Exploring coherent photon-atom interaction at quantum level has become more and more important in modern quantum physics and quantum information science. In this PhD thesis research work, we established two cold 85Rb atoms ensemble in 2-dimensional dark-line magneto-optical trap with OD more than 100 and produced long coherence time (~1us) heralded single photons via spontaneous four-wave-mixing process with full temporal waveform control from one of the cold atomic ensemble. With this system, optical precursor of a single photon was observed for the first time, which verifies that information carried by a single photon cannot be transferred faster than light speed in vacuum even in the quantum world. This closed the longtime debate on the true speed of the information carried by a single photon. Single photon reemission timing in a two-level atomic system was the first time been controlled on-demand. With this technique, the quantum timing order of the single photon absorption and reemission was first directly observed in time domain. This technique can also be further used in the field of efficient single atom excitation that is desired for the quantum network. Finally, a series of work were conducted to improve the quantum optical memory efficiency in cold atomic ensemble. We obtained the highest single-photon storage efficiency of about 50%, which brings the quantum light-matter interface closer to practical quantum information applications. Multi-bin and multi-channel optical memory were also exploited in the following work.
Exploring coherent photon-atom interaction at quantum level has become more and more important in modern quantum physics and quantum information science. In this PhD thesis research work, we established two cold 85Rb atoms ensemble in 2-dimensional dark-line magneto-optical trap with OD more than 100 and produced long coherence time (~1us) heralded single photons via spontaneous four-wave-mixing process with full temporal waveform control from one of the cold atomic ensemble. With this system, optical precursor of a single photon was observed for the first time, which verifies that information carried by a single photon cannot be transferred faster than light speed in vacuum even in the quantum world. This closed the longtime debate on the true speed of the information carried by a single photon. Single photon reemission timing in a two-level atomic system was the first time been controlled on-demand. With this technique, the quantum timing order of the single photon absorption and reemission was first directly observed in time domain. This technique can also be further used in the field of efficient single atom excitation that is desired for the quantum network. Finally, a series of work were conducted to improve the quantum optical memory efficiency in cold atomic ensemble. We obtained the highest single-photon storage efficiency of about 50%, which brings the quantum light-matter interface closer to practical quantum information applications. Multi-bin and multi-channel optical memory were also exploited in the following work.
Quantum memories are an essential building block for quantum information science, and in particular for the implementation of quantum communications across long distances. A quantum memory is defined as a system capable of storing and retrieving quantum states on-demand, such as quantum bits (qubits). Atomic ensembles are good candidates for this purpose because they enables strong light-matter coupling in case of a large number of atoms. Moreover, the collective effect, enhanced in the regime of large optical depth, can lead to storage efficiency close to unity. Thus, in this thesis, a large magneto-optical trap for cesium atoms is used as a atomic medium in order to implement a quantum memory protocol based on electromagnetically induced transparency (EIT). First, the EIT phenomenon is studied through a criterion for the discrimination between the EIT and the Autler-Townes splitting models. We then report on the implementation of an EIT-based memory for photonic qubits encoded in orbital angular momentum (OAM) of light. A reversible memory for Laguerre-Gaussian modes is implemented, and we demonstrate that the optical memory preserves the handedness of the helical structure at the single-photon level. Then, a full quantum state tomography of the retrieved OAM encoded qubits is performed, giving fidelities above the classical bound. This showed that our optical memory operates in the quantum regime. Finally, we present the implementation of the so-called DLCZ protocol in our ensemble of cold atoms, enabling the generation of heralded single photons. A homodyne detection setup allows us to realize the quantum tomography of the created photonic state.
The advances in laser cooling and trapping techniques allow samples of ultra-cold atoms to be created and controlled for the study of quantum physics. In this thesis, we focus on using ensembles of cold atoms to investigate novel quantum effects and their applications in quantum optics. Realization of a scalable intercontinental quantum system, e.g. a global quantum internet, relies on quantum memories with long lifetimes on the order of seconds. We have reduced the differential light shifts of the atomic ground states to a sub-Hz level and achieved a lifetime of 16 seconds. Achieving fast and efficient quantum operations, on the other hand, requires strongly-interacting systems. We explore highly excited Rydberg atoms towards this goal and demonstrate Rydberg excitation blockade, many-body Rabi oscillations, trapping of Rydberg atoms, deterministic single photon source, and atom-photon entanglement. Finally, we integrate the two essential capabilities for quantum information processing, fast quantum state generation and long-term storage, by simultaneously exploiting Rydberg levels for interactions and ground atomic levels for the storage of quantum state. Our work advances the control of coherence properties and interactions in cold atomic ensembles to a new level and opens new opportunities for studies of complex quantum systems.
