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Physical review. B./Physical review. B

Emergent topological orders and phase transitions in lattice Chern-Simons theory of quantum magnets

Rui Wang, Z. Y. Xie, Baigeng Wang, Tigran Sedrakyan

Published Sep 29, 2022• 20 citations
Publisher

Abstract

Topological phase transitions involving intrinsic topological orders are usually characterized by qualitative changes of ground state quantum entanglement, which cannot be described by conventional mean-field theories with local order parameters. Here, we apply the lattice Chern-Simons theory to study frustrated quantum magnets and show that the conventional concepts, such as the order parameter and symmetry breaking, can still play a crucial role in certain topological phase transitions. The lattice Chern-Simons representation establishes a nonlocal mapping from quantum spin models to interacting spinless Dirac fermions. We show that breaking certain emergent symmetries of the fermionic theory could provide a unified approach to describing both magnetic and topological orders, as well as the topological phase transitions between them. We apply this method to the perturbed spin-1/2 ${J}_{1}\ensuremath{-}{J}_{2}$ XY model on the honeycomb lattice and predict a nonuniform chiral spin liquid ground state in the strong frustration region. This is further verified by our high-precision tensor network calculations. These results suggest that the lattice Chern-Simons theory can simplify the complicated topological phase transitions to effective mean-field theories in terms of fermionic degrees of freedom, which lead to different understandings that help to understand the frustrated quantum magnets.

