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Physical Review A

Ultrastable laser referenced on velocity-grating atom interferometry

Haosen Shang, Duo Pan, Xiaogang Zhang, Xiaobo Xue, Tiantian Shi, Jingbiao Chen

Published May 23, 2022• 8 citations
Publisher

Abstract

A laser with superb frequency stability plays an important role in fundamental physics research and advanced technologies. Frequency references are usually utilized to stabilize the laser, such as high-finesse cavities and atomic ensembles, of which thermal atomic beams are attractive because of their balanced performance between simplicity and stability. However, due to the transverse-velocity distribution in the thermal atomic beams, most atoms (generally $>99%$) are wasted when interacting with the laser. Here, we propose a laser referenced on a version of velocity-grating Ramsey-Bord\'e atom interferometry with greatly improved atom utilization and thus superior laser frequency stability. Compared with a conventional atomic interferometry applied to stabilize the laser, the proposed system in principle generates optical Ramsey fringes with the amplitude enhanced by 1000-fold or more. Such a configuration has promising applications in diverse areas, including precision measurements and quantum metrology.

DOI
10.1103/physreva.105.l051101

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A laser with superb frequency stability plays an important role in fundamental physics research and advanced technologies. Frequency references are usually utilized to stabilize the laser, such as high-finesse cavities and atomic ensembles, of which thermal atomic beams are attractive because of their balanced performance between simplicity and stability. However, due to the transverse-velocity distribution in the thermal atomic beams, most atoms (generally >99>99%>99) are wasted when interacting with the laser. Here, we propose a laser referenced on a version of velocity-grating Ramsey-Bord'e atom interferometry with greatly improved atom utilization and thus superior laser frequency stability. Compared with a conventional atomic interferometry applied to stabilize the laser, the proposed system in principle generates optical Ramsey fringes with the amplitude enhanced by 1000-fold or more. Such a configuration has promising applications in diverse areas, including precision measurements and quantum metrology.
A thermal atomic ensemble-based laser source with superior frequency stability is proposed that relies on the accumulated contributions from an abundance of nonzero-transverse-velocity atomic ensembles. Compared with the traditional case in which only atoms with near-zero transverse velocities are utilized, the amplitude of the optical Ramsey fringes for a thermal calcium beam can be dramatically enhanced by three orders of magnitude or more, thus, the signal-to-noise ratio can be improved 33-fold. Based on the recent results of atomic interferometry-based laser stabilization, a quantum projection noise-limited frequency instability less than 2E-17/tau^0.5 is feasible. Such an ultrastable laser has promising applications in diverse areas, including metrology and astronomy.
This dissertation details the developments of a calcium thermal beam atom interferometer designed to act as an ultra-stable frequency reference over a broad range of timescales. The obtained fractional frequency instabilities of the final apparatus reached ≤ 10−16 after 10's of seconds of averaging without the aid of vibration isolation or significant apparatus temperature stabilization. The vastly superior stability performance of this calcium system compared to other thermal atomic references was facilitated by the enormous atom numbers from the thermal beam, which can be efficiently addressed with Bord\'e-Ramsey spectroscopy on the well-studied (4s2)1S0-(4s4p)3P1 (m=0) clock transition in neutral 40Ca. This method yields interrogation laser frequency dependent interference fringes with a linewidth of 1.6 kHz. This measurement is further enhanced with an electron-shelving detection scheme used for state detection after the interferometry process, causing each excited state atom to emit many hundreds of photons in the detection region. The exceptional instability results from this atom interferometer highlight an underutilized realm of precision measurement science based on relatively simple thermal ensembles. An intuitive understanding of the Bordé-Ramsey process is presented and relevant experimental techniques explained such that this dissertation should prove useful to a broad readership.
We demonstrate Ramsey-Bordé (RB) atom interferometry for high performance laser stabilization with fractional frequency instability <2×10^{-16} for timescales between 10 and 1000s. The RB spectroscopy laser interrogates two counterpropagating ^{40}Ca beams on the ^{1}S_{0}-^{3}P_{1} transition at 657 nm, yielding 1.6 kHz linewidth interference fringes. Fluorescence detection of the excited state population is performed on the (4s4p) ^{3}P_{1}-(4p^{2}) ^{3}P_{0} transition at 431 nm. Minimal thermal shielding and no vibration isolation are used. These stability results surpass performance from other thermal atomic or molecular systems by 1 to 2 orders of magnitude, and further improvements look feasible.
Quantum technologies are nowadays emerging as enabling tools for practical applications, such as quantum sensing, quantum computing and quantum metrology. Lasers play a central role in many of these technological platforms, e.g. for atomic clocks, ion-based or neutral atom-based quantum computers or atom interferometers. Here we present a complete laser system to cool, trap and control strontium atoms in an optical lattice or in tweezer arrays. A sub-Hz linewidth master laser, locked to a high-finesse optical cavity provides the frequency reference for an ultra-low noise comb. The rack-mounted laser system consists of all cooling, repumping, and clock lasers stabilized to the optical frequency comb. Each of the involved laser frequencies can therefore be tuned and mapped in the frequency domain with a high degree of stability. The system is controlled via a software interface, allowing to operate the cold-atom-based physics package autonomously. The system is tailored for the operation of 88Sr or 87Sr optical lattice clocks, or for quantum computing applications, but other sub-Hz lasers could be obtained by phase locking additional clock laser frequencies to the ultra-stable comb, enabling convenient and accurate optical frequency ratio measurements. The laser system architecture and the relevant characterization measurements will be presented, proposing some user-cases such as quantum computing and atom interferometry on strontium atoms. This represents a technological leap for quantum optics, allowing to explore further applications of quantum sensors outside a traditional lab.
Laser Frequency Stabilization at ≤10−16\leq 10^{-16}≤10−16 from a Thermal Atomic bBeam
We demonstrate laser frequency stabilization at the 10-16fractional frequency level in one second through spectroscopy on a 650 °C calcium atomic beam. The calcium beam is interrogated with a cavity stabilized 657 nm laser arranged in a Ramsey-Borde configuration. A second laser at 431 nm reads off the final atomic state populations while allowing for high signal-to-noise. Limitations of this method are being explored and, and, based on current noise analysis, there is potential to achieve fractional frequency stabilities in the 10-17range or below.