Laser-Induced Line-Narrowing Effects in Coupled Doppler-Broadened Transitions. II. Standing-Wave Features
B. J. Feldman, Michael S. Feld
Previous theoretical results on the influence of a laser on the line shape of a coupled transition-laser-induced line narrowing-have been restricted to the case where the laser is detuned from the center of its atomic gain profile or is in the form of a traveling wave. This paper extends those results to include the case where the laser is an intense standing-wave field tunable to the center of its atomic gain profile (conditions for Lamb dip). The effect may be observed either in transmission, by probing the coupled transition with a weak traveling-wave field coaxial with the laser field, or else in spontaneous emission from the coupled transition viewed along the axis of the laser field. It is now well known that for a laser detuned from the center of its atomic gain profile, two narrow Lorentzian resonances of different widths appear superimposed upon the broad background signal at frequencies symmetrically located about the corresponding line center. When the laser is tuned to the center of its gain profile, however, additional fine structure develops. This structure, which is particularly significant when the laser field is intense, may have important applications in highresolution spectroscopy and laser-frequency stabilization. In this paper the laser frequency may be smaller or larger than the frequency of the coupled transition. In the latter case an intense laser introduces additional splitting effects, even when the laser is detuned. Splitting effects due to weakly saturating laser fields are also discussed. The problem is formulated by expanding elements of the ensemble-averaged density matrix in an infinite series of spatial Fourier components. A perturbation technique is employed, valid for a weak probe field and a standing-wave field of arbitrary intensity. One obtains an expression for emission induced by the probe field due to atoms moving with one velocity, written in terms of continued fractions in the general case and with Bessel functions in an important special case. This expression is integrated over the atomic velocity distribution by means of a computer to obtain the total emission due to atoms moving with all velocities. In some cases the integrated expressions may be written in closed algebraic form. A detailed discussions of line shapes and of the physical processes involved is included.
Physical Review A•Feb 1, 1972•154 citations