Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Optical and Quantum Sensing and Precision Metrology II

Heralded spectroscopy of single nanocrystals

Gur Lubin, Ron Tenne, Arin Can Ülkü, Ivan Michel Antolović, Samuel Burri, Sean Karg, Venkata Jayasurya Yallapragada, Claudio E. Bruschini, Edoardo Charbon A, Dan Oron

Published Mar 9, 2022• 0 citations
Publisher

Abstract

Since the introduction of the intensity interferometer by Hanbury Brown and Twiss in the '50s and its subsequent adaptations to quantum optic experiments, photon correlations have played a significant role in optical research. An emerging detector technology, SPAD arrays, presents new opportunities to scale these experiments and exploit photon correlations in new regimes. I will describe a new temporal-spectral photon correlation technique based on these detectors, single-particle heralded spectroscopy. I will present new insights into the photophysics of multiply-excited semiconductor quantum dots uncovered by this method, hitherto inaccessible to existing approaches.

DOI
10.1117/12.2616990

Related papers

Photon Correlations in Spectroscopy and Microscopy

Gur Lubin, Dan Oron, Uri Rossman +2 more

Measurements of photon temporal correlations have been the mainstay of experiments in quantum optics. Over the past several decades, advancements in detector technologies have supported further extending photon correlation techniques to give rise to novel spectroscopy and imaging methods. This Perspective reviews the evolution of these techniques from temporal autocorrelations through multidimensional photon correlations to photon correlation imaging. State-of-the-art single-photon detector technologies are discussed, highlighting the main challenges and the unique current perspective of photon correlations to usher in a new generation of spectroscopy and imaging modalities.

ACS Photonics•Sep 7, 2022•30 citations

Measuring the Single-Photon Temporal-Spectral Wave Function

Alex O. C. Davis, Valérian Thiel, Michał Karpiński +1 more

Temporal-spectral modes of light provide a fundamental window into the nature of quantum systems and offer a robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding single-photon sources and their applications in emerging optical quantum technologies. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the pulse-mode structure of heralded single photons.

arXiv:1709.05248•Physical Review Letters•Aug 21, 2018•60 citations

Quantum imaging with SPAD arrays (Conference Presentation)

Gur Lubin, Ron Tenne, Ivan Michel Antolović +3 more

The emerging field of quantum imaging introduces new methods to overcome classical limitations in optical microscopy. A detection apparatus capable of analyzing the quantum signature of light, is a crucial component in the heart of any such method. We present a novel quantum imaging modality, based on a state-of-the-art single photon avalanche diode (SPAD) array in a confocal setup. This modality enables unprecedented simplicity and scalability in imaging temporal photon correlations. We demonstrate the potential of this approach by measuring temporal correlations of classical and quantum sources, as well as demonstrate a quantum super-resolution technique.

Single Molecule Spectroscopy and Superresolution Imaging•Mar 9, 2020•0 citations

Purification of Single Photons by Temporal Heralding of Quantum Dot Sources

Hamza A. Abudayyeh, Boaz Lubotzky, Somak Majumder +2 more

Efficient, high rate photon sources with high single-photon purity are essential ingredients for quantum technologies. Single-photon sources based on solid state emitters such as quantum dots are very advantageous for integrated photonic circuits, but they can suffer from a high two-photon emission probability, which in cases of noncryogenic environment cannot be spectrally filtered. Here we propose two temporal purification-by-heralding methods for using a two-photon emission process to yield highly pure and efficient single-photon emission, bypassing the inherent problem of spectrally overlapping biphoton emission at elevated temperatures. We experimentally emulate their feasibility on the emission from a single nanocrystal quantum dot at room temperature, exhibiting single-photon purities exceeding 99.5%, without a significant loss of single-photon efficiency. By utilizing these methods with commercially available components, nanocrystal quantum dots can be made realistic high-quality room-temperature sources for single photons. These approaches can also be applied for any indeterministic source of spectrally broadband photon pairs.

arXiv:1805.00201•ACS Photonics•Jan 24, 2019•22 citations

Generalized Hanbury Brown–Twiss interferometer

Yiqi Song, Meixue Chen, Yuhan Ma +7 more

The Hanbury Brown–Twiss (HBT) interferometer, which is used to measure the correlation of two photons or two light beams, has played a crucial role in quantum optics and quantum information. We propose a generalized HBT interferometer, which is able to measure the correlation of photons or light beams up to eight in a single experimental run. With an improved time correlated single-photon counting (TCSPC) algorithm, two-, three-, and four-photon coincidence counts, and the degree of fifth-order coherence of pseudothermal light are measured with a data collection time of 60 s. The generalized HBT interferometer can be used to measure the correlation of two multi-photon detection events by simulating photon number resolving detectors with multiple single-photon detectors. The generalized HBT interferometer and improved TCSPC algorithm provide a versatile framework for studying multi-photon correlations and interference, which is helpful to understand the physics of multi-photon interference and may find applications in fluorescence lifetime imaging and other techniques using TCSPC.

