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Materials for Quantum Technology

Fiber-coupled quantum light sources based on solid-state quantum emitters

Lucas Bremer, Sven Rodt, Stephan Reitzenstein

Published Nov 17, 2022• 22 citations
Publisher

Abstract

Abstract Photonic quantum technology is essentially based on the exchange of individual photons as information carriers. Therefore, the development of practical single-photon sources that emit single photons on-demand is a crucial contribution to advance this emerging technology and to promote its first real-world applications. In the last two decades, a large number of quantum light sources based on solid-state emitters have been developed on a laboratory scale. Corresponding structures today have almost ideal optical and quantum-optical properties. For practical applications, however, one crucial factor is usually missing, namely direct on-chip fiber coupling, which is essential, for example, for the direct integration of such quantum devices into fiber-based quantum networks. In fact, the development of fiber-coupled quantum light sources is still in its infancy, with very promising advances having been made in recent years. Against this background, this review article presents the current status of the development of fiber-coupled quantum light sources based on solid-state quantum emitters and discusses challenges, technological solutions and future prospects. Among other things, the numerical optimization of the fiber coupling efficiency, coupling methods, and important realizations of such quantum devices are presented and compared. Overall, this article provides an important overview of the state-of-the-art and the performance parameters of fiber-coupled quantum light sources that have been achieved so far. It is aimed equally at experts in the scientific field and at students and newcomers who want to get an overview of the current developments.