DOI
10.1103/physrevb.106.l121117

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Topological phase transitions involving intrinsic topological orders are usually characterized by qualitative changes of ground state quantum entanglement, which cannot be described by conventional mean-field theories with local order parameters. Here, we apply the lattice Chern-Simons theory to study frustrated quantum magnets and show that the conventional concepts, such as the order parameter and symmetry breaking, can still play a crucial role in certain topological phase transitions. The lattice Chern-Simons representation establishes a nonlocal mapping from quantum spin models to interacting spinless Dirac fermions. We show that breaking certain emergent symmetries of the fermionic theory could provide a unified approach to describing both magnetic and topological orders, as well as the topological phase transitions between them. We apply this method to the perturbed spin-1/2 J1\ensuremath−J2{J}_{1}\ensuremath{-}{J}_{2}J1​\ensuremath−J2​ XY model on the honeycomb lattice and predict a nonuniform chiral spin liquid ground state in the strong frustration region. This is further verified by our high-precision tensor network calculations. These results suggest that the lattice Chern-Simons theory can simplify the complicated topological phase transitions to effective mean-field theories in terms of fermionic degrees of freedom, which lead to different understandings that help to understand the frustrated quantum magnets.
Based on the Chern-Simons fermionization of spin-1/2 operators, we propose a systematic framework to investigate the competition between emergent phases in frustrated two-dimensional XY quantum magnets. Application of the method to the antiferromagnetic honeycomb spin-1/2 J1J_1J1​-J2J_2J2​ XY model reveals an unconventional phase transition between two Chern-Simons orders: the Chern-Simons superconductor and the exciton insulator of Chern-Simons fermions. We show that in the spin language, this transition translates to the transition from the planar Néel state to the non-uniform chiral spin-liquid that was proposed earlier in the literature. Namely, the Chern-Simons superconductor describes the planar Néel state, while the Chern-Simons exciton insulator corresponds to the non-uniform chiral spin-liquid. These results are further confirmed by our high-precision tensor network calculation, which provides the first numerical evidence for the transition from Néel order to a non-uniform chiral spin-liquid. We argue that the developed method can be applied to other frustrated quantum magnets of XXZ type and can detect unconventional phase transitions.
Two-dimensional quantum antiferromagnets host rich physics, including long-range ordering, high-Tc{T}_{c}Tc​ superconductivity, quantum spin-liquid behavior, topological ordering, a variety of other exotic phases, and quantum criticalities. Frustrating perturbations in antiferromagnets may give rise to strong quantum fluctuations, challenging the theoretical understanding of the many-body ground state. Here we develop a method to describe the quantum antiferromagnets using fermionic degrees of freedom. The method is based on a formally exact mapping between spin-exchange models and theories describing fermionic matter with the emergent U(1)\text{U}(1)U(1) Chern-Simons gauge field. For the planar N\'eel state, this mapping self-consistently generates the Chern-Simons superconductor mean-field ground state of introduced spinless fermions. We systematically compare the Chern-Simons superconductor state with the planar N\'eel state at the level of collective modes as well as order parameters. We reveal qualitative and quantitative correspondences between these two states. We demonstrate that such a construction using the fractionalized excitations and Chern-Simons gauge field can not only describe the N\'eel order, but can also be applied to study quantum spin liquids. Furthermore, we show that the confinement-deconfinement transitions from the N\'eel order to quantum spin liquids are signaled and characterized by the instabilities of Chern-Simons superconductors, driven by strong frustration. The results suggest observing and classifying the descendants of antiferromagnets, including other ordered states and unconventional superconductors, as well as emergent quantum spin liquids.
We develop an approach to describe antiferromagnetic magnons on a bipartite lattice supporting the N\'eel state using fractionalized degrees of freedom typically inherent to quantum spin liquids. In particular, we consider a long-range magnetically ordered state of interacting two-dimensional quantum spin-1/21/21/2 XY models using the Chern-Simons (CS) fermion representation of interacting spins. The interaction leads to Cooper instability and pairing of CS fermions, and to CS superconductivity which spontaneously violates the continuous U(1)\mathrm{U}(1)U(1) symmetry generating a linearly dispersing gapless Nambu-Goldstone mode due to phase fluctuations. We evaluate this mode and show that it is in high-precision agreement with magnons of the corresponding N\'eel antiferromagnet irrespective to the lattice symmetry. Using the fermion formulation of the system with frustration, we show that the competing interactions emerge in the form of long-range interaction vertices mediated by the CS gauge field, which are responsible for restoring the continuous symmetry at sufficiently strong frustration. We identify these new interaction vertices and discuss their implications for unconventional phase transitions. We also apply the proposed theory to a model of anyons that can be tuned continuously from fermions to bosons, and discuss the results.
Quantum phase transitions in quantum magnets constitute an important field that has attracted great interests. Although a variety of analytic and numerical methods have been introduced in this direction, faithful fermionic descriptions are still desired because they can transform the spin models to a form tractable by conventional many-body techniques, yielding more transparent physical pictures. We generalize the Chern-Simons fermionization approach and apply it to the XXZ quantum magnets. After fermionzation, the Ising interaction of the XXZ spin model leads to a fermion-fermion interaction. We show that the additional fermion-fermion interaction generates an interesting phase transition between two fermionic ordered states, i.e., the Chern-Simons superconductor and the Chern-Simons exciton insulator. We also demonstrate that this transition in the fermionic language essentially describes the quantum phase transition between the planar and out-of-plane N\'eel orders in the spin picture. The fermionic mean-field theory further leads to a nonlinear $\ensuremath{\sigma}$ model that describes the quantum phase transition, which is further supported by our density matrix renormalization group calculations in the original spin model. Our work introduces a fermionic interpretation of quantum phase transitions and advances the existing knowledge of quantum magnets.
Chiral topological orders formed in correlated fermion systems have been widely explored. However, the mechanism of how they emerge from interacting fermions is still unclear. Here, we propose a susceptibility condition. Under this condition, we show that chiral topological orders can spontaneously take place in correlated fermion systems. The condition leads to a low-energy effective theory of bosons with strong frustration, mimicking flat-band systems. The frustration then melts the long-range orders and results in topological orders with time-reversal symmetry breaking. We apply the theory to strongly correlated semiconductors doped to the metallic phase. An excitonic topological order with semionic excitations and a chiral excitonic edge state is revealed. We also discuss the application to frustrated magnets. The theory predicts a chiral spin-liquid state, which is numerically confirmed by our tensor network calculations. These results demonstrate an indicator for chiral topological orders, which bridges the existing gap between interacting fermions and correlated topological matter.
Quantum spin liquids (QSLs) are highly entangled states of quantum magnets which lie beyond the Landau paradigm of classifying phases of matter via broken symmetries. A physical route to arriving at QSLs is via frustration-induced quantum melting of ordered states such as valence bond crystals or magnetic orders. Here we show, using extensive exact diagonalization (ED) and density-matrix renormalization group (DMRG) studies of concrete SU(2)SU(2)SU(2) invariant spin models on honeycomb, triangular, and square lattices, that chiral spin liquids (CSLs) emerge as descendants of triple-QQQ spin crystals with tetrahedral magnetic order and a large scalar spin chirality. Such ordered-to-CSL melting transitions may yield lattice realizations of effective Chern-Simons-Higgs field theories. Our work provides a distinct unifying perspective on the emergence of CSLs and suggests that materials with certain noncoplanar magnetic orders might provide a good starting point to search for CSLs.