Single photons are the best carriers of quantum information for long-distance transmission. Nevertheless, maximal achievable distance is limited by the exponential decay of photons as a function of link length. The protocol of quantum repeater provides a promising solution by replacing direction transmission with segmented entanglement distribution and entanglement connection via swapping. The quantum repeater necessitates a key element of quantum memory for making efficient interconnections. An atomic ensemble is very suitable for this purpose due to the collective enhanced interaction. Single photons are stored as collective excitations in an atomic ensemble. Thus a comprehensive study of the physics relating to collective excitations is crucially important for improving the quantum memory performance and its reachable applications in quantum repeater and quantum network. In this article, we review our experimental work on cold atomic ensembles in recent years, focusing on the coherent manipulation of collective excitations. We first briefly introduce the general concept of collective excitations and the preparation process through spontaneous Raman scattering, and we review our experimental work on extending the coherence time, such as suppressing motional dephasing by increasing the spin-wave wavelength, by confining atoms with a three-dimensional optical lattice. Afterwards, we discuss about the retrieval process of collective excitations and review our experiments on using a ring-cavity enhanced setup to improve the retrieval efficiency. The coherent qubit operation in a quantum memory is very useful for enabling new functionalities for a quantum network, in a subsequent section, we thus review our work on developing Raman-based coherent operations for single excitations. Afterwards, we mention our experiments on creating a pair of atom-photon entanglement by interfering two modes of a collective excitation. Improving the entanglement preparation efficiency is crucially important, and Rydberg-based interaction provides a promising solution. Our experimental work in this direction is also reviewed. Additionally, as an application in coherent manipulation with collective excitations, we show several experiments on using excitations in remote atomic memories and demonstrating basic functionality of quantum repeater and quantum network. In short, significant progress has been made in the coherent manipulation of single collective excitations in cold atomic ensembles, and further improvement will be accelerated by the Rydberg-enabled interactions; practical applications in quantum repeater and quantum network is foreseeable in the near future.
The light wave propagating in a dispersive medium can be formularized as electromagnetic (EM) fields or quantized as a pair of Hermitian operators. The fascinating optical phenomena display classical and nonclassical properties, depending on whether they can be described by the classical EM field theory. A cold atomic ensemble with neligible inhomogenous Doppler broadening is ideal to explore the interaction between light and matter. A typical problem in classical pulse propagation is optical transients, which induced by rapid response of dispersive medium to the sudden change of the driving radiation fields. With cold atoms confined in the two-dimensional magneto-optical trap, whose optical depth is controllable in our system, optical precursor and free-induction decay both classified as optical transients are observed in a single experiment with different conditions. Moreover, the information velocity limit is verified in superluminal medium, with the observation and analysis of precursors. Characterized with narrow linewidth and long coherence time, paired photons generated from cold atomic ensemble in four-wave mixing process possess irreplaceable advantage in quantum optics area. Temporal modulation of narrow-band paired photons can be achieved by directly modulating the generated photons or by modulating the classical control fields. After successfully reshaping the temporal waveform of the paired photons, heralded single photon source is well prepared for studying the propagation of nonclassical single photon in dispersive medium. The speed limit imposed by Einstein Causality principle is firstly experimentally verified on single photon level.
