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Science

Controlled Single-Photon Emission

Published Jul 14, 2005• 0 citations
Publisher
DOI
10.1126/science.309.5733.351f

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Tailored nanoscale quantum light sources, matching the specific needs of use cases, are crucial building blocks for photonic quantum technologies. Several different approaches to realize solid-state quantum emitters with high performance have been pursued and different concepts for energy tuning have been established. However, the properties of the emitted photons are always defined by the individual quantum emitter and can therefore not be controlled with full flexibility. Here we introduce an all-optical nonlinear method to tailor and control the single photon emission. We demonstrate a laser-controlled down-conversion process from an excited state of a semiconductor quantum three-level system. Based on this concept, we realize energy tuning and polarization control of the single photon emission with a control-laser field. Our results mark an important step towards tailored single photon emission from a photonic quantum system based on quantum optical principles.
In the single-photon emission from a two-level system, multiphotons are generally regarded as accidental, undesired, and unrelated to the mechanism. In coherently driven systems, however, they form the cornerstone of single-photon emission, which arises from quantum interferences between virtual multiphoton fluctuations of the emitter and the Poissonian superposition of all number states induced by the driving. Here, we demonstrate how one can control the multiphoton dynamics by disrupting these quantum interferences through an external homodyne control of the emitter's mean field. Experimentally, we observed a transition from single-photon to multiphoton emission, up to three-photon correlations. We show that, counterintuitively, quantum fluctuations always play a major qualitative role, even and, in fact, especially when their quantitative contribution is vanishing. Our findings provide distinct insights into the paradoxical character of quantum mechanics and open pathways for mean-field engineering as a tool for precision multiphoton control.