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Optics Communications

Competition of collimated ultraviolet lights generated by four-wave mixing process in Cs vapor

Shu Hu, Baodong Gai, Juntao Li, Ying Chen, Xianglong Cai, Pengyuan Wang, Jinbo Liu, Jingwei Guo

Published Sep 6, 2022• 4 citations
Publisher
DOI
10.1016/j.optcom.2022.128960

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Collimated ultraviolet (UV) light is generated via four-wave mixing (FWM) in cesium vapor by continuously tuning the wavelength of the pump laser. Terahertz (THz) Stokes light is generated by the stimulated Raman scattering (SRS) effect in the FWM process, and its frequency is adjustable. When exciting the cesium atom to a virtual level using different combinations of pump lasers (P1 and P2), the strength distribution of UV light is asymmetric, which can be explained through a phase-matching mechanism. Furthermore, the SRS effect and phase matching influence the FWM.
We demonstrate the generation of polychromatic and collimated lights at 456 nm, 459 nm, and 761 nm based on cesium ( 133 Cs) 6S 1/2 - 6P 3/2 - 8S 1/2 - 7P 3/2 , 7P 1/2 , 6P 1/2 - 6S 1/2 multi-diamond-type atomic system via two-photon excitation with two IR pump lasers at 852 nm and 795 nm. The 456 nm, 459 nm (7P 3/2 , 7P 1/2 → 6S 1/2 ) collimated blue lights result from the self-seeded four-wave mixing process (FWM), and the 761 nm coherent light (8S 1/2 → 6P 1/2 ) is from a seeded FWM process with the injection of a third laser at 895 nm. We measure the dependency of generated polychromatic fields on the temperature of 133 Cs vapor cell and the powers of input lasers, clearly demonstrating the competition between the self-seeded FWM and seeded FWM, as they share the same excitation path. This work is helpful to further produce entangled multi-color photons for quantum communication.