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Physics World

Photons singled out

Published Aug 1, 2000• 0 citations
Publisher

Abstract

The ability to generate single photons on demand is one of the most crucial tasks in quantum optics. Such a photon source could be used in quantum cryptography where each bit of information is encoded on a single photon, or to make quantum logic gates. Now two teams of researchers from Germany and France have shown that certain defects within synthetic diamond can emit single photons at room temperature. Moreover, these solid-state devices have a high quantum efficiency and could potentially be miniaturized – making them ideal candidates as single-photon sources for practical applications (C Kurtsiefer et al. 2000 Phys. Rev. Lett.85 290, R Broui et al.. xxx.lanl.gov/abs/quant-ph/0007032).

DOI
10.1088/2058-7058/13/8/1

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•Aug 3, 2009•3 citations
The ability to generate single photons on demand is one of the most crucial tasks in quantum optics. Such a photon source could be used in quantum cryptography where each bit of information is encoded on a single photon, or to make quantum logic gates. Now two teams of researchers from Germany and France have shown that certain defects within synthetic diamond can emit single photons at room temperature. Moreover, these solid-state devices have a high quantum efficiency and could potentially be miniaturized – making them ideal candidates as single-photon sources for practical applications (C Kurtsiefer et al. 2000 Phys. Rev. Lett.85 290, R Broui et al.. xxx.lanl.gov/abs/quant-ph/0007032).
The development of reliable devices to generate single photons is crucial for applications in quantum cryptography, as well as for fundamental quantum optics experiments. Due to their extremely high photostability at room temperature, optically active defects in solids, the so called color centers, are among the most promising candidates. Single NV (nitrogen-vacancy) centers in diamond have been demonstrated to be able to generate single photons and have already shown advantages compared to attenuated laser pulses in a quantum cryptography experiment. The nitrogen-vacancy center (NV center) in diamond consists of a substitutional nitrogen atom and an adjacent vacancy. This complex exhibits an optical transition with a fluorescence lifetime of 11.6 ns. The room temperature spectrum of the NV center consists of the zero-phonon line at 637 nm and broad phononic sidebands with a FWHM of more than 100 nm. Due to the existence of a shelving level the efficiency of the NV center as a single photon source is limited. Additionally, the high diffraction index of bulk diamond restricts the efficiency to collect the fluorescence light.
Operation at the single-photon level is beneficial for energy efficiency in optical and optoelectronic devices and opens new prospects for novel applications, ranging from quantum cryptography to quantum computations. In this regard, efficient single-photon sources operating upon electrical injection at room temperature are crucially important. Color centers in diamond are currently considered to be the best candidates capable of room temperature operation. These defects in the lattice structure have been studied intensively during the last two decades, and optically driven single-photon sources have been demonstrated. However, the possibility of operation upon electrical injection was not clear until recently mainly because diamond is a unique material at the interface between solid-state and semiconductor physics. The demonstrated photon emission rate under electrical pumping did not exceed a few tens of kcounts per second [1], which is several orders of magnitude lower than the emission rate of optically pumped centers [2] and is well below the level required for practical applications. Since the mechanism of electroluminescence of the color center in diamond was not known, it was not clear to what extent the single-photon emission rate upon electrical injection could be increased.
Single photon sources are key devices for optical quantum information processing, miniaturized optical elements, as well as light standards. Several systems have been exploited so far such as semiconductor quantum dots, defect centers in diamond, alkali atoms, and parametric down-conversion sources. In this contribution we will review some of these sources and highlight their unique properties with respect to applications in quantum information processing. A focus lies on two different room temperature sources based on cavity-enhanced parametric downconversion and on nitrogen-vacancy centers in diamond.
The exploitation of emerging quantum technologies requires efficient fabrication of key building blocks. Sources of single photons are extremely important across many applications as they can serve as vectors for quantum information—thereby allowing long-range (perhaps even global-scale) quantum states to be made and manipulated for tasks such as quantum communication or distributed quantum computation. At the single-emitter level, quantum sources also afford new possibilities in terms of nanoscopy and bio-marking. Color centers in diamond are prominent candidates to generate and manipulate quantum states of light, as they are a photostable solid-state source of single photons at room temperature. In this review, we discuss the state of the art of diamond-based single-photon emitters and highlight their fabrication methodologies. We present the experimental techniques used to characterize the quantum emitters and discuss their photophysical properties. We outline a number of applications including quantum key distribution, bio-marking and sub-diffraction imaging, where diamond-based single emitters are playing a crucial role. We conclude with a discussion of the main challenges and perspectives for employing diamond emitters in quantum information processing.
The development of a robust light source that emits one photon at a time is an outstanding challenge in quantum science and technology. Here, at the transition from many to single photon optical communication systems, fully quantum mechanical effects may be utilized to achieve new capabilities, most notably perfectly secure communication via quantum cryptography. Practical implementations place stringent requirements on the device properties, including stable photon generation, room temperature operation, and efficient extraction of many photons. Single photon light emitting devices based on fluorescent dye molecules, quantum dots, and carbon nanotube material systems have all been explored, but none have simultaneously demonstrated all criteria. Here, we describe the design, fabrication, and characterization of a bright source of single photons consisting of an individual Nitrogen-vacancy color center (NV center) in a diamond nanowire operating in ambient conditions. The nanowire plays a positive role in increasing the number of single photons collected from the NV center by an order of magnitude over devices based on bulk diamond crystals, and allows operation at an order of magnitude lower power levels. This result enables a new class of nanostructured diamond devices for room temperature photonic and quantum information processing applications, and will also impact fields as diverse as biological and chemical sensing, opto-mechanics, and scanning-probe microscopy.