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Scientific Reports

Numerical renormalization group study of the Loschmidt echo in Kondo systems

Tomasz Ślusarski, Kacper Wrześniewski, Ireneusz Weymann

Published Jun 13, 2022• 1 citation
Publisher

Abstract

We study the dynamical properties of the one-channel and two-channel spin-1/2 Kondo models after quenching in Hamiltonian variables. Eigen spectrum of the initial and final Hamiltonians is calculated by using the numerical renormalization group method implemented within the matrix product states formalism. We consider multiple quench protocols in the considered Kondo systems, also in the presence of external magnetic field of different intensities. The main emphasis is put on the analysis of the behavior of the Loschmidt echo L(t), which measures the ability of the system's revival to its initial state after a quench. We show that the decay of the Loschmidt echo strongly depends on the type of quench and the ground state of the system. For the one-channel Kondo model, we show that L(t) decays as, [Formula: see text], where [Formula: see text] is the Kondo temperature, while for the two-channel Kondo model, we demonstrate that the decay is slower and given by [Formula: see text]. In addition, we also determine the dynamical behavior of the impurity's magnetization, which sheds light on identification of the relevant time scales in the system's dynamics.

DOI
10.1038/s41598-022-14108-x

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We study the dynamical properties of the one-channel and two-channel spin-1/2 Kondo models after quenching in Hamiltonian variables. Eigen spectrum of the initial and final Hamiltonians is calculated by using the numerical renormalization group method implemented within the matrix product states formalism. We consider multiple quench protocols in the considered Kondo systems, also in the presence of external magnetic field of different intensities. The main emphasis is put on the analysis of the behavior of the Loschmidt echo L(t), which measures the ability of the system's revival to its initial state after a quench. We show that the decay of the Loschmidt echo strongly depends on the type of quench and the ground state of the system. For the one-channel Kondo model, we show that L(t) decays as, [Formula: see text], where [Formula: see text] is the Kondo temperature, while for the two-channel Kondo model, we demonstrate that the decay is slower and given by [Formula: see text]. In addition, we also determine the dynamical behavior of the impurity's magnetization, which sheds light on identification of the relevant time scales in the system's dynamics.
We investigate the time evolution of the Kondo resonance in response to a quench by applying the time-dependent numerical renormalization group (TDNRG) approach to the Anderson impurity model in the strong correlation limit. For this purpose, we derive within the TDNRG approach a numerically tractable expression for the retarded two-time nonequilibrium Green function $G(t+{t}^{\ensuremath{'}},t)$, and its associated time-dependent spectral function, $A(\ensuremath{\omega},t)$, for times ttt both before and after the quench. Quenches from both mixed valence and Kondo correlated initial states to Kondo correlated final states are considered. For both cases, we find that the Kondo resonance in the zero temperature spectral function, a preformed version of which is evident at very short times $t\ensuremath{\rightarrow}{0}^{+}$, only fully develops at very long times $t\ensuremath{\gtrsim}1/{T}_{K}$, where TK{T}_{K}TK​ is the Kondo temperature of the final state. In contrast, the final state satellite peaks develop on a fast time scale $1/\mathrm{\ensuremath{\Gamma}}$ during the time interval $\ensuremath{-}1/\mathrm{\ensuremath{\Gamma}}\ensuremath{\lesssim}t\ensuremath{\lesssim}+1/\mathrm{\ensuremath{\Gamma}}$, where $\mathrm{\ensuremath{\Gamma}}$ is the hybridization strength. Initial and final state spectral functions are recovered in the limits $t\ensuremath{\rightarrow}\ensuremath{-}\ensuremath{\infty}$ and $t\ensuremath{\rightarrow}+\ensuremath{\infty}$, respectively. Our formulation of two-time nonequilibrium Green functions within the TDNRG approach provides a first step towards using this method as an impurity solver within nonequilibrium dynamical mean field theory.
