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Physica Scripta

A giant self-Kerr nonlinearity using phase-sensitive excitation in a closed three-level atomic system

Ayyappan J, T. Beena

Published Jul 13, 2022• 8 citations
Publisher

Abstract

Abstract A third-order nonlinear response is investigated theoretically using a closed lambda system. In this scheme, a pair of optical fields and a microwave field connect three hyperfine levels in a cyclic fashion, rendering the atomic response sensitive to the relative phase of all three fields. Changing the relative phase, we can suppress the linear response of the probe field and enhance its third order self-Kerr nonlinear response using the underlying electromagnetically induced transparency (EIT) effect. The resultant giant self-Kerr nonlinear response is comparable to or exceeding that found in atomic systems at room temperature. Most importantly, we show that the self-Kerr nonlinear response at an optical frequency can be controlled using the phase and amplitude of a frequency-separated microwave field.

DOI
10.1088/1402-4896/ac80db

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Physical Review A•May 14, 2015•94 citations
Abstract A third-order nonlinear response is investigated theoretically using a closed lambda system. In this scheme, a pair of optical fields and a microwave field connect three hyperfine levels in a cyclic fashion, rendering the atomic response sensitive to the relative phase of all three fields. Changing the relative phase, we can suppress the linear response of the probe field and enhance its third order self-Kerr nonlinear response using the underlying electromagnetically induced transparency (EIT) effect. The resultant giant self-Kerr nonlinear response is comparable to or exceeding that found in atomic systems at room temperature. Most importantly, we show that the self-Kerr nonlinear response at an optical frequency can be controlled using the phase and amplitude of a frequency-separated microwave field.
In this work, we present an analytical method to achieve giant Kerr nonlinearity without absorption in a five-level atomic medium. By using iterative perturbation technique on density matrix equations, we have derived the analytical expressions of nonlinear susceptibility and Kerr nonlinear coefficient in the presence of spontaneously generated coherence (SGC) and relative phase between applied laser fields. It shows that, this five-level atomic medium exhibits multiple electromagnetically induced transparency (EIT) at three different frequencies, at the same time, the Kerr nonlinear coefficient is enhanced around three transparent spectral regions; in each such EIT region appears a pair of positive-negative peaks of Kerr nonlinear coefficient. In particular, these nonlinear peaks are moved to the center of the EIT windows via SGC. This means that the Kerr nonlinear coefficient is enhanced with completely suppressed absorption at different transparency frequencies. Furthermore, the magnitude and the sign of the Kerr nonlinear coefficient are easily controlled according to the SGC strength, the coupling laser intensity, and the relative phase between applied laser fields. Such a giant nonlinear medium can be useful for photonic devices working in the resonant frequency region without absorption. As a typical application, this giant Kerr nonlinear material has been applied to an interferometer for the formation of optical bistability, and showed the appearance of OB at the resonant frequency with significantly reduced threshold intensity and OB width.
In this work, Electromagnetically Induced Transparency (EIT) has been studied in a microwave driven closed cyclic Lambda atomic system. It is observed that in the absence of microwave field a normal transparency window is obtained, but when a microwave field is also applied between hyperfine levels along with the optical fields an amplification and attenuation in EIT signal is observed depending upon the relative phase between fields driving the atomic system. In fact, a new probe field is generated by microwave and coupling field which interfere constructively or destructively with incident probe field leading to either amplification, attenuation or asymmetricity in probe transmission signal. Also, dependency of phase sensitive amplification on ground state decoherence is also studied. This novel, controllable and amplified EIT signal can be potentially used for the transfer of coherent microwave analog or digital message signal over larger distance using optical fibers where amplification is preliminary requirement.
We study the nonlinear effect in a three-level atomic system in Λ configuration. As two or more fields are confined within the common electromagnetically induced transparency (EIT) window, they directly disturb EIT dark state at the same time, which leads to the self- and cross-Kerr nonlinear interactions. Our scheme is different from the existed schemes based on three-level or multilevel systems only existing single type of nonlinear interactions. In the common EIT windows, the self- and cross-Kerr nonlinearities are established with suppressed linear absorption and our scheme can be generalized polychromatic Kerr nonlinearity. Because the atoms are almost trapped in the ground states and the atom population becomes unchanged, the scheme is robust to the atomic spontaneous emission. Our scheme is a promising avenue for preparation of squeezing and entanglement .
In this paper, we propose an analytical model to study the effect of Doppler broadening on self-Kerr nonlinearity in a five-level ladder-type atomic system. First- and third-order susceptibilities and the self-Kerr nonlinear coefficient are found as the function of temperature and parameters of laser fields. The analytical model is applied to hot $^{85}{\rm Rb}$85Rb and $^{87}{\rm Rb}$87Rb atoms, and it is shown that under the electromagnetically induced transparency (EIT) effect, the self-Kerr nonlinear coefficient is enhanced around three transparent spectral regions. When the temperature of atomic vapor increases (i.e., Doppler width increases), the depth and width of the EIT windows decrease accordingly, and therefore the amplitude of the Kerr nonlinear coefficient decreases significantly. In addition, because the frequency gaps between hyperfine levels of upper excited state ${{5\rm D}_{5/2}}$5D5/2 of $^{85}{\rm Rb}$85Rb atoms are much smaller than those of $^{87}{\rm Rb}$87Rb atoms, the EIT windows as well as the nonlinear dispersion curves for $^{85}{\rm Rb}$85Rb atoms are closer than those for $^{87}{\rm Rb}$87Rb atoms as the Doppler effect presents. The analytical results agree well with the experimental observation when reducing to a three-level atomic system. The analytical model can be used to easily fit the experimental observations of self-Kerr nonlinearity in a five-level atomic system under different temperature conditions and apply to a variety of applications relating to all-optical-switching techniques.
Abstract We study the enhancement of cross-Kerr nonlinearity in a six-level inverted-Y-type inhomogeneously broadened atomic medium. The explicit analytical expressions for first- and third-order susceptibilities and cross-Kerr nonlinear coefficient are found in the presence of Doppler broadening. The analytical model is applied to 87 Rb atoms and it is shown that under the electromagnetically induced transparency (EIT) condition, the cross-Kerr nonlinearity is enhanced at multiple frequencies around three EIT windows. The amplitude and sign of the cross-Kerr nonlinear coefficient of the probe field are controlled by changing the parameters of the coupling field. The effect of Doppler broadening leads to a reduction in the transparent efficiency and thus reduces the amplitude of the cross-Kerr nonlinear coefficient. The analytical model can be used to easily fit the experimental observations at different temperatures and support future studies related to the cross-Kerr nonlinear effect.
The third-order susceptibility is investigated in a five-level atomic system in which the laser beams couple the ground state to a four-level closed-loop system. It is found that under the condition of the multiphoton resonance, one can enhance the Kerr nonlinearity of such a medium by properly adjusting the amplitudes and phases of the applied fields. In this case, the linear and nonlinear absorption reduce considerably in a region with a positive group velocity. It is demonstrated that the third-order susceptibility is very sensitive to the relative phase of the applied fields. An analytical model is presented to elucidate such phase control of the Kerr nonlinearity. A comparison is also made between the Kerr-nonlinear indices for the five-, four-, and three-level systems. It is realized that the magnitude of the Kerr nonlinearity for the five-level system is larger than that of the three- and four-level counterparts. Finally, it is shown that effect of Doppler broadening can lead to an enhanced Kerr nonlinearity while maintaining linear and nonlinear absorption.