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Conference on Lasers and Electro-Optics

Ultrafast energy exchange between two single Rydberg atoms on the nanosecond timescale

Yuki Torii Chew, Takafumi Tomita, Tirumalasetty Panduranga Mahesh, Seiji Sugawa, Sylvain de Léséleuc, Kenji Ohmori

Published Jan 1, 2022• 1 citation
Publisher

Abstract

We observed a nanosecond-scale dynamics between two single atoms trapped in optical tweezers separated by ~ 1 µm and excited to Rydberg state with picosecond laser pulses. This opens the path for ultrafast quantum computation.
DOI
10.1364/cleo_qels.2022.fm4d.2

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Abstract Rydberg atoms, with their enormous electronic orbitals, exhibit dipole–dipole interactions reaching the gigahertz range at a distance of a micrometre, making them a prominent contender for realizing ultrafast quantum operations. However, such strong interactions between two single atoms have so far never been harnessed due to the stringent requirements on the fluctuation of the atom positions and the necessary excitation strength. Here we introduce novel techniques to explore this regime. First, we trap and cool atoms to the motional quantum ground state of holographic optical tweezers, which allows control of the inter-atomic distance down to 1.5 μm with a quantum-limited precision of 30 nm. We then use ultrashort laser pulses to excite a pair of these nearby atoms to a Rydberg state simultaneously, far beyond the Rydberg blockade regime, and perform Ramsey interferometry with attosecond precision. This allows us to induce and track an ultrafast interaction-driven energy exchange completed on nanosecond timescales—two orders of magnitude faster than in any other Rydberg experiments in the tweezers platform so far. This ultrafast coherent dynamics gives rise to a conditional phase, which is the key resource for a quantum gate, opening the path for quantum simulation and computation operating at the speed limit set by dipole–dipole interactions with this ultrafast Rydberg platform.
Rydberg atoms in optical lattices and tweezers is now a well-established platform for simulating quantum spin systems. However, the role of the atoms' spatial wave function has not been examined in detail experimentally. Here, we show a strong spin-motion coupling emerging from the large variation of the interaction potential over the wave function spread. We observe its clear signature on the ultrafast many-body nanosecond-dynamics of atoms excited to a Rydberg S state, using picosecond pulses, from an unity-filling atomic Mott-insulator. We also propose an approach to tune arbitrarily the strength of the spin-motion coupling relative to the motional energy scale set by trapping potentials. Our work provides a new direction for exploring the dynamics of strongly correlated quantum systems by adding the motional degree of freedom to the Rydberg simulation toolbox.
Quantum excitation is usually regarded as a transient process occurring instantaneously, leaving the underlying physics shrouded in mystery. Recent research shows that Rydberg-state excitation with ultrashort laser pulses can be investigated and manipulated with state-of-the-art few-cycle pulses. We theoretically find that the efficiency of Rydberg state excitation can be enhanced with a short laser pulse and modulated by varying the laser intensities. We also uncover new facets of the excitation dynamics, including the launching of an electron wave packet through strong-field ionization, the re-entry of the electron into the atomic potential and the crucial step where the electron makes a U-turn, resulting in twin captures into Rydberg orbitals. By tuning the laser intensity, we show that the excitation of the Rydberg state can be coherently controlled on a sub-optical-cycle timescale. Our work paves the way toward ultrafast control and coherent manipulation of Rydberg states, thus benefiting Rydberg-state-based quantum technology.
We demonstrate a physical quantum simulator of ultrafast phenomena, in which time-varying forces on neutral atoms in a tunable optical trap emulate the electric fields of a pulsed laser acting on electrons or nuclei in a binding potential. The simulator operates in regimes equivalent to those of ultrafast and strong-field pulsed-laser experiments, opening up a hitherto unexplored application of quantum simulation techniques and a complementary path towards investigating open questions in ultrafast science. Counter-intuitively, this approach emulates some of the fastest processes in atomic physics with some of the slowest, giving rise to a temporal magnification factor of up to twelve orders of magnitude which greatly simplifies experimental access to the dynamics. The correspondence with ultrafast science is demonstrated by a sequence of experiments: we perform nonlinear spectroscopy of a many-body bound state, control the excitation spectrum by shaping the potential, observe sub-cycle unbinding dynamics during strong few-cycle pulses, and directly measure carrier-envelope phase dependence of the response to an ultrafast-equivalent pulse.