Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Nature Communications

All-optical switching based on plasmon-induced Enhancement of Index of Refraction

Rakesh Dhama, Ali Panahpour, Tuomas Pihlava, Dipa Ghindani, Hümeyra Çağlayan

Published Jun 3, 2022• 46 citations
Publisher

Abstract

In quantum optical Enhancement of Index of Refraction (EIR), coherence and quantum interference render the atomic systems to exhibit orders of magnitude higher susceptibilities with vanishing or even negative absorption at their resonances. Here we show the plasmonic analogue of the quantum optical EIR effect in an optical system and further implement this in a linear all-optical switching mechanism. We realize plasmon-induced EIR using a particular plasmonic metasurface consisting of a square array of L-shaped meta-molecules. In contrast to the conventional methods, this approach provides a scheme to modulate the amplitude of incident signals by coherent control of absorption without implementing gain materials or nonlinear processes. Therefore, light is controlled by applying ultra-low intensity at the extreme levels of spatiotemporal localization. In the pursuit of potential applications of linear all-optical switching devices, this scheme may introduce an effective tool for improving the modulation strength of optical modulators and switches through the amplification of input signals at ultra-low power.

DOI
10.1038/s41467-022-30750-5

Related papers

Refraction enhancement in plasmonics by coherent control of plasmon resonances

Ali Panahpour, Abolfazl Mahmoodpoor, Andrei V. Lavrinenko

Optical materials exhibit significant losses over the resonance frequency of their constituent atoms and so they are practically implemented at frequencies far from resonances. Electromagnetically induced transparency (EIT) provides a method for effective suppression of optical loss in a narrow window over the resonance, where the medium exhibits significant dispersion but at the expense of zero susceptibility. The classical or plasmonic analogs of the EIT effect are introduced and widely used in the context of electromagnetic or optical metamaterials (MMs). In another interesting phenomenon in quantum optics known as enhancement of index of refraction (EIR), the optical loss of the medium can be zero or even negative at the region of maximal susceptibility and negligible dispersion. This condition is interesting for applications where a strong electromagnetic response of the medium with negligible loss is required, such as zero- or negative-index metamaterials (MMs). Here we introduce a plasmonic analog of the EIR which allows for coherent control over the polarizability and absorption of plasmonic nanoantennas. It can open up the way for loss-compensated propagation of optical waves in zero-index to high-refractive-index plasmonic MMs. The scheme also offers an approach to all-optical switching and coherent control of transmission, diffraction, and polarization conversion properties of plasmonic nanostructures, as well as propagation properties of surface plasmon polaritons on metasurfaces.

arXiv:1903.11888•Physical review. B./Physical review. B•Aug 20, 2019•11 citations

Plasmonic metamaterial for electromagnetically induced transparency analogue and ultra-high figure of merit sensor

Dong Wu, Yumin Liu, Li Yu +7 more

In this work, using finite-difference time-domain method, we propose and numerically demonstrate a novel way to achieve electromagnetically induced transparency (EIT) phenomenon in the reflection spectrum by stacking two different types of coupling effect among different elements of the designed metamaterial. Compared with the conventional EIT-like analogues coming from only one type of coupling effect between bright and dark meta-atoms on the same plane, to our knowledge the novel approach is the first to realize the optically active and precise control of the wavelength position of EIT-like phenomenon using optical metamaterials. An on-to-off dynamic control of the EIT-like phenomenon also can be achieved by changing the refractive index of the dielectric substrate via adjusting an optical pump pulse. Furthermore, in near infrared region, the metamaterial structure can be operated as an ultra-high resolution refractive index sensor with an ultra-high figure of merit (FOM) reaching 3200, which remarkably improve the FOM value of plasmonic refractive index sensors. The novel approach realizing EIT-like spectral shape with easy adjustment to the working wavelengths will open up new avenues for future research and practical application of active plasmonic switch, ultra-high resolution sensors and active slow-light devices.

