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Springer series in chemical physics

Mapping of the Optical Frequency Comb to the Atom Velocity Comb

Ticijana Ban, Damir Aumiler, Hrvoje Skenderović, Goran Pichler

Published Jan 1, 2007• 1 citation
Publisher
DOI
10.1007/978-3-540-68781-8_41

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We present the experimental and theoretical study of the resonant excitation of rubidium and cesium atoms with fs pulse train in the conditions when the pulse repetition period is shorter than the atomic relaxation time. Velocity selective optical pumping of the ground state hyperfine levels and velocity comb‐like excited state hyperfine level populations is demonstrated. Both effects are a direct consequence of the fs pulse train excitation considered in the frequency domain. A simple experimental apparatus was employed to develop a modified direct frequency comb spectroscopy which uses a fixed frequency comb for the 85,87Rb 5s 2S1/2 → 5s 2P1/2,3/2 and 133Cs 6s 2S1/2 → 6p 2P1/2,3/2 excitation, and a weak cw scanning probe laser at 780 and 852 nm for Rb and Cs ground levels population monitoring.

AIP conference proceedings•Jan 1, 2006•6 citations
A mode-locked femtosecond laser is used to physically map the laser frequency comb into the velocity comb of the excited Rb atoms at room temperature. Upon resonant excitation by discrete optical frequencies the velocity distribution of the excited Rb atoms shows comblike structure. Simultaneously, velocity-selective population transfer occurs between ground-state hyperfine levels. Both facts are observed by modified direct frequency comb spectroscopy and verified by a detailed density matrix treatment of the multilevel system in resonant field.
We present the experimental and theoretical study of the resonant excitation of rubidium and cesium atoms with fs pulse train in the conditions when the pulse repetition period is shorter than the atomic relaxation time. Velocity selective optical pumping of the ground state hyperfine levels and velocity comb‐like excited state hyperfine level populations is demonstrated. Both effects are a direct consequence of the fs pulse train excitation considered in the frequency domain. A simple experimental apparatus was employed to develop a modified direct frequency comb spectroscopy which uses a fixed frequency comb for the 85,87Rb 5s 2S1/2 → 5s 2P1/2,3/2 and 133Cs 6s 2S1/2 → 6p 2P1/2,3/2 excitation, and a weak cw scanning probe laser at 780 and 852 nm for Rb and Cs ground levels population monitoring.