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Journal of Modern Optics

Two independent photon pairs versus four-photon entangled states in parametric down conversion

Hugues de Riedmatten, Valerio Scarani, I. Marcikic, Antonio Acín, Wolfgang Tittel, Hugo Zbinden, Nicolas Gisin

Published Apr 30, 2004• 13 citations
Publisher

Abstract

We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t ph c is much shorter than the duration of the pump pulse Δt, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter χ, which is a function of t ph c Δt. We present a direct measurement of χ through a simple experimental set-up. The full theoretical analysis is also provided.

DOI
10.1080/09500340310001654991

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We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t ph c is much shorter than the duration of the pump pulse Δt, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter χ, which is a function of t ph c Δt. We present a direct measurement of χ through a simple experimental set-up. The full theoretical analysis is also provided.
We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t ph c is much shorter than the duration of the pump pulse Δt, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter χ, which is a function of t ph c Δt. We present a direct measurement of χ through a simple experimental set-up. The full theoretical analysis is also provided.
We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t_c is much shorter than the duration of the pump pulse Delta t, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter chi, which is a function of tphc/∆t. We present a direct measurement of chi through a simple experimental setup. The full theoretical analysis is also provided
Spectral and temporal coincidence and single-particle photon wave packets are described and their widths and durations are found. The degree of entanglement is characterized by the experimentally measurable parameter R defined as the ratio of the coincidence and single-particle spectral widths. In the frequency representation, this parameter is found as a function of the pump-pulse duration. This function is shown to have a minimum and even in the minimum, at rather natural conditions, the parameter R is found to be very high (R=73>>1). The Schmidt number K is found for both short and long pump pulses and interpolated for arbitrary pulse durations. All functional dependences of R and K are found to be identical and numerical difference between them is shown to be not exceeding 20%. Two-time temporal wave function of a biphoton state is investigated in details, and a rather significant difference between the cases of short and long pump pulses is found to occur. In the case of long pulses, the temporal parameter R is defined as the ratio of durations of the single-particle and coincidence signals, and the defined in such a way parameter R is shown to be very close to the Schmidt number K.
The process of parametric down-conversion pumped by a short coherent pulse is analysed. The coherence properties of the down-converted field are investigated. It is found that the spectrum of the down-conversion is mostly determined by the nonlinear medium and is independent of the width of the short pumping pulse and that it is impossible to realize a transform-limited two-photon state. Fourth-order interference between a weak coherent pulse and the down-converted pulse is considered. It is found that high visibility near 100% is achievable by means of narrow optical filtering. It is shown that by gating the detection on one of the down-converted photons, a transform-limited single-photon pulse is achievable in the other conjugate field, but its pulse width is shorter than that of the down-converted pulse and its peak position is uncertain within the pulse width of the down-converted light. However, with narrow optical filtering on the gating detection process, a transform-limited single-photon state can be obtained in the gated field with its peak position synchronized to the pump pulse. The possibility for the realization of a multi-photon interference experiment is explored for the quantum state measurement of the single-photon state.
We investigate spectral and temporal features and entanglement of biphoton wave packets formed in spontaneous parametric down-conversion with a pulsed laser pump. The degree of entanglement is characterized by the experimentally measurable parameter RRR defined as the ratio of the coincidence and single-particle spectral widths. In the frequency representation, this parameter is found as a function of the pump-pulse duration $\ensuremath{\tau}$. The function $R(\ensuremath{\tau})$ is shown to have a minimum and even in the minimum, at rather natural conditions, the degree of entanglement is found to be very high (Rmin=73)({R}_{\mathrm{min}}=73)(Rmin​=73). The Schmidt number KKK is found analytically for both short and long pump pulses and interpolated for arbitrary pulse durations. All functional dependences of RRR and KKK are found to be identical and numerical coefficients are found to be rather close. Two-time temporal wave function of a biphoton state is investigated in detail, and a rather significant difference between the cases of short and long pump pulses is found to occur. In the case of long pulses, the temporal parameter Rt{R}_{t}Rt​ (defined as the ratio of durations of the single-particle and coincidence signals) is shown to be very close to the Schmidt number KKK.
Coherence properties of the down-converted beams generated in spontaneous parametric down-conversion are investigated in detail using an iCCD camera. Experimental results are compared with those from a theoretical model developed for pulsed pumping with a Gaussian transverse profile. The results allow us to tailor the shape of correlation area of the signal and idler photons using pump-field and crystal parameters. As an example, splitting of a correlation area caused by a two-peak pump-field spectrum is experimentally studied.