Scientific Reports•Mar 23, 2017•63 citations

All-optical switching via enhanced Kerr nonlinearity in three-level atoms

Hai Wang, David J. Goorskey, Min Xiao

Summary form only given. The reduced absorption and enhanced nonlinearity in a three-level electromagnetically induced transparency (EIT) system are very important in achieving an effective all-optical switching action. The Kerr-nonlinear index of refraction of a three-level EIT medium can be greatly enhanced near resonance due to atomic coherence induced in such a system in comparison with a two-level atomic system, as we have shown by using an optical ring cavity. Both the magnitude and sign of the Kerr-nonlinear index change dramatically for different frequency detunings of the controlling (or coupling) or cavity (or probe) field. Bistability and dynamic instability occur when such a three-level /spl Lambda/-type EIT system is placed inside an optical ring cavity and the controlling and cavity input intensities to exceed certain threshold values. In this paper, we present a recent experimental demonstration of controlling the cavity output intensity by modulating the frequency detuning of the controlling beam.

Quantum Electronics and Laser Science Conference•Jun 25, 2003•0 citations

Optically induced diffraction gratings based on periodic modulation of linear and nonlinear effects for atom-light coupling quantum systems near plasmonic nanostructures

Azar Vafafard, Mostafa Sahrai, Vahid Siahpoush +2 more

We investigate the quantum linear and nonlinear effects in a novel five-level quantum system placed near a plasmonic nanostructure. Such a quantum scheme contains a double-V-type subsystem interacting with a weak probe field. The double-V-subsystem is then coupled to an excited state by a strong coupling field, which can be a position-dependent standing-wave field. We start by analyzing the first-order linear as well as the third and fifth order nonlinear terms of the probe susceptibility by systematically solving the equations for the matter-fields. When the quantum system is near the plasmonic nanostructure, the coherent control of linear and nonlinear susceptibilities becomes inevitable, leading to vanishing absorption effects and enhancing the nonlinearities. We also show that when the coupling light involves a standing-wave pattern, the periodic modulation of linear and nonlinear spectra results in an efficient scheme for the electromagnetically induced grating (EIG). In particular, the diffraction efficiency is influenced by changing the distance between the quantum system and plasmonic nanostructure. The proposed scheme may find potential applications in future nanoscale photonic devices.

Scientific Reports•Oct 7, 2020•21 citations

Ensembles of single-molecule picocavities as nonlinear optical metamaterials

Felipe Herrera, Marina Litinskaya

Strong coupling with single molecules in plasmonic picocavities has emerged as a resource for room-temperature quantum control with nanoscale light. Tip-based nanoprobes can measure the local dynamics of individual molecular picocavities, but the overhead associated with sampling an inhomogeneous picocavity distribution can be challenging for scalability. We propose a macroscopic approach in which an ensemble of molecular picocavities acts as a nonlinear plasmonic metamaterial. Using a quantum optics perspective, we study theoretical performance limits for optical cross-phase modulation in the system, taking into account realistic distributions of picocavity volumes and molecular transition frequencies. The medium nonlinearity is mediated by local strong coupling with the lowest vibronic emission sideband of individual organic chomophores. The local vacua change the refractive index of the medium at the frequency of a weak probe field $\omega_p$, set to drive the bare zero-phonon absorption band. Refractive index variations $\Delta n/n$ of a few percent, relative to a molecule-free scenario, are feasible with dilute ensembles. The probe phase evolution can be switched off in the presence of a signal field at a higher frequency $\omega_s$, for intensities as low as 10 kW/cm$^2$. The mechanism for optical switching involves a novel ($\omega_p+\omega_s$) two-photon absorption channel, assisted by local vacuum fields. Our work paves the way for future studies of plasmonic metamaterials that exploit strong light-molecule interactions, for applications in optical state preparation and control.