DOI
10.1088/2633-4356/aca3f3

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Abstract Photonic quantum technology is essentially based on the exchange of individual photons as information carriers. Therefore, the development of practical single-photon sources that emit single photons on-demand is a crucial contribution to advance this emerging technology and to promote its first real-world applications. In the last two decades, a large number of quantum light sources based on solid-state emitters have been developed on a laboratory scale. Corresponding structures today have almost ideal optical and quantum-optical properties. For practical applications, however, one crucial factor is usually missing, namely direct on-chip fiber coupling, which is essential, for example, for the direct integration of such quantum devices into fiber-based quantum networks. In fact, the development of fiber-coupled quantum light sources is still in its infancy, with very promising advances having been made in recent years. Against this background, this review article presents the current status of the development of fiber-coupled quantum light sources based on solid-state quantum emitters and discusses challenges, technological solutions and future prospects. Among other things, the numerical optimization of the fiber coupling efficiency, coupling methods, and important realizations of such quantum devices are presented and compared. Overall, this article provides an important overview of the state-of-the-art and the performance parameters of fiber-coupled quantum light sources that have been achieved so far. It is aimed equally at experts in the scientific field and at students and newcomers who want to get an overview of the current developments.
Abstract Photonic quantum science—which harnesses light-matter interactions down to the single photon level—provides advanced light sources for quantum sensing, communication, and computing. Integrating solid-state light sources on a photonic chip provides a means of creating scalable on-chip quantum networks with sophisticated optoelectronic circuitry. Extending beyond single emitters to multi-emitter systems is a frontier that offers substantial opportunities for fundamental scientific advances as well as applications that require multi-emitter quantum states. A key challenge in this endeavor is the spectral inhomogeneity of solid-state emitters, which results in non-identical emitters that cannot be interfaced with one another. This review describes recent advances in tailoring the emission properties of individual emitters and the multi-emitter demonstrations that are enabled by this control for a variety of prominent materials, as well as prospects for further development.
The goal of integrated quantum photonics is to combine components for the generation, manipulation, and detection of nonclassical light in a phase-stable and efficient platform. Solid-state quantum emitters have recently reached outstanding performance as single-photon sources. In parallel, photonic integrated circuits have been advanced to the point that thousands of components can be controlled on a chip with high efficiency and phase stability. Consequently, researchers are now beginning to combine these leading quantum emitters and photonic integrated circuit platforms to realize the best properties of each technology. In this paper, we review recent advances in integrated quantum photonics based on such hybrid systems. Although hybrid integration solves many limitations of individual platforms, it also introduces new challenges that arise from interfacing different materials. We review various issues in solid-state quantum emitters and photonic integrated circuits, the hybrid integration techniques that bridge these two systems, and methods for chip-based manipulation of photons and emitters. Finally, we discuss the remaining challenges and future prospects of on-chip quantum photonics with integrated quantum emitters.
The controlled generation of non-classical states of light is a challenging task at the heart of quantum optics. Aside from the mere spirit of science, the related research is strongly driven by applications in photonic quantum technologies, including the fields of quantum communication, quantum computation, and quantum metrology. In this context, the realization of integrated solid-state-based quantum-light sources is of particular interest, due to the prospects for scalability and device integration. This topical review focuses on solid-state quantum-light sources which are fabricated in a deterministic fashion. In this framework we cover quantum emitters represented by semiconductor quantum dots, colour centres in diamond, and defect-/strain-centres in two-dimensional materials. First, we introduce the topic of quantum-light sources and non-classical light generation for applications in photonic quantum technologies, motivating the need for the development of scalable device technologies to push the field towards real-world applications. In the second part, we summarize material systems hosting quantum emitters in the solid-state. The third part reviews deterministic fabrication techniques and comparatively discusses their advantages and disadvantages. The techniques are classified in bottom-up approaches, exploiting the site-controlled positioning of the quantum emitters themselves, and top-down approaches, allowing for the precise alignment of photonic microstructures to pre-selected quantum emitters. Special emphasis is put on the progress achieved in the development of in situ techniques, which significantly pushed the performance of quantum-light sources towards applications. Additionally, we discuss hybrid approaches, exploiting pick-and-place techniques or wafer-bonding. The fourth part presents state-of-the-art quantum-dot quantum-light sources based on the fabrication techniques presented in the previous sections, which feature engineered functionality and enhanced photon collection efficiency. The article closes by highlighting recent applications of deterministic solid-state-based quantum-light sources in the fields of quantum communication, quantum computing, and quantum metrology, and by discussing future perspectives in the field of solid-state quantum-light sources.
Sources of quantum light that utilize photonic nanowire designs have emerged as potential candidates for high efficiency non-classical light generation in quantum information processing. In this review we cover the different platforms used to produce nanowire-based sources, highlighting the importance of waveguide design and material properties in achieving optimal performance. The limitations of the sources are identified and routes to optimization are proposed. State-of-the-art nanowire sources are compared to other solid-state quantum emitter platforms with regard to the key metrics of single photon purity, indistinguishability and entangled-pair fidelity to maximally entangled Bell states. We also discuss the unique ability of the nanowire platform to incorporate multiple emitters in the same optical mode and consider potential applications. Finally, routes to on-chip integration are discussed and the challenges facing the development of a nanowire-based scalable architecture are presented.
Solid-state quantum emitters operating in the telecom wavelength range are pivotal for the development of scalable quantum information processing technologies. In this review, we provide a comprehensive overview of the state-of-the-art solid-state emitters of single photons targeting quantum information processing in the discrete-variable regime and telecom wavelength range. We focus on quantum dots, color centers, and erbium ion dopants, detailing their synthesis methods and their applications. The review addresses the strategies for the integration of these quantum emitters into photonic devices alongside the associated challenges. We also discuss their applications in quantum technologies, examining current limitations, including performance constraints, decoherence, and scalability. Finally, we propose future directions for advancing photonic-based quantum technologies.
The development of single-photon sources has been nothing but rapid in recent years, with quantum emitter-based systems showing especially impressive progress. In this article, we give an overview of the developments in single-photon sources based on single molecules. We will introduce polycyclic hydrocarbons as the most commonly used emitter systems for the realization of an organic solid-state single-photon source. At cryogenic temperatures this special class of fluorescent molecules demonstrates remarkable optical properties such as negligible dephasing, indefinite photostability, and high photon rates, which make them attractive as fundamental building blocks in emerging quantum technologies. To better understand the general properties and limitations of these molecules, we discuss sample preparation and relevant emitter parameters such as absorption and emission spectra, lifetime, and dephasing. We will also give an overview of light extraction strategies as a crucial part of a single-photon source. Finally, we conclude with a look into the future, displaying current challenges and possible solutions.