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Physics

Frequency Comb Measures Quantum Interference

Philip Ball

Published Oct 21, 2022• 0 citations
Publisher

Abstract

A multiwavelength laser source known as a frequency comb provides a new technique for atom interferometry, potentially leading to new tests of fundamental physics.
DOI
10.1103/physics.15.161

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The measurement and manipulation of coherent optical fields have been transformed by the optical frequency comb. Today, the optical frequency comb grants measurements precise enough to count individual cycles of light as well as the generation of nearly any coherent electromagnetic field from the ultraviolet through the infrared. These capabilities have enabled the most precise realizations and comparisons of time, precision spectroscopy over broad bandwidths, and the ability to convert stable signals between optical and microwave fields–seamlessly connecting the entire electromagnetic spectrum from hertz (100 ) to petahertz (1015). These applications involve the interference of a frequency comb with another coherent light source, such as another frequency comb or a single-frequency continuous-wave laser. However, coherent light represents only one type of light. The vast majority of light emanates from “black bodies” such as stars, which is in a thermal state as opposed to a coherent state, and carries profound information about the universe and humanity’s place within it. Other types of light defy classical electromagnetism and are known as non-classical or quantum light. Such quantum light may play central roles in quantum communication, quantum computation, and quantum-enhanced metrology. In this thesis, the use of the optical frequency comb in the interferometric measurement of thermal and quantum light is investigated, with a focus on assessing fundamental limits to the sensitivity of such measurements. In order to measure thermal light, a technique called dual-comb correlation spectroscopy is explored. This technique entails heterodyne measurement of the field of thermal light and subsequent correlation of the field in time. This process reveals the spectrum of thermal light at high resolution and across broad bandwidths. New theoretical work uncovers previously unknown fundamental limits on sensitivity when measuring realistically weak thermal light. Experimental investigation verifies this scaling and is accompanied by a demonstration of spectroscopy at the equivalent power spectral density of our Sun, realizing a greater than 1000-fold sensitivity increase over past demonstrations of this technique. These insights pave the way for expansion of this technique to comb-based spatial correlation of thermal fields. This advancement would allow for extended baseline synthetic aperture hyperspectral imaging throughout the optical spectrum, facilitating novel and profound observations of the universe. The use of frequency combs for the measurement of quantum light is also investigated. This scenario breaks typical quantum optics assumptions, such as large, mode-matched local oscillators, and necessitates new quantum measurement operators. Such measurement operators are derived, which not only describe homodyne measurements on any quantum state of light with a frequency comb local oscillator, but also indicate that the shot noise limit generally reached in comb-based measurements of coherent light (such as in continuous-wave laser heterodyne and dual-comb spectroscopy) does not correspond to the quadrature or coherent state-overlap description standard in quantum optics. Efforts to experimentally reach this “standard” quantum limit demonstrate a significant improvement in the signal-to-noise ratio over the conventional comb-based shot noise limit, paving the way for lower-power portable optical clocks and quantum-enhanced frequencycomb metrology.
We demonstrate a light-pulse atom interferometer based on the diffraction of free-falling atoms by a picosecond frequency-comb laser. More specifically, we coherently split and recombine wave packets of cold ^{87}Rb atoms by driving stimulated Raman transitions between the |5s ^{2}S_{1/2},F=1⟩ and |5s ^{2}S_{1/2},F=2⟩ hyperfine states, using two trains of picosecond pulses in a counterpropagating geometry. We study the impact of the pulses' length as well as the interrogation time onto the contrast of the atom interferometer. Our experimental data are well reproduced by a numerical simulation based on an effective coupling that depends on the overlap between the pulses and the atomic cloud. These results pave the way for extending light-pulse interferometry to transitions in other spectral regions and therefore to other species, for new possibilities in metrology, sensing of gravito-inertial effects, and tests of fundamental physics.
We have implemented of a light pulse atom interferometer based on the diffraction of free-falling atoms of Rubidium by a picosecond frequency-comb laser. We have studied the impact of the pulses’ length as well as of the interrogation time on the contrast of the fringes. Our data are well reproduce by a theoretical model based on the effective coupling which depend on the overlap between the pulses and the atoms. This technique, which we demonstrated in the visible spectrum on Rb atoms, paves the way for extending light-pulse interferometry to other spectral regions (deep-UV to X-UV) and therefore to new species, since one can benefit from the high peak intensity of the ultrashort pulses which makes nonlinear frequency conversion in crystals and gas targets more efficient.