath⟩+∣0\ensuremath⟩∣N\ensuremath⟩)/2. Our paper introduces to the optical toolbox a practical technique that is beneficial for quantum communication and quantum metrology.
Fock states are a fundamental resource for many quantum technologies such as quantum metrology. While much progress has been made in single-photon source technologies, preparing Fock states with a large photon number remains challenging. We present and analyze a bootstrapped approach for nondeterministically preparing large photon-number Fock states by iteratively fusing smaller Fock states on a beamsplitter. We show that by employing state recycling we are able to exponentially improve the preparation rate over conventional schemes, allowing the efficient preparation of large Fock states. The scheme requires single-photon sources, beamsplitters, number-resolved photodetectors, fast-feedforward, and an optical quantum memory.
Multiphoton indistinguishability is a key resource for photonic quantum technologies, yet its characterization typically relies on resource-intensive methods. In this work, we develop two efficient and experimentally friendly protocols to estimate or bound the fidelity Find of an N-photon state to the closest perfectly indistinguishable state. The first protocol applies to sources preparing separable states, uses a single Fourier interferometer together with photon-number-resolving detection, and yields tight two-sided bounds on Find. The second protocol combines randomized implementations of linear-optical interferometers with photon counting, enabling direct estimation of Find for arbitrary N-photon states. Both protocols can certify Find=1−O(ε) using provably optimal O(1/ε) samples, in contrast to previous approaches which required prior assumptions on the model of partial distinguishability. Our methods, based on a multiphoton generalization of the Hong-Ou-Mandel test, bring the rigorous and operationally meaningful certification of multiphoton indistinguishability within reach of current photonic technologies.
We present two types of photon sources designed for secure quantum communication, e.g. for quantum cryptography. Both types are based on the creation of photon pairs by spontaneous parametric downconversion in nonlinear crystals. The first is a heralded single photon source and the second is a source of polarization-entangled photon pairs. For the heralded single photon source the detection of one of the photons of a downconversion pair is used as a trigger to announce the presence of the other: the single photon. The source is characterized by a highly sub-Poisson photon number statistics making it very suitable for use in quantum cryptography protocols using single photonic qubits to create correlated information between a sender and a receiver. The entanglement source instead uses the inherent non-classical correlations between entangled qubits. We also present a hybrid-encoding where the sender uses polarization to encode information while the receiver uses time-bins. Both sources create photons with highly non-degenerate wavelengths of 810 nm and 1550 nm, taking advantage of the efficient detectors at near-infrared and the low transmission loss of optical fibers at telecommunication wavelengths.
This thesis presents a study of photon generation and conversion processes in nonlinear optics. Our results extend beyond the first order perturbative regime, in which only pairs of photons are generated in spontaneous parametric down-conversion or four wave mixing. They also allow us to identify the limiting factors for achieving unit efficiency frequency conversion, and to correctly account for the propagation of bright nonclassical photon states generated in the nonlinear material. This is done using the Magnus expansion, which allows us to incorporate corrections due to time-ordering effects in the time evolution of the state, while also respecting the quantum statistics associated with squeezed states (in photon generation) and single photons or coherent states (in photon conversion). We show more generally that this expansion should be the preferred strategy when dealing with any type of time-dependent Hamiltonian that is a quadratic form in the creation and annihilation operators of the fields involved. Using the Magnus expansion, simple figures of merit to estimate the relevance of these time-ordering corrections are obtained. These quantities depend on the group velocities of the modes involved in the nonlinear process and provide a very simple physical picture of the interactions between the photons at different times. These time-ordering effects are shown to be important only when the photons and pump beam overlap within the nonlinear material for a significant amount of time. We also discuss the possibility of preparing Fock states with many photons using parametric down-conversion sources and realistic photon-number-resolving detectors. After discussing photon generation processes, we study photon conversion processes in which a nonlinear material and a classical strong pump field are used modify the frequency of a second incoming low-intensity field. We show that time-ordering effects limit the efficiency of this conversion process, re-examine strategies to get around this problem, and show that it should be possible to have a clear observation of modified upconversion probabilities due to these effects, and thus have an experimental demonstration of time-ordering effects in nonlinear optics.
Optical quantum computing, quantum information and quantum communication protocols rely on the generation of qubits encoded in optical systems, many of which can be generate via the process of spontaneous parametric down-conversion. In this thesis, we investigate down-converted states, in the context of quantum computing and quantum information. In the high gain regime, a type I down-converted state can be described as a single-mode squeezed vacuum state. We present an analysis of photon-subtracted squeezed vacuum states as a resource for teleportation of coherent state qubits and propose proof-of-principle experiments for the demonstration of coherent-state teleportation and entanglement swapping. In the low gain regime, the output state of a type II parametric down-converter can be approximated as containing pairs of single photons, which can be used to herald the presence of one- or two- photon Fock states in one mode, conditional on the detection of the same number of photons in the other mode. We explore the effects of spectral filtering and inefficient detection, of the heralding mode, on the count rate, g(2) and purity of the heralded state, as well as the fidelity between the resulting state and an ideal Fock state. We also develop a technique for controlling the joint spectral profile of the down-converted photons. By exploiting the dependence of the effective nonlinearity of a periodically poled crystal on its poling order, we tailor the nonlinearity profile and therefore the phase matching function of the down-converted photons. Finally, we consider the validity of the Taylor series expansion of the unitary operator which governs the evolution of the fields within the crystal, in comparison to the strictly correct time-ordered Dyson series expansion.
Non-Gaussian states of light are essential for numerous quantum information protocols; thus, certifying non-Gaussianity is crucial. Full quantum state tomography, commonly used for this purpose, is a complicated procedure and yields inconclusive results for strongly mixed states. Certifying non-Gaussianity through directly measurable parameters is a simpler alternative, typically achieved by measuring photon-number probabilities - either directly, using photon-number resolving detectors, or through Hanbury Brown--Twiss type measurements with single-photon detectors. Here, we demonstrate theoretically and experimentally that optical parametric amplification combined with conventional intensity detectors can effectively replace this approach without the need for photon-number resolution. In our method, we measure the mean photon number and the second-order correlation function for the amplified state. Using it, we successfully certify the non-Gaussianity of a heralded quasi-single-photon state. Since optical parametric amplification is a broadband and multimode process, our method provides a foundation for developing high-dimensional quantum technologies utilizing broadband multimode non-Gaussian states.