A general approach to quantum dynamics using a variational master equation: Application to phonon-damped Rabi rotations in quantum dots
Dara P. S. McCutcheon, Nikesh S. Dattani, Erik M. Gauger +2 more
We develop a versatile master equation approach to describe the nonequilibrium dynamics of a two-level system in contact with a bosonic environment, which allows for the exploration of a wide range of parameter regimes within a single formalism. As an experimentally relevant example, we apply this technique to the study of excitonic Rabi rotations in a driven quantum dot, and compare its predictions to the numerical Feynman integral approach. We find excellent agreement between the two methods across a generally difficult range of parameters. In particular, the variational master equation technique captures effects usually considered to be nonperturbative, such as multiphonon processes and bath-induced driving renormalization, and can give reliable results even in regimes in which previous master equation approaches fail.
arXiv:1105.6015•Physical Review B•Aug 25, 2011•155 citations