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Possible chiral spin liquid state in the S = 1/2 kagome Heisenberg model

Rong-Yang Sun, Hui-Ke Jin, Hong-Hao Tu, Yi Zhou

Published Sep 28, 2022• 0 citations
Publisher

Abstract

Abstract The nature of the ground state for the S = 1/2 kagome Heisenberg antiferromagnet (KHAF) has been elusive. We revisit this challenging problem and provide numerical evidence that its ground state might be a chiral spin liquid. Combining the density matrix renormalization group method and analytical analyses, we demonstrate that the previously observed chiral spin liquid phase in the KHAF with longer-range couplings is stable in a broader region. We characterize the nature of the ground state by computing energy derivatives, revealing ground-state degeneracy arising from spontaneous breaking of time-reversal symmetry, and targeting the semion sector. We further investigate the phase diagram in the vicinity of the KHAF and observe a √3 × √3 magnetically ordered phase and two valence-bond crystal phases.

DOI
10.21203/rs.3.rs-2051231/v1

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Abstract The nature of the ground state for the S = 1/2 kagome Heisenberg antiferromagnet (KHAF) has been elusive. We revisit this challenging problem and provide numerical evidence that its ground state might be a chiral spin liquid. Combining the density matrix renormalization group method and analytical analyses, we demonstrate that the previously observed chiral spin liquid phase in the KHAF with longer-range couplings is stable in a broader region. We characterize the nature of the ground state by computing energy derivatives, revealing ground-state degeneracy arising from spontaneous breaking of time-reversal symmetry, and targeting the semion sector. We further investigate the phase diagram in the vicinity of the KHAF and observe a √3 × √3 magnetically ordered phase and two valence-bond crystal phases.
Abstract The nature of the ground state for the S = 1/2 Kagome Heisenberg antiferromagnet (KHAF) has been elusive. We revisit this challenging problem and provide numerical evidence that its ground state is a chiral spin liquid. Combining the density matrix renormalization group method with analytical analyses, we demonstrate that the previously observed chiral spin liquid phase in the KHAF with longer-range couplings is stable in a broader region of the phase diagram. We characterize the nature of the ground state by computing energy derivatives, revealing the ground-state degeneracy arising from the spontaneous breaking of the time-reversal symmetry, and targeting the semion sector. We further investigate the phase diagram in the vicinity of the KHAF and observe a 3×3\sqrt{3}\times \sqrt{3}3​×3​ 3 × 3 magnetically ordered phase and two valence-bond crystal phases.
By using the density matrix renormalization group, we study the spin-liquid phases of spin-1/21/21/2 XXZ kagome antiferromagnets. We find that the emergence of spin liquid phase does not depend on the anisotropy of the XXZ interaction. In particular, the two extreme limits---Ising (strong SzS^zSz interaction) and XY (zero SzS^zSz interaction)---host the same spin-liquid phases as the isotropic Heisenberg model. Both the time-reversal-invariant spin liquid and the chiral spin liquid with spontaneous time-reversal symmetry breaking are obtained. We show they evolve continuously into each other by tuning the second- and third-neighbor interactions. To understand the continuous phase transition between these two spin liquids, we construct a phenomenological theory, and propose the double-semion spin liquid as the candidate ground state of nearest-neighbor XXZ kagome antiferromagnets, including the most studied nearest-neighbor spin-1/21/21/2 kagome antiferromagnetic Heisenberg model.
We perform a density-matrix renormalization group (DMRG) study of the S=1/2 Heisenberg antiferromagnet on the kagome lattice to identify the conjectured spin liquid ground state. Exploiting SU(2) spin symmetry, which allows us to keep up to 16,000 DMRG states, we consider cylinders with circumferences up to 17 lattice spacings and find a spin liquid ground state with an estimated per site energy of -0.4386(5), a spin gap of 0.13(1), very short-range decay in spin, dimer and chiral correlation functions and finite topological entanglement gamma consistent with gamma=ld 2, ruling out gapless, chiral or non-topological spin liquids. At the same time, DMRG results provide strong evidence for a gapped topological Z2 spin liquid.
We perform a density-matrix renormalization group (DMRG) study of the S=1/2 Heisenberg antiferromagnet on the kagome lattice to identify the conjectured spin liquid ground state. Exploiting SU(2) spin symmetry, which allows us to keep up to 16,000 DMRG states, we consider cylinders with circumferences up to 17 lattice spacings and find a spin liquid ground state with an estimated per site energy of -0.4386(5), a spin gap of 0.13(1), very short-range decay in spin, dimer and chiral correlation functions, and finite topological entanglement γ consistent with γ=log(2)2, ruling out gapless, chiral, or nontopological spin liquids in favor of a topological spin liquid of quantum dimension 2, with strong evidence for a gapped topological Z(2) spin liquid.
We study the quantum phase diagram of the spin-1/21/21/2 Heisenberg model on the kagome lattice with first-, second-, and third-neighbor interactions J1,J2{J}_{1},{J}_{2}J1​,J2​, and J3{J}_{3}J3​ by means of density matrix renormalization group. For small J2{J}_{2}J2​ and J3{J}_{3}J3​, this model sustains a time-reversal invariant quantum spin-liquid phase. With increasing J2{J}_{2}J2​ and J3{J}_{3}J3​, we find in addition a q=(0,0)q=(0,0)q=(0,0) N\'eel phase, a chiral spin-liquid phase, an apparent valence-bond crystal phase, and a complex noncoplanar magnetically ordered state with spins forming the vertices of a cuboctahedron known as a cuboc1 phase. Both the chiral spin liquid and cuboc1 phase break time-reversal symmetry in the sense of spontaneous scalar spin chirality. We show that the chiralities in the chiral spin liquid and cuboc1 are distinct, and that these two states are separated by a strong first-order phase transition. The transitions from the chiral spin liquid to both the q=(0,0)q=(0,0)q=(0,0) phase and to time-reversal symmetric spin liquid, however, are consistent with continuous quantum phase transitions.
By using the density matrix renormalization group approach, we study spin-liquid phases of spin-1/2 XXZ kagome antiferromagnets. We find that the emergence of the spin-liquid phase is independent of the anisotropy of the XXZ interaction. In particular, the two extreme limits-the Ising (a strong S^{z} interaction) and the XY (zero S^{z} interaction)-host the same spin-liquid phases as the isotropic Heisenberg model. Both a time-reversal-invariant spin liquid and a chiral spin liquid with spontaneous time-reversal symmetry breaking are obtained. We show that they evolve continuously into each other by tuning the second- and the third-neighbor interactions. And last, we discuss possible implications of our results for the nature of spin liquid in nearest-neighbor XXZ kagome antiferromagnets, including the nearest-neighbor spin-1/2 kagome antiferromagnetic Heisenberg model.