•Apr 2, 2021•0 citations

All-optical switching of continuous-variable entanglement in an absorption-suppressed plasmonic nanodimer

Elif Ozturk, Mehmet Gunay, Ramazan Sahin +1 more

A subwavelength quantum-photonic circuit element should simultaneously generate nonclassical light, suppress plasmonic loss, and remain dynamically tunable. We show that an orthogonal plasmonic nanorod dimer can satisfy all three requirements. A phase-locked control polarization induces plasmonic refractive-index enhancement, driving the probe response toward a near-zero-extinction regime while simultaneously tuning the local second-harmonic parametric interaction. The resulting nonlinear plasmonic source operates in an absorption-suppressed regime and enables all-optical control of quantum correlations. We demonstrate switchable logarithmic negativity and single-mode nonclassicality, establishing a route toward actively tunable quantum-plasmonic circuit elements operating well below the diffraction limit.

quant-pharXiv:2606.30315•Jun 30, 2026•0 citations
In quantum optical Enhancement of Index of Refraction (EIR), coherence and quantum interference render the atomic systems to exhibit orders of magnitude higher susceptibilities with vanishing or even negative absorption at their resonances. Here we show the plasmonic analogue of the quantum optical EIR effect in an optical system and further implement this in a linear all-optical switching mechanism. We realize plasmon-induced EIR using a particular plasmonic metasurface consisting of a square array of L-shaped meta-molecules. In contrast to the conventional methods, this approach provides a scheme to modulate the amplitude of incident signals by coherent control of absorption without implementing gain materials or nonlinear processes. Therefore, light is controlled by applying ultra-low intensity at the extreme levels of spatiotemporal localization. In the pursuit of potential applications of linear all-optical switching devices, this scheme may introduce an effective tool for improving the modulation strength of optical modulators and switches through the amplification of input signals at ultra-low power.
Optical materials exhibit significant losses over the resonance frequency of their constituent atoms and so they are practically implemented at frequencies far from resonances. Electromagnetically induced transparency (EIT) provides a method for effective suppression of optical loss in a narrow window over the resonance, where the medium exhibits significant dispersion but at the expense of zero susceptibility. The classical or plasmonic analogs of the EIT effect are introduced and widely used in the context of electromagnetic or optical metamaterials (MMs). In another interesting phenomenon in quantum optics known as enhancement of index of refraction (EIR), the optical loss of the medium can be zero or even negative at the region of maximal susceptibility and negligible dispersion. This condition is interesting for applications where a strong electromagnetic response of the medium with negligible loss is required, such as zero- or negative-index metamaterials (MMs). Here we introduce a plasmonic analog of the EIR which allows for coherent control over the polarizability and absorption of plasmonic nanoantennas. It can open up the way for loss-compensated propagation of optical waves in zero-index to high-refractive-index plasmonic MMs. The scheme also offers an approach to all-optical switching and coherent control of transmission, diffraction, and polarization conversion properties of plasmonic nanostructures, as well as propagation properties of surface plasmon polaritons on metasurfaces.
In this work, using finite-difference time-domain method, we propose and numerically demonstrate a novel way to achieve electromagnetically induced transparency (EIT) phenomenon in the reflection spectrum by stacking two different types of coupling effect among different elements of the designed metamaterial. Compared with the conventional EIT-like analogues coming from only one type of coupling effect between bright and dark meta-atoms on the same plane, to our knowledge the novel approach is the first to realize the optically active and precise control of the wavelength position of EIT-like phenomenon using optical metamaterials. An on-to-off dynamic control of the EIT-like phenomenon also can be achieved by changing the refractive index of the dielectric substrate via adjusting an optical pump pulse. Furthermore, in near infrared region, the metamaterial structure can be operated as an ultra-high resolution refractive index sensor with an ultra-high figure of merit (FOM) reaching 3200, which remarkably improve the FOM value of plasmonic refractive index sensors. The novel approach realizing EIT-like spectral shape with easy adjustment to the working wavelengths will open up new avenues for future research and practical application of active plasmonic switch, ultra-high resolution sensors and active slow-light devices.
