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Physical Review Letters

Coupled Parametric Downconversion and Upconversion with Simultaneous Phase Matching

R. A. Andrews, Herbert Rabin, C. L. Tang

Published Sep 28, 1970• 2 citations
Publisher
DOI
10.1103/physrevlett.25.902.5

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Spontaneous parametric upconversion (SPUC) and spontaneous parametric downconversion (SPDC) have been observed in the β-barium borate (BBO) crystal, and their mechanisms are experimentally and theoretically investigated. SPUC, tuned from 530 to 600 nm with a FWHM of about 25 nm, can be attributed to the sum frequency between the quantum noise and the fundamental laser pulse in the type II phase matching condition (e+o→e). SPDC, tuned from 480 to 520 nm with a FWHM of about 15 nm, can be attributed to the difference frequency between the quantum noise and the fundamental laser pulse in the type I phase matching condition (e→o+o).
We study parametric interactions in a new type of nonlinear photonic structure, which is realized in the volume between a pair of nonlinear crystals. In this kind of structure, which we call binary, multiple nonlinear optical processes can be implemented simultaneously, owing to multiple phase-matching conditions, fulfilled separately in the constituent crystals. The coupling between the nonlinear processes by means of modes sharing similar frequency is attained by the spatially broadband nature of the parametric fields. We investigate the spatial properties of the fields generated in the binary structure constructed from periodically poled crystals for the two examples: (1) single parametric downconversion and (2) coupled parametric downconversion and upconversion processes. The efficacy of the fields’ generation in these examples is analyzed through comparison with the cases of a traditional single periodically poled crystal and an aperiodic photonic structure, respectively. For this, we have devised a method that allowed us to solve the field equations numerically without resorting to statistically modeling the input vacuum states. It has been shown that the relative shift between the periodic crystal lattices has a crucial effect on the generated spatial field spectrum and overall efficiency. In addition, the influence of the intercrystal distance on these characteristics has been studied. Therefore, our study suggests that one can construct optical elements with sophisticated nonlinear properties from simpler elements without significant sacrifice of efficacy.
Quasi-phase-matched parametric downconversion via cascaded optical nonlinearities in an aperiodically poled MgO:LiNbO3 superlattice was studied in theory and experiment. Coupling equations reveal that multiple-wavelength parametric downconversion in a wide infrared spectrum range can occur in a single crystal. Enhancement of the conversion efficiency and output stability through coupling of two nonlinear processes is demonstrated. The result also reveals that cascaded parametric downconversion process can be used to efficiently downconvert the fundamental wavelength to longer wavelength of infrared region.