A detailed derivation of the recently proposed time-dependent numerical renormalization-group (TD-NRG) approach to nonequilibrium dynamics in quantum-impurity systems is presented. We demonstrate that the method is suitable for fermionic as well as bosonic baths. Comparisons with exact analytical results for the charge relaxation in the resonant-level model and for dephasing in the spin-boson model establish the accuracy of the method. The real-time dynamics of a single spin coupled to each type of bath is investigated. We use the TD-NRG to calculate the spin relaxation and spin precession of a single Kondo impurity. The short- and long-time dynamics are studied as a function of temperature in the ferromagnetic and antiferromagnetic regimes. The short-time dynamics agrees very well with analytical results obtained at second order in the exchange coupling JJJ. In the ferromagnetic regime, the transient spin decay is described by the scaling variable $x=2{\ensuremath{\rho}}_{F}\ensuremath{\mid}J(T)\ensuremath{\mid}Tt$. In the antiferromagnetic regime, the long-time decay is governed for T<TKT<{T}_{K}T<TK​ by the Kondo time scale 1∕TK1∕{T}_{K}1∕TK​. Here ${\ensuremath{\rho}}_{F}$ is the conduction-electron density of states, TK{T}_{K}TK​ is the Kondo temperature, and J(T)J(T)J(T) is the effective exchange coupling at temperature TTT. Results for spin precession are obtained by rotating the external magnetic field from the xxx axis to the zzz axis.
A boundary transfer matrix formulation allows to calculate the Loschmidt echo for one-dimensional quantum systems in the thermodynamic limit. We show that nonanalyticities in the Loschmidt echo and zeros for the Loschmidt amplitude in the complex plane (Fisher zeros) are caused by a crossing of eigenvalues in the spectrum of the transfer matrix. Using a density-matrix renormalization group algorithm applied to these transfer matrices, we numerically investigate the Loschmidt echo and the Fisher zeros for quantum quenches in the XXZ model with a uniform and a staggered magnetic field. We give examples---both in the integrable and the nonintegrable cases---where the Loschmidt echo does not show nonanalyticities although the quench leads across an equilibrium phase transition, and examples where nonanalyticities appear for quenches within the same phase. For a quench to the free fermion point, we analytically show that the Fisher zeros sensitively depend on the initial state and can lie exactly on the real axis already for finite system size. Furthermore, we use bosonization to analyze our numerical results for quenches within the Luttinger liquid phase.
The equilibrium physics of quantum impurities frequently involves a universal crossover from weak to strong reservoir-impurity coupling, characterized by single-parameter scaling and an energy scale TK{T}_{K}TK​ (Kondo temperature) that breaks scale invariance. For the noninteracting resonant level model, the nonequilibrium time evolution of the Loschmidt echo after a local quantum quench was recently computed explicitly [R. Vasseur, K. Trinh, S. Haas, and H. Saleur, Phys. Rev. Lett. 110, 240601 (2013)]. It shows single-parameter scaling with variable TKt{T}_{K}tTK​t. Here, we scrutinize whether similar universal dynamics can be observed in various interacting quantum impurity systems. Using density matrix and functional renormalization group approaches, we analyze the time evolution resulting from abruptly coupling two noninteracting Fermi or interacting Luttinger liquid leads via a quantum dot or a direct link. We also consider the case of a single Luttinger liquid lead suddenly coupled to a quantum dot. We investigate whether the field-theory predictions for the universal scaling as well as for the large-time behavior successfully describe the time evolution of the Loschmidt echo and the entanglement entropy of microscopic models. Our study shows that for the considered local quench protocols the above quantum impurity models fall into a class of problems for which the nonequilibrium dynamics can largely be understood based on the knowledge of the corresponding equilibrium physics.
We have studied the quadrupolar Kondo effect for an impurity in cubic environment with taking account of a singlet excited state Γ1Γ_1Γ1​, which models a Pr3+\mathrm{Pr}^{3+}Pr3+ ion with a non-Kramers double ground state Γ3Γ_3Γ3​. We have used the numerical renormalization group approach and determined the phase diagram with varying quadrupole Kondo coupling JJJ and Γ1Γ_1Γ1​ excitation energy ΔΔΔ. Two phases are found and identified as local Fermi liquid and non-Fermi liquid. This non-Fermi liquid phase is characteristic to the two-channel Kondo impurity, and a similar phase diagram has been also found in other extended quadrupole models. We have analyzed in detail the JJJ-dependence of the Kondo temperature TKT_KTK​ near the phase boundary $J_c (Δ) $ and found a nice scaling behavior with an stretched exponential form TK∼δJαexp⁡(−const./δJ)T_K \sim δJ^α \exp (-\mathrm{const.}/\sqrt{δJ})TK​∼δJαexp(−const./δJ​) where δJ≡J−Jc(Δ)δJ \equiv J - J_c (Δ)δJ≡J−Jc​(Δ). This differs from the standard scaling form and indicates that one needs to consider renormalization of multiple coupling constants.
The two-channel Kondo Hamiltonian has recently been proposed as a description of several experimental systems. Our numerical renormalization-group treatment of a pair of magnetic impurities shows that at low temperatures, interimpurity interactions destabilize the ``marginal-Fermi-liquid'' behavior predicted by a single-impurity model. We find four stable zero-temperature regimes, three of which can be described by Fermi-liquid theory. The fourth possesses a complex many-body ground state and non-Fermi-liquid properties which are expected to be governed by nonuniversal critical exponents.