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WORLD SCIENTIFIC eBooks

Optical Coherent Transient Effects

Published Dec 1, 1999• 0 citations
Publisher
DOI
10.1142/9789812816665_0010

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When an intense and short laser pulse or a fast-switching-on/off laser field interacts with a resonant absorbing medium, several optical coherent transient effects can be observed, including the self-induced transparency effect, photon echo effect, optical nutation effect, and the optical free induction decay effect. The study of these effects enables us to gain a deeper understanding of the coherent transient interaction of an intense pulsed or rapidly switched optical field with the resonant medium, and to measure the magnitude of the dipole-moment matrix elements, relaxation parameters, and spectral broadening mechanisms of the investigated materials. On the other hand, these optical coherent transient effects can also be applied for developing special techniques of optical pulse delay, pulse reshaping, and optical pulse manipulation.

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The general formalism of transient four-wave mixing is developed using the diagrammatic technique of Yee and Gustafson, and applied systematically to two-, three-, and four-level systems. The results predict all possible photon-echo phenomena including free-induction decay in the low-intensity limit. Connections to transient saturation spectroscopy and other coherent transient effects can also be made. The treatment can be readily extended to the more general problem of coherent transient optical effects with $n$ waves.

Physical Review A•Apr 1, 1982•67 citations
When an intense and short laser pulse or a fast-switching-on/off laser field interacts with a resonant absorbing medium, several optical coherent transient effects can be observed, including the self-induced transparency effect, photon echo effect, optical nutation effect, and the optical free induction decay effect. The study of these effects enables us to gain a deeper understanding of the coherent transient interaction of an intense pulsed or rapidly switched optical field with the resonant medium, and to measure the magnitude of the dipole-moment matrix elements, relaxation parameters, and spectral broadening mechanisms of the investigated materials. On the other hand, these optical coherent transient effects can also be applied for developing special techniques of optical pulse delay, pulse reshaping, and optical pulse manipulation.
The general formalism of transient four-wave mixing is developed using the diagrammatic technique of Yee and Gustafson, and applied systematically to two-, three-, and four-level systems. The results predict all possible photon-echo phenomena including free-induction decay in the low-intensity limit. Connections to transient saturation spectroscopy and other coherent transient effects can also be made. The treatment can be readily extended to the more general problem of coherent transient optical effects with nnn waves.