Journal of the Optical Society of America B•Mar 3, 2026•0 citations

All-Optical Fiber Hanbury Brown & Twiss Interferometer to study 1300 nm single photon emission of a metamorphic InAs Quantum Dot

Guillermo Muñoz‐Matutano, David Barrera, Carlos R. Fernández‐Pousa +6 more

New optical fiber based spectroscopic tools open the possibility to develop more robust and efficient characterization experiments. Spectral filtering and light reflection have been used to produce compact and versatile fiber based optical cavities and sensors. Moreover, these technologies would be also suitable to study N-photon correlations, where high collection efficiency and frequency tunability is desirable. We demonstrated single photon emission of a single quantum dot emitting at 1300 nm, using a Fiber Bragg Grating for wavelength filtering and InGaAs Avalanche Photodiodes operated in Geiger mode for single photon detection. As we do not observe any significant fine structure splitting for the neutral exciton transition within our spectral resolution (46 μeV), metamorphic QD single photon emission studied with our all-fiber Hanbury Brown &Twiss interferometer could lead to a more efficient analysis of entangled photon sources at telecom wavelength. This all-optical fiber scheme opens the door to new first and second order interferometers to study photon indistinguishability, entangled photon and photon cross correlation in the more interesting telecom wavelengths.

Scientific Reports•Jun 3, 2016•38 citations
Since the introduction of the intensity interferometer by Hanbury Brown and Twiss in the '50s and its subsequent adaptations to quantum optic experiments, photon correlations have played a significant role in optical research. An emerging detector technology, SPAD arrays, presents new opportunities to scale these experiments and exploit photon correlations in new regimes. I will describe a new temporal-spectral photon correlation technique based on these detectors, single-particle heralded spectroscopy. I will present new insights into the photophysics of multiply-excited semiconductor quantum dots uncovered by this method, hitherto inaccessible to existing approaches.
Measurements of photon temporal correlations have been the mainstay of experiments in quantum optics. Over the past several decades, advancements in detector technologies have supported further extending photon correlation techniques to give rise to novel spectroscopy and imaging methods. This Perspective reviews the evolution of these techniques from temporal autocorrelations through multidimensional photon correlations to photon correlation imaging. State-of-the-art single-photon detector technologies are discussed, highlighting the main challenges and the unique current perspective of photon correlations to usher in a new generation of spectroscopy and imaging modalities.
Temporal-spectral modes of light provide a fundamental window into the nature of quantum systems and offer a robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding single-photon sources and their applications in emerging optical quantum technologies. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the pulse-mode structure of heralded single photons.
The emerging field of quantum imaging introduces new methods to overcome classical limitations in optical microscopy. A detection apparatus capable of analyzing the quantum signature of light, is a crucial component in the heart of any such method. We present a novel quantum imaging modality, based on a state-of-the-art single photon avalanche diode (SPAD) array in a confocal setup. This modality enables unprecedented simplicity and scalability in imaging temporal photon correlations. We demonstrate the potential of this approach by measuring temporal correlations of classical and quantum sources, as well as demonstrate a quantum super-resolution technique.
Efficient, high rate photon sources with high single-photon purity are essential ingredients for quantum technologies. Single-photon sources based on solid state emitters such as quantum dots are very advantageous for integrated photonic circuits, but they can suffer from a high two-photon emission probability, which in cases of noncryogenic environment cannot be spectrally filtered. Here we propose two temporal purification-by-heralding methods for using a two-photon emission process to yield highly pure and efficient single-photon emission, bypassing the inherent problem of spectrally overlapping biphoton emission at elevated temperatures. We experimentally emulate their feasibility on the emission from a single nanocrystal quantum dot at room temperature, exhibiting single-photon purities exceeding 99.5%, without a significant loss of single-photon efficiency. By utilizing these methods with commercially available components, nanocrystal quantum dots can be made realistic high-quality room-temperature sources for single photons. These approaches can also be applied for any indeterministic source of spectrally broadband photon pairs.
The Hanbury Brown–Twiss (HBT) interferometer, which is used to measure the correlation of two photons or two light beams, has played a crucial role in quantum optics and quantum information. We propose a generalized HBT interferometer, which is able to measure the correlation of photons or light beams up to eight in a single experimental run. With an improved time correlated single-photon counting (TCSPC) algorithm, two-, three-, and four-photon coincidence counts, and the degree of fifth-order coherence of pseudothermal light are measured with a data collection time of 60 s. The generalized HBT interferometer can be used to measure the correlation of two multi-photon detection events by simulating photon number resolving detectors with multiple single-photon detectors. The generalized HBT interferometer and improved TCSPC algorithm provide a versatile framework for studying multi-photon correlations and interference, which is helpful to understand the physics of multi-photon interference and may find applications in fluorescence lifetime imaging and other techniques using TCSPC.
New optical fiber based spectroscopic tools open the possibility to develop more robust and efficient characterization experiments. Spectral filtering and light reflection have been used to produce compact and versatile fiber based optical cavities and sensors. Moreover, these technologies would be also suitable to study N-photon correlations, where high collection efficiency and frequency tunability is desirable. We demonstrated single photon emission of a single quantum dot emitting at 1300 nm, using a Fiber Bragg Grating for wavelength filtering and InGaAs Avalanche Photodiodes operated in Geiger mode for single photon detection. As we do not observe any significant fine structure splitting for the neutral exciton transition within our spectral resolution (46 μeV), metamorphic QD single photon emission studied with our all-fiber Hanbury Brown &Twiss interferometer could lead to a more efficient analysis of entangled photon sources at telecom wavelength. This all-optical fiber scheme opens the door to new first and second order interferometers to study photon indistinguishability, entangled photon and photon cross correlation in the more interesting telecom wavelengths.