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Scientific Reports

Frequency stabilization of multiple lasers to a reference atomic transition of Rb

Shubham Utreja, Harish Kumar Rathore, Manoj Das, Subhasis Panja

Published Nov 30, 2022• 17 citations
Publisher

Abstract

Abstract Modern atomic clocks based on the interrogation of an atomic transitions in the optical regions require multiple lasers at different wavelength for producing atomic ions, trapping and laser cooling of neutral atoms or atomic ions. In order to achieve highest efficiency for laser cooling or any other atomic transition, frequencies of each of the lasers involved need to be stabilized by mitigating its drifts or fluctuations arise due to ambient temperature variation or other kind of perturbations. The present article describes simultaneous frequency stabilization of multiple number of lasers, required for production and laser cooling of ytterbium (171Yb) ions, to a reference transition frequency of rubidium (Rb) atoms. In this technique, a diode laser operating at ~ 780 nm is frequency stabilized to one of the Doppler broadening-free absorption peak of rubidium atoms (85Rb) and then used as a reference frequency for calibrating a wavelength meter and subsequent simultaneous frequency stabilization of four lasers operating at different wavelengths.

DOI
10.1038/s41598-022-24952-6

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Quantum Electronics•Jun 30, 2014•3 citations
Abstract Modern atomic clocks based on the interrogation of an atomic transitions in the optical regions require multiple lasers at different wavelength for producing atomic ions, trapping and laser cooling of neutral atoms or atomic ions. In order to achieve highest efficiency for laser cooling or any other atomic transition, frequencies of each of the lasers involved need to be stabilized by mitigating its drifts or fluctuations arise due to ambient temperature variation or other kind of perturbations. The present article describes simultaneous frequency stabilization of multiple number of lasers, required for production and laser cooling of ytterbium (171Yb) ions, to a reference transition frequency of rubidium (Rb) atoms. In this technique, a diode laser operating at ~ 780 nm is frequency stabilized to one of the Doppler broadening-free absorption peak of rubidium atoms (85Rb) and then used as a reference frequency for calibrating a wavelength meter and subsequent simultaneous frequency stabilization of four lasers operating at different wavelengths.
We have demonstrated simultaneous laser frequency stabilization of a UV and IR laser, to coupled transitions of ions in the same spectroscopic sample, by detecting only the absorption of the UV laser. Separate signals for locking the different lasers are obtained by modulating each laser at a different frequency and using lock-in detection of a single photodiode signal. Experimentally, we simultaneously lock a 369 nm and a 935 nm laser to the (2)S(1/2) → (2)(P(1/2) and (2)D(3/2) → (3)D([3/2]1/2) transitions, respectively, of Yb(+) ions generated in a hollow cathode discharge lamp. Stabilized lasers at these frequencies are required for cooling and trapping Yb(+) ions, used in quantum information and in high precision metrology experiments. This technique should be readily applicable to other ion and neutral atom systems requiring multiple stabilized lasers.
Laser cooling experiments developed in the last decade enable physicists to slow down and spatially confine neutral atoms of a gas, thus lowering the temperature of trapped atoms into the μK range. One of the challenges associated with laser cooling is to stabilize a laser so that its output frequency matches that of a hyperfine structure transition and has an absolute stability of several MHz. In this project, we establish the groundwork for future laser cooling experiments with Rb by performing saturated-absorption Doppler-free spectroscopy studies. We acquire Doppler-free spectra of Rb that resolve individual hyperfine structure transitions, including the transition that the laser must excite in laser cooling experiments. The spectra we obtained can readily be repeated and the experimental apparatus can provide the feedback for an electronic laser stabilization circuit.
We present a scheme for stabilizing multiple lasers at wavelengths between 795 and 866 nm to the same atomic reference line. A reference laser at 852 nm is stabilized to the Cs D 2 line using a Doppler-free frequency modulation technique. Through transfer cavities, four lasers are stabilized to the relevant atomic transitions in 40 Ca + . The rms linewidth of a transfer-locked laser is measured to be 123 kHz over 200 ms with respect to an independent atomic reference, the Rb D 1 line. This stability is confirmed by the comparison of an excitation spectrum of a single 40 Ca + ion to an eight-level Bloch equation model. The long-term stability with respect to the same reference is measured to be 130 kHz over a period of 2 h. The high degree of stability is demonstrated by the measured Allan deviation around 10 −11 between 1 and 100 s.
We demonstrate a robust method of stabilizing a diode laser frequency to an atomic transition. This technique employs the Zeeman shift to generate an antisymmetric signal about a Doppler-broadened atomic resonance, and therefore offers a large recapture range as well as high stability. The frequency of a 780-nm diode laser, stabilized to such a signal in Rb, drifted less than 0.5 MHz peak-peak (1 part in 10(9)) in 38 h. This tunable frequency lock can be constructed inexpensively, requires little laser power, rarely loses lock, and can be extended to other wavelengths by use of different atomic species.
In the development of atomic physics, laser sources with Frequencies corresponding to atomic transition and high stability are essential. The Faraday laser is a special diode laser using the Faraday anomalous dispersion optical filter (FADOF) to realize frequency selection, so the output laser frequency is automatically limited to the atomic Doppler broadening. However, the frequency of a Faraday laser corresponds to the range around only one atomic hyperfine transition. Here, we realize a switchable Faraday laser with two isotopes laser frequencies corresponding to 85Rb 52S1/2 (F=3)→52P3/2 and 87Rb 52S1/2 (F=2)→52P3/2 transitions based on a single isotope 87Rb-FADOF. The laser has good robustness against the fluctuation of diode current and temperature, with wavelength fluctuating within 0.8 pm from 16 to 30 °C of diode temperature, and has a free-running linewidth of 18 kHz. We also lock the laser frequency to the two cycling transitions of 85Rb 52S1/2 (F=3)→52P3/2 (F′=4) and 87Rb 52S1/2 (F=2)→52P3/2 (F′=3) by the modulation transfer spectroscopy technique. The Allan deviation of the residual error signal is 3×10−14/τ, and the frequency stability of the beat detection reaches 2.8×10−12 at 1 s integration time. This 780 nm switchable Faraday laser expands the application scenarios of Faraday lasers, which can be used in laser cooling atoms, optical frequency standards, and other quantum precision measurement fields.
A laser system for Doppler cooling of ytterbium ion on the transition in a single-ion optical frequency standard is developed. The second harmonic of a semiconductor laser with a wavelength of is used for cooling. The laser frequency is doubled in a nonlinear BiBO crystal embedded in a ring resonator, which also serves as a reference for laser frequency stabilisation. Second-harmonic power of is generated at a wavelength of . Diode laser radiation is modulated by an electro-optic modulator at to generate a sideband exciting the hyperfine component of the cooling transition that is not excited by resonant cooling light. The sideband relative intensity of a few percent proved to be sufficient to reduce the ion dwelling time in the state to less than and increase the cooling efficiency.