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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

"Experimental realization of Wheeler's delayed-choice Gedanken Experiment"

V. Jacques, E Wu, Frédéric Grosshans, François Treussart, Alain Aspect, Philippe Grangier, Jean-François Roch

Published Jun 1, 2007• 54 citations
Publisher

Abstract

We report an almost ideal realization of wheeler's "delayed-choice" experiment where the light pulses are true single photons, allowing unambiguous which-way measurements. The clock-triggered single-photon source at the heart of the experiment, previously developed for quantum key distribution, is based on the pulsed, optically excited photoluminescence of a single N-V colour centre in a diamond nanocrystal. This system, which consists in a substitutional nitrogen atom (N) associated to a vacancy (V) in an adjacent lattice site of the diamond crystalline matrix, has an unsurpassed efficiency and photostability at room temperature.

DOI
10.1109/cleoe-iqec.2007.4386903

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We report an almost ideal realization of wheeler's "delayed-choice" experiment where the light pulses are true single photons, allowing unambiguous which-way measurements. The clock-triggered single-photon source at the heart of the experiment, previously developed for quantum key distribution, is based on the pulsed, optically excited photoluminescence of a single N-V colour centre in a diamond nanocrystal. This system, which consists in a substitutional nitrogen atom (N) associated to a vacancy (V) in an adjacent lattice site of the diamond crystalline matrix, has an unsurpassed efficiency and photostability at room temperature.
We present a full implementation of a quantum key distribution (QKD) system with a single photon source, operating at night in open air. The single photon source at the heart of the functional and reliable setup relies on the pulsed excitation of a single nitrogen-vacancy color center in diamond nanocrystal. We tested the effect of attenuation on the polarized encoded photons for inferring longer distance performance of our system. For strong attenuation, the use of pure single photon states gives measurable advantage over systems relying on weak attenuated laser pulses. The results are in good agreement with theoretical models developed to assess QKD security.
We report the realization of a solid-state triggered single-photon source with narrow emission in the near infrared at room temperature. It is based on the photoluminescence of a single nickel–nitrogen NE8 colour centre in a chemical vapour deposited diamond nanocrystal. Stable single-photon emission has been observed in the photoluminescence under both continuous-wave and pulsed excitations. The realization of this source represents a step forward in the application of diamond-based single-photon sources to quantum key distribution (QKD) under practical operating conditions.
We describe the implementation of a quantum key distribution (QKD) system using a single-photon source, operating at night in open air. The single-photon source at the heart of the functional and reliable set-up relies on the pulsed excitation of a single nitrogen-vacancy colour centre in a diamond nanocrystal. We tested the effect of attenuation on the polarized encoded photons for inferring the longer distance performance of our system. For strong attenuation, the use of pure single-photon states gives measurable advantage over systems relying on weak attenuated laser pulses. The results are in good agreement with theoretical models developed to assess QKD security.
The development of reliable devices to generate single photons is crucial for applications in quantum cryptography, as well as for fundamental quantum optics experiments. Due to their extremely high photostability at room temperature, optically active defects in solids, the so called color centers, are among the most promising candidates. Single NV (nitrogen-vacancy) centers in diamond have been demonstrated to be able to generate single photons and have already shown advantages compared to attenuated laser pulses in a quantum cryptography experiment. The nitrogen-vacancy center (NV center) in diamond consists of a substitutional nitrogen atom and an adjacent vacancy. This complex exhibits an optical transition with a fluorescence lifetime of 11.6 ns. The room temperature spectrum of the NV center consists of the zero-phonon line at 637 nm and broad phononic sidebands with a FWHM of more than 100 nm. Due to the existence of a shelving level the efficiency of the NV center as a single photon source is limited. Additionally, the high diffraction index of bulk diamond restricts the efficiency to collect the fluorescence light.
Wave-particle duality constitutes one of the most intriguing features in quantum physics. A well-known gedanken experiment that provides evidence for this is Wheeler's delayed-choice experiment based on a Mach-Zehnder interferometer [J. A. Wheeler, in Mathematical Foundations of Quantum Theory, edited by A. R. Marlow (Academic, New York, 1978), pp. 9--48; in Quantum Theory and Measurement, edited by J. A. Wheeler and W. H. Zurek (Princeton University Press, Princeton, 1984), pp. 182--213]. Many different versions of delayed-choice experiments have been conducted with both classical and quantum detecting devices. Recently, it was proposed that the delayed-choice experiment could be devised from the perspective of a device-independent prepare-and-measure scenario [R. Chaves et al., Causal Modeling the Delayed-Choice Experiment, Phys. Rev. Lett. 120, 190401 (2018)]. In our work, we experimentally realize this modified version with a deterministic single-photon source and examine the wave-particle objective in a causal-modeled scheme without the assistance of entanglement, which is achieved by violating the dimension-witness inequalities. Our experiment also provides an intriguing perspective and exhibits the benefits of studying quantum theory from the casual model point of view.