Abstract Time crystals represent temporal analogues of the spatial self-ordering exhibited by atomic or molecular building blocks of solid-state crystals. The pursuit of discrete time crystals (DTCs) in periodically forced Floquet closed systems has revealed how they can evade thermalization and loss of temporal order. Recently, it has been shown that even with coupling to the ambient and its concomitant noise, some states maintain their time crystalline order, formingdissipativeDTCs. Here, we introduce a scheme for the realization and state control of dissipative DTCs hinging on pumping a Kerr optical resonator with a phase-modulated continuous-wave laser. We show the possible symmetry breaking states possess temporal long-range order and analyze the phase noise of the accompanying signature radio frequency (RF) subharmonic. Besides offering a technique for generating high-spectral-purity RF signals, this versatile platform empowers controlled switching between various DTC states through accessible experimental knobs, hence facilitating the future study of DTC phase transitions.
Abstract Time crystals represent temporal analogues of the spatial self-ordering exhibited by atomic or molecular building blocks of solid-state crystals. The pursuit of discrete time crystals (DTCs) in periodically forced Floquet closed systems has revealed how they can evade thermalization and loss of temporal order. Recently, it has been shown that even with coupling to the ambient and its concomitant noise, some states maintain their time crystalline order, formingdissipativeDTCs. Here, we introduce a scheme for the realization and state control of dissipative DTCs hinging on pumping a Kerr optical resonator with a phase-modulated continuous-wave laser. We show the possible symmetry breaking states possess temporal long-range order and analyze the phase noise of the accompanying signature radio frequency (RF) subharmonic. Besides offering a technique for generating high-spectral-purity RF signals, this versatile platform empowers controlled switching between various DTC states through accessible experimental knobs, hence facilitating the future study of DTC phase transitions.
Discrete (DTCs) and continuous time crystals (CTCs) are novel dynamical many-body states, that are characterized by robust self-sustained oscillations, emerging via spontaneous breaking of discrete or continuous time translation symmetry. DTCs are periodically driven systems that oscillate with a subharmonic of the external drive, while CTCs are continuously driven and oscillate with a frequency intrinsic to the system. Here, we explore a phase transition from a continuous time crystal to a discrete time crystal. A CTC with a characteristic oscillation frequencyωCTCis prepared in a continuously pumped atom-cavity system. Modulating the pump intensity of the CTC with a frequencyωdrclose to2ωCTCleads to robust locking ofωCTCtoωdr/2, and hence a DTC arises. This phase transition in a quantum many-body system is related to subharmonic injection locking of non-linear mechanical and electronic oscillators or lasers.
Non-equilibrium Rydberg gases exhibit exotic many-body phases stabilized by the interplay of coherent interactions and dissipation. Strong Rydberg interactions drive sustained limit cycle oscillations, whose robustness, long-range temporal order, and spontaneous time-translation symmetry breaking establish a dissipative time crystal (DTC). Collective self-entrainment in driven ensembles leads to global synchronization and a dominant oscillation frequency. Here, injection locking of a Rydberg DTC is demonstrated using a radio-frequency (RF) electric field that gradually pulls the intrinsic oscillation toward the injected frequency. Above a critical threshold, full synchronization occurs, with the locking bandwidth scaling linearly with RF amplitude. This includes synchronization of higher-order harmonics, revealing entrainment of the system's nonlinear temporal dynamics. The phenomenon parallels injection locking in classical nonlinear systems, but emerges here in a strongly interacting quantum medium. This approach establishes a new method for stabilizing and controlling time-crystalline temporal order, with applications in precision sensing, quantum metrology, and timekeeping.
Non-equilibrium Rydberg gases exhibit exotic many-body phases stabilized by the interplay of coherent interactions and dissipation. Strong Rydberg interactions drive sustained limit cycle oscillations, whose robustness, long-range temporal order, and spontaneous time-translation symmetry breaking establish a dissipative time crystal (DTC). Collective self-entrainment in driven ensembles leads to global synchronization and a dominant oscillation frequency. Here, injection locking of a Rydberg DTC is demonstrated using a radio-frequency (RF) electric field that gradually pulls the intrinsic oscillation toward the injected frequency. Above a critical threshold, full synchronization occurs, with the locking bandwidth scaling linearly with RF amplitude. This includes synchronization of higher-order harmonics, revealing entrainment of the system’s nonlinear temporal dynamics. The phenomenon parallels injection locking in classical nonlinear systems, but emerges here in a strongly interacting quantum medium. This approach establishes a new method for stabilizing and controlling time-crystalline temporal order, with applications in precision sensing, quantum metrology, and timekeeping. Non-equilibrium Rydberg gases exhibit unique many-body phases arising from the interplay of coherent interactions and dissipation, yet controlling their temporal order remains challenging. This work demonstrates injection locking of a Rydberg dissipative time crystal using a radio-frequency electric field, achieving full synchronization and revealing dynamical behavior relevant to precision sensing and quantum metrology.