Optical quantum memory plays an important role in scaling-up linear optical quantum computations and longdistance quantum communication. For effectively realizing such tasks, a long-lived and highly-efficient quantum memory is needed. The dynamic electromagnetically-induced-transparency (EIT) process can be used for completing an absorptive storage scheme in an atomic ensemble. In such a process, the quantum states of coming single photons can be coherently transformed into spin waves associated with coherences between atomic ground levels via switching off controlling light beam. For storing a single-mode optical signal, a pair of ground levels is involved. While for storing an optical polarization qubit, i.e., two orthogonal polarization modes, the coherence between two pairs of ground levels will be involved. Also, to obtain a high efficiency in the EIT optical storage, the optical-depth of the cold ensemble should be high. For prolonging the coherent time of the spin waves stored in atomic ensemble, decoherence between spin waves due to atomic motion and non-uniform Zeeman shift of ground levels should be effectively suppressed. Recently, a long-lived and highly-efficient optical quantum memory for single-mode storage in a high-optical-depth cold atom ensemble has been experimentally demonstrated via the gradient echo memory scheme (2016 Optical 3 100). While, for the optical polarization qubit storage, a long lifetime (in ms) and high-fidelity EIT storage experiment has been achieved by our group, but the storage efficiency in the experiment is very low (8%) due to lower optical depth of the cold ensemble (2013 Phys. Rev. Lett. 111 240503). The storage efficiency in long-lived storage of two orthogonal polarization modes still needs further improving. Here in this paper we demonstrate an experiment of long-lived and highly-efficient storage of two optical orthogonal polarization modes in a high optical-depth cold atomic ensemble via dynamic EIT process. For achieving a long lifetime in the storage experiment, we follow the two steps, which are used in our previous work (2013 Phys. Rev. Lett. 111 240503). 1) We make the signal and writing-reading light beams collinearly pass through the cold-atom cloud along the z direction to suppress the decoherence between the spin waves due to atomic motion. 2) We apply a moderate magnetic field (13.5 G) to the cold-atom ensemble to lift Zeeman degeneracy. So, the magnetic-field-sensitive transitions are removed from EIT system and the two optical orthogonal polarization modes are stored as two magnetic-field-insensitive spin waves. In contrast to our previous experiment, we finish the storage in the high optical-depth cold atomic ensemble. To obtain such a high optical-depth cold atomic ensemble, we expand the diameters of the trapping laser beams and use a pair of rectangular magnetic coils in a magnetic optical trap (MOT) to prepare a cigar-shaped cold atomic ensemble. The MOT magnetic field is further compressed, and then the optical-depth of the cold atomic ensemble increases up to ~11 in the present experiment, which allows us to achieve a storage efficiency of 30%, which exceeds the previous value (8%). At an MOT repetition rate of 10 Hz, the measured zero-delay storage efficiencies for the two orthogonal polarization modes are symmetric, which go up to ~30%. The 1/e-folding lifetimes of the two orthogonal polarization modes rise up to 3 ms. We also measure the dependence of the zero-delay retrieval efficiency on the MOT repetition rate F and find that the storage efficiency is still more than 20% when the repetition rate F is 50 Hz. The present results will allow one to achieve a long lifetime and highly-efficient quantum memory for photonic polarization qubit and then find applications in scaling-up linear-optical quantum computations and long-distance quantum communication.
Quantum networks are composed of quantum nodes which coherently interact by way of quantum channels. They offer powerful capabilities for quantum computation, communication, and metrology. A generic requirement for these realizations is the capability to generate and store quantum states among multiple quantum nodes, and to disseminate these resources throughout the network via the quantum channels. In this thesis, I describe a series of experiments whereby single excitations in atomic ensembles are strongly coupled to optical modes and provide efficient means for the coherent control of entangled states between matter and light. By following the seminal proposal by Duan et al., we have generated measurement-induced entanglement of an excitation between two cold atomic ensembles. Using this system, we investigated the relationship for the global bipartite entanglement and local correlations in its subsystems. In addition, we achieved functional quantum nodes for entanglement distribution. Two pairs of remote ensembles at two quantum nodes were prepared into entangled states in a heralded and asynchronous fashion by the conditional controls of the entanglement. The quantum states of the ensembles were then distributed into polarization entangled states of photons. We also prepared an analogous quantum state and transferred the nonlocal coherence between two pairs of heralded entangled atomic ensembles, providing a step towards entanglement connection. Beyond such probabilistic approaches, we demonstrated an experiment where entanglement between two quantum memories is created by the reversible and deterministic mapping of an entangled state of light via dynamic electromagnetically induced transparency. This experiment opens novel prospects of integrating hybrid quantum systems by way of reversible quantum interfaces between light and matter. Then, we extended our work to multipartite quantum systems. We theoretically investigated the characterization of multipartite mode-entangled states by way of quantum uncertainty relations, and introduced theoretical tools to verify the entanglement orders in multipartite systems. In particular, we achieved entanglement for one delocalized photon among multiple optical modes (N > 2). Finally, we have achieved measurement-induced entanglement of spin waves among four quantum memories. The individual atomic components for the entangled W state of the four ensembles were then coherently converted into four propagating entangled beams of light via superradiant emissions. We observed the statistical and dynamic transitions for the multipartite entangled spin waves. Experiments described in this thesis thereby represent significant advances of experimental and theoretical capabilities to generate, store, transfer, and characterize entanglement of matter and light over quantum networks.