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The Multi-Photon Induced Fano Effect

K. L. Litvinenko

Published Sep 12, 2019• 0 citations
Publisher

Abstract

The ordinary Fano effect occurs in many-electron atoms and requires an auto-ionizing state.With such a state, photo-ionization may proceed via pathways that interfere, and the characteristicasymmetric resonance structures appear in the continuum. Here we demonstrate that Fano structure15may also be induced without need of auto-ionization, by dressing the continuum with an ordinarybound state in any atom by a coupling laser. Using multi-photon processes gives complete, ultra-fastcontrol over the interference. We show that a line-shape indexqnear unity (maximum asymmetry)may be produced in hydrogenic silicon donors with a relatively a weak beam. Since the Fanolineshape has both constructive and destructive interference, the laser control opens the possibility20of state-selective detection with enhancement on one side of resonance and invisibility on the other.We discuss a variety of atomic and molecular spectroscopies, and in the case of silicon donors weprovide a calculation for a qubit readout application

DOI
10.5281/zenodo.3406203

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The ordinary Fano effect occurs in many-electron atoms and requires an auto-ionizing state.With such a state, photo-ionization may proceed via pathways that interfere, and the characteristicasymmetric resonance structures appear in the continuum. Here we demonstrate that Fano structure15may also be induced without need of auto-ionization, by dressing the continuum with an ordinarybound state in any atom by a coupling laser. Using multi-photon processes gives complete, ultra-fastcontrol over the interference. We show that a line-shape indexqnear unity (maximum asymmetry)may be produced in hydrogenic silicon donors with a relatively a weak beam. Since the Fanolineshape has both constructive and destructive interference, the laser control opens the possibility20of state-selective detection with enhancement on one side of resonance and invisibility on the other.We discuss a variety of atomic and molecular spectroscopies, and in the case of silicon donors weprovide a calculation for a qubit readout application
The ordinary Fano effect occurs in many-electron atoms and requires an autoionizing state. With such a state, photo-ionization may proceed via pathways that interfere, and the characteristic asymmetric resonance structures appear in the continuum. Here we demonstrate that Fano structure may also be induced without need of auto-ionization, by dressing the continuum with an ordinary bound state in any atom by a coupling laser. Using multi-photon processes gives complete, ultra-fast control over the interference. We show that a line-shape index q near unity (maximum asymmetry) may be produced in hydrogenic silicon donors with a relatively weak beam. Since the Fano lineshape has both constructive and destructive interference, the laser control opens the possibility of state-selective detection with enhancement on one side of resonance and invisibility on the other. We discuss a variety of atomic and molecular spectroscopies, and in the case of silicon donors we provide a calculation for a qubit readout application.
States behaving like autoionizing states can be selectively induced by laser radiation into one of the continuum spin channels in the photoionization of polarized excited alkaki atoms. As a result of destructive or constructive interference between the direct ionization channel and those introduced by the dressing laser radiation, the cross section of this specific spin component is completely suppressed or enhanced, while leaving the other spin channel unaffected. The qqq parameter which determines the line shape of the Fano-type resonance can be resonantly tuned as a function of the dressing laser frequency.
Spectroscopic signatures associated with symmetric Lorentzian and asymmetric Fano line shapes are ubiquitous. Distinct features of Fano resonances in contrast with conventional symmetric resonances have found several applications in photonics such as optical switching, sensing, lasing, and nonlinear and slow-light devices. It is therefore important to effectively generate and control these resonances. In this work, we show through ab initio simulations of coupled light–matter systems that Fano interference phenomena can be realized in a multimode photonic environment by strong coupling to the electromagnetic continuum. Specifically, we show that by effectively enhancing the light–matter coupling strength to the photon continuum in an experimentally feasible way, we can achieve a transition from Lorentzian to Fano lines shapes for both electronic and polaritonic excitations. An important outcome of switching between these spectral signatures is the possibility to control the Purcell enhancement of spontaneous emission alongside electromagnetically induced transparency, which is a special case of Fano resonances. Switching from Fano back to a Lorentzian profile can be achieved by physically reducing the coupling strength to the continuum of modes. Our results hold potential for realizing tunable Fano resonances of molecules and materials interacting with the electromagnetic continuum within multimode photonic environments.
Photon absorption spectroscopy is a powerful tool for uncovering the structure of atoms, molecules, and solids. Symmetric Lorentzian and asymmetric Fano line shapes are fundamental spectroscopic signatures related to the structural and dynamical properties. Recently, Ott et al. [Science 340, 716 (2013)] successfully transferred Fano profile into Lorentzian line shape using an intense infrared laser, after excitation of autoionizing states in helium by attosecond XUV pulse. This is a very important step forward in quantum phase control. However, here we show experimentally that an autoionizing state can have both Fano and Lorentzian behavior naturally, depending on the process involved. This study utilized the inverse process of photon absorption ionization, i.e., electron ion recombination with photon emission, making sure the resonant autoionizing state is not modified or decorated by the laser fields. Our result implies that excitation of the state through different paths---for example, one photon versus multiphoton excitation, or even one step versus multistep excitation---can lead to different Fano profiles for the same resonant state. We also report an experimental determination of the energy shifts in the recombination photon-intensity peaks due to the interference between the resonant and nonresonant processes.
We know that the Fano profile is obtained for single-photon absorption to the ionization continuum in the presence of an autoionizing state. We have shown that, in the case of (1+1)-photon absorption to an autoionizing state embedded in the ionization continuum, the absorption profile changes radically to a mirror image of the Fano profile for the value of q=\ifmmode\pm\else\textpm\fi{}1, q being the Fano q parameter. Moreover, for higher values of q, the (1+1)-photon absorption profile exhibits a broad minimum, while a distinct interference pattern is obtained in the profile of single-photon absorption. The absorption line shape has been found to oscillate between the Fano and a modified Fano profile for the autoionization through odd and even number of steps, respectively, via resonances.