Periodically driven quantum systems host a range of non-equilibrium phenomena which are unrealizable at equilibrium. Discrete time-translational symmetry in a periodically driven many-body system can be spontaneously broken to form a discrete time crystal, a putative quantum phase of matter. We present the observation of discrete time crystalline order in a driven system of paramagnetic P -donor impurities in isotopically enriched 28Si cooled below 10 K. The observations exhibit a stable subharmonic peak at half the drive frequency which remains pinned even in the presence of pulse error, a signature of DTC order. We propose a theoretical model based on the paradigmatic central spin model which is in good agreement with experimental observations, and investigate the role of dissipation in the stabilisation of the DTC. Both experiment and theory indicate that the order in this system is primarily a dissipative effect, and which persists in the presence of spin-spin interactions. We present a theoretical phase diagram as a function of interactions and dissipation for the central spin model which is consistent with the experiments. This opens up questions about the interplay of coherent interaction and dissipation for time-translation symmetry breaking in many-body Floquet systems.
A discrete time crystal (DTC) is an essentially nonequilibrium phase that breaks discrete time-translation symmetry in periodically driven (Floquet) systems.In ideal isolated quantum systems without dissipation, many kinds of DTCs have been theoretically proposed and experimentally verified in various artificial quantum systems, such as trapped ions, NV centers in diamond, and quantum computers.However, in real physical systems, we cannot avoid dissipation stemming from coupling to an external environment.Nevertheless, the effects of dissipation on DTCs have not been fully explored yet.This thesis reports the author's two original studies on dissipative DTCs.First, we formulate a symmetry-based theory of dissipative DTCs.To this end, we introduce Floquet dynamical symmetry (FDS) governing the long-time dynamics of dissipative Floquet systems.The FDS protects the quantum coherence of the system from dissipation and dephasing and leads to two types of time crystals: the discrete time crystal (DTC) and discrete time quasicrystal (DTQC), which are different in periodicity.We show that these time crystals appear in spin-S Bose-and Fermi-Hubbard models driven by an ac field and that their periodicity can be tuned by adjusting the field strength.Since these time crystals rely on the FDS alone, they appear even in the presence of perturbations as long as the FDS exists.We also elucidate that the FDS explains the symmetry structure behind the conventional DTCs proposed in the previous studies.Second, we investigate dissipative DTCs in solid-state materials by considering a dissipative quantum Ising model periodically driven by π-pulses.While the previous studies on dissipative DTCs have focused on well-controllable artificial quantum systems, we show that realistic dissipation in solids does not destroy but can stabilize the DTC order.Using the time-dependent mean-field theory, we analyze the DTC phase transition and determine critical exponents, including a dynamical one.We also find a novel reentrant phase transition in varying the pulse interval.This transition is due to a nontrivial interplay of the periodic drive and dissipation and has no equilibrium counterparts in the corresponding undriven system.Furthermore, to demonstrate the rigidity (stability) of the DTC, we consider imperfect πpulses, showing that the DTC is robust against minor imperfections and finding that DTQC appears for major imperfections.These results uncover a general symmetry aspect of dissipative DTCs and lay the foundation for realizing DTCs in material science.
We consider a dissipative quantum Ising model periodically driven by a train of $\ensuremath{\pi}$ pulses and investigate dissipative discrete time crystals (DTCs) in solids. In this model, the interaction between the spins spontaneously breaks the discrete time translation symmetry, giving rise to a dissipative DTC, where two ferromagnetic states are switched alternately by each pulse. We microscopically describe the generic dissipation due to thermal contact to an equilibrium heat bath using the Bloch-Redfield equation. In contrast to other DTC studies, this dissipation stabilizes, rather than destroys, the DTC order without fine-tuning as long as the temperature is low enough. Invoking the time-dependent mean-field theory and solving self-consistently the periodic drive, dissipation, and DTC order parameter, we investigate the nonequilibrium DTC phase transition and determine the critical exponents, including a dynamical one. We also find phase transitions without an equilibrium counterpart: a nontrivial interplay of the periodic drive and dissipation gives rise to reentrant DTC transition when changing the pulse interval at a fixed temperature. Also, to demonstrate the rigidity of the DTC, we consider imperfect $\ensuremath{\pi}$ pulses, showing that the DTC is robust against the small imperfections and finding that discrete time quasicrystals can appear for the larger imperfections. Together with experimental proposals in magnetic materials, our results pave the way for realizing the DTC and for uncovering nonequilibrium critical phenomena in real solid-state materials.