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The European Physical Journal Plus

Pump-probe optical response of a semiconductor quantum dot-metallic nanosphere hybrid system

Elife Öznur Karabulut, İbrahim Karabulut

Published Jul 1, 2022• 3 citations
Publisher
DOI
10.1140/epjp/s13360-022-03028-4

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We study optical effects in a hybrid system composed of a semiconductor quantum dot (SQD) and a spherical metal nanoparticle (MNP) that interacts with a weak probe and a strong pump electromagnetic field. We use modified nonlinear density matrix equations for the description of the optical properties of the system and calculate, numerically, the first-order susceptibilities of the SQD, the MNP, and the total hybrid nanostructure of the probe field in the presence of the pump field. We investigate the dependence of the probe absorption and dispersion spectra of the SQD, the MNP, and the total nanostructure on the interparticle distance and the detuning of the pump field, and stress the influence of the MNP contribution to the total optical response. The results we find are explained according to the theory of two distinct metastates, which constitute conjugations of the SQD excitonic and the MNP plasmonic excitations. We also show that the optical response strongly depends on the actual values of the SQD material parameters.
Abstract Splitting of the effective Rabi frequencies for plasmonic fields when the interaction occurs between semiconductor quantum dot and three metallic nanospheres in the presence of three electromagnetic fields is examined. We study theoretically the role of the dipole–dipole interactions in creating many Multipoles. Then, we split the effective Rabi frequencies into three parts according to the quantitative Multipoles of the plasmonic fields. The density matrix equations are derived for the description of the optical properties of the SQD-MNPs nanosystem. We investigate the influence of each part of the effective Rabi frequencies and compare them with each other individually. The three parts of the effective Rabi frequency for the probe field are affected by changing the angles, the strong probe field and other parameters for the hybrid system.
In the present work, we investigate the modified nonlinear pump-probe optical properties due to the excitonic–plasmonic interaction of a double semiconductor quantum dot (SQD) molecule coupled to a metal nanoparticle (MNP). More specifically, we study the absorption and the dispersion spectra of a weak electromagnetic field in a hybrid structure with two counterparts, a molecule of two coupled SQDs, and a spherical MNP driven by a field of high intensity. We solve the relevant density matrix equations, calculate the first-order optical susceptibility of the probe field in the strong pumping regime, and investigate the way in which the distance between the two counterparts modifies the optical response, for a variety of values of the physical constants of the system, including the pump-field detuning, the tunnelling rate, and the energy separation gap associated with the excited states of the coupled SQDs.