Summary form only given. The reduced absorption and enhanced nonlinearity in a three-level electromagnetically induced transparency (EIT) system are very important in achieving an effective all-optical switching action. The Kerr-nonlinear index of refraction of a three-level EIT medium can be greatly enhanced near resonance due to atomic coherence induced in such a system in comparison with a two-level atomic system, as we have shown by using an optical ring cavity. Both the magnitude and sign of the Kerr-nonlinear index change dramatically for different frequency detunings of the controlling (or coupling) or cavity (or probe) field. Bistability and dynamic instability occur when such a three-level /spl Lambda/-type EIT system is placed inside an optical ring cavity and the controlling and cavity input intensities to exceed certain threshold values. In this paper, we present a recent experimental demonstration of controlling the cavity output intensity by modulating the frequency detuning of the controlling beam.
We investigate the quantum linear and nonlinear effects in a novel five-level quantum system placed near a plasmonic nanostructure. Such a quantum scheme contains a double-V-type subsystem interacting with a weak probe field. The double-V-subsystem is then coupled to an excited state by a strong coupling field, which can be a position-dependent standing-wave field. We start by analyzing the first-order linear as well as the third and fifth order nonlinear terms of the probe susceptibility by systematically solving the equations for the matter-fields. When the quantum system is near the plasmonic nanostructure, the coherent control of linear and nonlinear susceptibilities becomes inevitable, leading to vanishing absorption effects and enhancing the nonlinearities. We also show that when the coupling light involves a standing-wave pattern, the periodic modulation of linear and nonlinear spectra results in an efficient scheme for the electromagnetically induced grating (EIG). In particular, the diffraction efficiency is influenced by changing the distance between the quantum system and plasmonic nanostructure. The proposed scheme may find potential applications in future nanoscale photonic devices.
Strong coupling with single molecules in plasmonic picocavities has emerged as a resource for room-temperature quantum control with nanoscale light. Tip-based nanoprobes can measure the local dynamics of individual molecular picocavities, but the overhead associated with sampling an inhomogeneous picocavity distribution can be challenging for scalability. We propose a macroscopic approach in which an ensemble of molecular picocavities acts as a nonlinear plasmonic metamaterial. Using a quantum optics perspective, we study theoretical performance limits for optical cross-phase modulation in the system, taking into account realistic distributions of picocavity volumes and molecular transition frequencies. The medium nonlinearity is mediated by local strong coupling with the lowest vibronic emission sideband of individual organic chomophores. The local vacua change the refractive index of the medium at the frequency of a weak probe field ωp\omega_pωp​, set to drive the bare zero-phonon absorption band. Refractive index variations Δn/n\Delta n/nΔn/n of a few percent, relative to a molecule-free scenario, are feasible with dilute ensembles. The probe phase evolution can be switched off in the presence of a signal field at a higher frequency ωs\omega_sωs​, for intensities as low as 10 kW/cm2^22. The mechanism for optical switching involves a novel (ωp+ωs\omega_p+\omega_sωp​+ωs​) two-photon absorption channel, assisted by local vacuum fields. Our work paves the way for future studies of plasmonic metamaterials that exploit strong light-molecule interactions, for applications in optical state preparation and control.
A subwavelength quantum-photonic circuit element should simultaneously generate nonclassical light, suppress plasmonic loss, and remain dynamically tunable. We show that an orthogonal plasmonic nanorod dimer can satisfy all three requirements. A phase-locked control polarization induces plasmonic refractive-index enhancement, driving the probe response toward a near-zero-extinction regime while simultaneously tuning the local second-harmonic parametric interaction. The resulting nonlinear plasmonic source operates in an absorption-suppressed regime and enables all-optical control of quantum correlations. We demonstrate switchable logarithmic negativity and single-mode nonclassicality, establishing a route toward actively tunable quantum-plasmonic circuit elements operating well below the diffraction limit.