An atomic system that can be addressed via a single optical mode, hereafter called a one-dimensional atom, is central for many applications in optical quantum technologies. A cavity with a large Purcell factor is required to collect the emission efficiently, but a small Purcell factor is required for long-time memory storage. Here, we introduce an effective and versatile one-dimensional atom consisting of two interacting quantum emitters efficiently coupled to a cavity mode with a large Purcell factor. The dipole–dipole interaction gives rise to a subradiant state with a tunable bandwidth. We demonstrate generation of time-shaped single photons and implementation of quantum memory. We discuss experimental challenges and practical implementation using different systems.
Optical nonlinearities at the single-photon level are key features to build efficient photon-photon gates and to implement quantum networks. Such optical nonlinearities can be obtained using an ideal two-level system such as a single atom coupled to an optical cavity. While efficient, such atom-photon interface however presents a fixed bandwidth, determined by the spontaneous emission time and thus the spectral width of the cavity-enhanced two-level transition, preventing an efficient transmission to bandwidth-mismatched atomic systems in a single quantum network. In the present work, we propose a tunable atom-photon interface making use of the direct dipole-dipole coupling of two slightly different atomic systems. We show that, when weakly coupled to a cavity mode and directly coupled through dipole-dipole interaction, the subradiant mode of two slightly detuned atomic systems is optically addressable and presents a widely tunable bandwidth and single-photon nonlinearity.
Motivated by developments in quantum information science, much recent effort has been directed toward coupling individual quantum emitters to optical microcavities. Such systems can be used to produce single photons on demand, enable nonlinear optical switching at a single photon level, and implement functional nodes of a quantum network, where the emitters serve as processing nodes and photons are used for long-distance quantum communication. For many of these practical applications, it is important to develop techniques that allow one to generate outgoing single photons of desired frequency and bandwidth, enabling hybrid networks connecting different types of emitters and long-distance transmission over telecommunications wavelengths. Here, we propose a novel approach that makes use of a nonlinear optical resonator, in which the single photon originating from the atom-like emitter is directly converted into a photon with desired frequency and bandwidth using the intracavity nonlinearity. As specific examples, we discuss a high-finesse, TE-TM double-mode photonic crystal cavity design that allows for direct generation of single photons at telecom wavelengths starting from an InAs/GaAs quantum dot with a 950 nm transition wavelength, and a scheme for direct optical coupling of such a quantum dot with a diamond nitrogen-vacancy center at 637 nm.
Much recent effort has focused on coupling individual quantum emitters to optical microcavities in order to produce single photons on demand, enable single-photon optical switching, and implement functional nodes of a quantum network. Techniques to control the bandwidth and frequency of the outgoing single photons are of practical importance, allowing direct emission into telecommunications wavelengths and "hybrid" quantum networks incorporating different emitters. Here, we describe an integrated approach involving a quantum emitter coupled to a nonlinear optical resonator, in which the emission wavelength and pulse shape are controlled using the intra-cavity nonlinearity. Our scheme is general in nature, and demonstrates how the photonic environment of a quantum emitter can be tailored to determine the emission properties. As specific examples, we discuss a high Q-factor, TE-TM double-mode photonic crystal cavity design that allows for direct generation of single photons at telecom wavelengths (1425 nm) starting from an InAs/GaAs quantum dot with a 950 nm transition wavelength, and a scheme for direct optical coupling between such a quantum dot and a diamond nitrogen-vacancy center at 637 nm.
Quantum memories are a key technology for distributing entanglement in large-scale quantum networks. They allow for coherent control and temporal reordering of single photons which is a fundamental prerequisite for quantum repeaters, local synchronization and buffering of quantum information. These applications require bright and pure sources of indistinguishable single photons, as well as long-lived, efficient, and high-bandwidth quantum memories with minimal noise. The demonstration of robust, scalable, multi-mode photonic interfaces between different types of quantum memories and single-photon sources remains an open experimental challenge. This work contributes to this endeavor by investigating a heterogeneous interface between a semiconductor quantum dot single-photon source and a room-temperature atomic vapor memory. The first part of this work presents the first room-temperature, ladder-type atomic vapor memory that operates on the Cs D1 line at 895\,nm. The performance of the memory is characterized using attenuated laser pulses at the single-photon level. The memory achieves an internal efficiency of
ηint=15(1)% at a storage time of
τs=17.4(2)\,ns. We derive a quantitative benchmark for the memory compatibility with quantum dot single-photon sources. The memory's high signal-to-noise ratio of 830(80), and its spectral acceptance window of
W=560\,MHz promise compatibility with single photons from state-of-the-art InGaAs quantum dot devices. Furthermore, we present such a nano-integrated quantum dot device and characterize its optical properties. We measure a radiative lifetime of 1.3(1)\,ns and an inhomogeneously broadened linewidth of 5.1(1)\,GHz. The temperature tuning of the emission wavelength to the Cs D1 line allows coupling of the quantum dot to the memory in a joint experiment. The storage of single photons from a quantum dot source in a room-temperature atomic memory is demonstrated with on-demand retrieval. The variable storage time of up to
τs=19.8\,ns and the memory's fractional delay of
Df=14(1) present a significant advancement in the research field. We compare our results with other types of interfaces between single-photon sources and quantum memories and discuss the performance in the context of quantum network applications. This work marks an important step towards local buffering and synchronization of quantum information in heterogeneous quantum network nodes.
A quantum emitter interacting with photons in a single optical-mode constitutes a one-dimensional atom. A coherent and efficiently coupled one-dimensional atom provides a large nonlinearity, enabling photonic quantum gates. Achieving a high coupling efficiency (β factor) and low dephasing is challenging. Here, we use a semiconductor quantum dot in an open microcavity as an implementation of a one-dimensional atom. With a weak laser input, we achieve an extinction of 99.2% in transmission and a concomitant bunching in the photon statistics of g^{(2)}(0)=587, showcasing the reflection of the single-photon component and the transmission of the multi-photon components of the coherent input. The tunable nature of the microcavity allows β to be adjusted and gives control over the photon statistics-from strong bunching to antibunching-and the phase of the transmitted photons. We obtain excellent agreement between experiment and theory by going beyond the single-mode Jaynes-Cummings model. Our results pave the way towards the creation of exotic photonic states and two-photon phase gates.