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Proceedings of the National Academy of Sciences

A stability bound on the T-linear resistivity of conventional metals

Chaitanya Murthy, Akshat Pandey, Ilya Esterlis, Steven Allan Kivelson

Published Jan 12, 2023• 0 citations
Publisher

Abstract

Perturbative considerations account for the properties of conventional metals, including the range of temperatures where the transport scattering rate is 1/ τ tr = 2 π λ T , where λ is a dimensionless strength of the electron–phonon coupling. The fact that measured values satisfy λ ≲ 1 has been noted in the context of a possible “Planckian” bound on transport. However, since the electron–phonon scattering is quasielastic in this regime, no such Planckian considerations can be relevant. We present and analyze Monte Carlo results on the Holstein model which show that a different sort of bound is at play: a “stability” bound on λ consistent with metallic transport. We conjecture that a qualitatively similar bound on the strength of residual interactions, which is often stronger than Planckian, may apply to metals more generally.

DOI
10.1073/pnas.2216241120

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Perturbative considerations account for the properties of conventional metals, including the range of temperatures where the transport scattering rate is 1/ τ tr = 2 π λ T , where λ is a dimensionless strength of the electron–phonon coupling. The fact that measured values satisfy λ ≲ 1 has been noted in the context of a possible “Planckian” bound on transport. However, since the electron–phonon scattering is quasielastic in this regime, no such Planckian considerations can be relevant. We present and analyze Monte Carlo results on the Holstein model which show that a different sort of bound is at play: a “stability” bound on λ consistent with metallic transport. We conjecture that a qualitatively similar bound on the strength of residual interactions, which is often stronger than Planckian, may apply to metals more generally.
A stability bound on the TTT-linear resistivity of conventional metals
Perturbative considerations account for the properties of conventional metals, including the range of temperatures where the transport scattering rate is 1/τtr=2πλT1/τ_\text{tr} = 2πλT1/τtr​=2πλT, where λλλ is a dimensionless strength of the electron-phonon coupling. The fact that measured values satisfy λ≲1λ\lesssim 1λ≲1 has been noted in the context of a possible "Planckian" bound on transport. However, since the electron-phonon scattering is quasi-elastic in this regime, no such Planckian considerations can be relevant. We present and analyze Monte Carlo results on the Holstein model which show that a different sort of bound is at play: a "stability" bound on λλλ consistent with metallic transport. We conjecture that a qualitatively similar bound on the strength of residual interactions, which is often stronger than Planckian, may apply to metals more generally.
“Strange” metals that do not follow the predictions of Fermi liquid theory are prevalent in materials that feature superconductivity arising from electron interactions. In recent years, it has been hypothesized that spatial randomness in electron interactions must play a crucial role in strange metals for their hallmark linear-in-temperature ( T ) resistivity to survive down to low temperatures where phonon and umklapp processes are ineffective, as is observed in experiments. However, a clear picture of how this happens has not yet been provided in a realistic model free from artificial constructions, such as large- N limits and replica tricks. We study a realistic model of two-dimensional metals with spatially random antiferromagnetic interactions in a nonperturbative regime, using numerically exact high-performance, large-scale hybrid Monte Carlo simulation and exact averages over the quenched spatial randomness. Our simulations reproduce strange metals’ key experimental signature of linear-in- T resistivity with a universal “Planckian” transport scattering rate Γ tr ∼ k B T / ℏ that is independent of coupling constants. We further find that strange metallicity in these systems is not associated with a quantum critical point and, instead, arises from a phase of matter with gapless antiferromagnetic fluctuations that lacks long-range correlations and spans an extended region of parameter space: A feature that is also observed in several experiments. These gapless antiferromagnetic fluctuations take the form of spatially localized overdamped modes, whose presence could possibly be detected using recently developed nanoscale magnetometry methods. Our work paves the way for an eventual microscopic understanding of the role of spatial disorder in determining important properties of correlated-electron materials.
We present a lattice model of fermions with N flavors and random interactions that describes a Planckian metal at low temperatures T→0 in the solvable limit of large N. We begin with quasiparticles around a Fermi surface with effective mass m^{*} and then include random interactions that lead to fermion spectral functions with frequency scaling with k_{B}T/ℏ. The resistivity ρ obeys the Drude formula ρ=m^{*}/(ne^{2}τ_{tr}), where n is the density of fermions, and the transport scattering rate is 1/τ_{tr}=fk_{B}T/ℏ; we find f of order unity and essentially independent of the strength and form of the interactions. The random interactions are a generalization of the Sachdev-Ye-Kitaev models; it is assumed that processes nonresonant in the bare quasiparticle energies only renormalize m^{*}, while resonant processes are shown to produce the Planckian behavior.
Phonons have long been thought to be incapable of explaining key phenomena in strange metals, including linear-in-\textit{T} Planckian resistivity from high to very low temperatures. We argue that these conclusions were based on static, perturbative approaches that overlooked essential time-dependent and nonperturbative electron-lattice physics. In fact ``phonons'' are not the best target for discussion, just like ``photons'' are not the best way to think about Maxwell's equations. Quantum optics connects photons and electromagnetism, as developed 60 years ago by Glauber and others. We have been developing the parallel world of quantum acoustics. Far from being only of academic interest, the new tools are rapidly exposing the secrets of the strange metals, revealing strong vibronic (vibration-electronic) interactions playing a crucial role forming polarons and charge density waves, linear-in-TTT resistivity at the Planckian rate over thousands of degrees, resolution of the Drude peak infrared anomaly, and the absence of a T4T^4T4 low-temperature resistivity rise in 2D systems, and of a Mott-Ioffe-Regel resistivity saturation. We derive Planckian transport, polarons, CDWs, and pseudogaps from the Fröhlich model. The ``new physics'' has been hiding in this model all along, in the right parameter regime, if it is treated nonperturbatively. In the course of this work we have uncovered the generalization of Anderson localization to dynamic media: a universal Planckian diffusion emerges, a ``ghost'' of Anderson localization. Planckian diffusion is clearly defined and is more fundamental than the popular but elusive, model dependent concept of ``Planckian speed limit''.
Strange metals—ubiquitous in correlated quantum materials—transport electrical charge at low temperatures but not by the individual electronic quasiparticle excitations, which carry charge in ordinary metals. In this work, we consider two-dimensional metals of fermions coupled to quantum critical scalars, the latter representing order parameters or fractionalized particles. We show that at low temperatures ( T ), such metals generically exhibit strange metal behavior with a T -linear resistivity arising from spatially random fluctuations in the fermion-scalar Yukawa couplings about a nonzero spatial average. We also find a T ln(1/ T ) specific heat and a rationale for the Planckian bound on the transport scattering time. These results are in agreement with observations and are obtained in the large N expansion of an ensemble of critical metals with N fermion flavors.