A Solid Observation of Strong Kerr Nonlinearity

Hamid Reza Hamedi, Seyyed Hossein Asadpour, Mostafa Sahrai

Jon D. Pritchett, Liam A. P. Gallagher, Alistair Brewin +5 more

Microwave–optical conversion is key to future networks of quantum devices, such as those based on superconducting technology. Conversion at the single quantum level requires strong nonlinearity, high bandwidth, and compatibility with a millikelvin environment. A large nonlinearity is observed in Rydberg atoms, but combining atomic gases with dilution refrigerators is technically challenging. Here, we demonstrate a strong microwave–optical nonlinearity in a cryogenic, solid-state system by exploiting Rydberg states of excitons in Cu2O. We measure a microwave–optical cross-Kerr coefficient of B0 = 0.022 ± 0.008 m V−2 at 4 K, which is several orders of magnitude larger than other solid-state systems. The results are in quantitative agreement with a nonlinear susceptibility model based on the giant microwave dipole moment between nearby excitonic states. Our results highlight the potential of Rydberg excitons for nonlinear optics and form the basis for a microwave–optical frequency converter based on Cu2O.

Zhengyang Bai, Weibin Li, Guoxiang Huang

Realizing single light bullets and vortices that are stable in high dimensions is a long-standing goal in the study of nonlinear optical physics. On the other hand, the storage and retrieval of such stable high dimensional optical pulses may offer a variety of applications. Here we present a scheme to generate such optical pulses in a cold Rydberg atomic gas. By virtue of electromagnetically induced transparency, strong, long-range atom-atom interaction in Rydberg states is mapped to light fields, resulting in a giant, fast-responding nonlocal Kerr nonlinearity and the formation of light bullets and vortices carrying orbital angular momenta, which have extremely low generation power, very slow propagation velocity, and can stably propagate, with the stability provided by the combination of local and the nonlocal Kerr nonlinearities. We demonstrate that the light bullets and vortices obtained can be stored and retrieved in the system with high efficiency and fidelity. Our study provides a new route for manipulating high-dimensional nonlinear optical processes via the controlled optical nonlinearities in cold Rydberg gases.

James A. McKelvie

Hoonsoo Kang, Lingling Wen, Yifu Zhu

Zeyun Shi, Guoxiang Huang

We investigate the formation and control of stationary optical patterns in a cold Rydberg atomic gas via double electromagnetically induced transparency. We show that, through the modulational instability of the plane-wave state of a laser field with two polarization components, the system undergoes a spontaneous symmetry breaking and hence the emergence of plentiful self-organized spatial optical structures, which can be manipulated by the ratio between the cross- and self-Kerr nonlinearities, the nonlocality degree of the Kerr nonlinearities, and the populations initially prepared in the two atomic ground states. Interestingly, a crossover from mixture to separation in space (optical phase separation) of the two polarization components occurs when the ratio between the cross- and self-Kerr nonlinearities exceeds a critical value. We also show that the system supports nonlocal two-component spatial optical solitons and vortices when the parameters of the system are selected suitably. The rich diversity and active controllability of the self-organized optical structures reported here provide a way for realizing novel optical patterns and solitons and their structural phase transitions based on Rydberg atomic gases.