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Applied Physics Letters

Slow-light dispersion of a cavity polariton in an organic crystal microcavity

Masamitsu Amano, Kazuhito Otsuka, Tohru Fujihara, Hisao Kondo, Kazuki Bando

Published Mar 28, 2022• 3 citations
Publisher

Abstract

Herein, we have measured the phase dispersion of a cavity polariton in a single-crystalline anthracene microcavity via interference spectroscopy. Results show slow-light dispersion at the cavity polariton's lower polariton resonance, which agrees well with the transfer matrix method calculation results. According to the theoretical calculations, the slow-light dispersion's group refractive index is 24. We found that the structural dispersion due to a phenomenological photon cavity and material dispersion caused by the exciton contributed to the large group refractive index. These efforts will aid in realizing optical buffer memories for organic microcavities.

DOI
10.1063/5.0079497

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Herein, we have measured the phase dispersion of a cavity polariton in a single-crystalline anthracene microcavity via interference spectroscopy. Results show slow-light dispersion at the cavity polariton's lower polariton resonance, which agrees well with the transfer matrix method calculation results. According to the theoretical calculations, the slow-light dispersion's group refractive index is 24. We found that the structural dispersion due to a phenomenological photon cavity and material dispersion caused by the exciton contributed to the large group refractive index. These efforts will aid in realizing optical buffer memories for organic microcavities.
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We discuss the prospects for enhancing absorption and scattering of light from a weakly coupled atom in a high-finesse optical cavity by adding a medium with large, positive group index of refraction. The slow-light effect is known to narrow the cavity transmission spectrum and increase the photon lifetime, but the quality factor of the cavity is not increased in a metrologically useful sense. Specifically, detection of the weakly coupled atom through either cavity ringdown measurements or the Purcell effect fails to improve with the addition of material slow light. A single-atom model of the dispersive medium helps elucidate why this is the case.
Optical microcavities with ultralong photon storage times are of central importance for integrated nanophotonics. To date, record quality (Q) factors up to 10^{11} have been measured in millimetric-size single-crystal whispering-gallery-mode (WGM) resonators, and 10^{10} in silica or glass microresonators. We show that, by introducing slow-light effects in an active WGM microresonator, it is possible to enhance the photon lifetime by several orders of magnitude, thus circumventing both fabrication imperfections and residual absorption. The slow-light effect is obtained from coherent population oscillations in an erbium-doped fluoride glass microsphere, producing strong dispersion of the WGM (group index n_{g}∼10^{6}). As a result, a photon lifetime up to 2.5 ms at room temperature has been measured, corresponding to a Q factor of 3×10^{12} at 1530 nm. This system could yield a new type of optical memory microarray with ultralong storage times.
We discuss the prospects for enhancing absorption and scattering of light from a weakly coupled atom in a high-finesse optical cavity by adding a medium with large, positive group index of refraction. The slow-light effect is known to narrow the cavity transmission spectrum and increase the photon lifetime, but the quality factor of the cavity may not be increased in a metrologically useful sense. Specifically, detection of the weakly coupled atom through either cavity ringdown measurements or the Purcell effect fails to improve with the addition of material slow light. A single-atom model of the dispersive medium helps elucidate why this is the case.
Slow and fast light processes, based on both structural and material dispersions, are realized in a wide tuning range in this article. Coherent population oscillations (CPO) in electrically tunable quantum dot semiconductor optical amplifiers lead to a variable group index ranging from the background index ( n bgd ) to ∼ 30. A photonic crystal waveguide is then dispersion engineered and a group index of 260 with the normalized delay-bandwidth product (NDBP) of 0.65 is achieved in the proposed waveguide. Using comprehensive numerical simulations, we show that a considerable enhancement of slow light effect can be achieved by combining both the material and the structural dispersions in the proposed active QDPCW structure. We compare our developed FDTD results with analytical results and show that there is good agreement between the results, which demonstrates that the proposed electrically-tunable slow light idea is obtainable in the QDPCW structure. We achieve a total group index in a wide tuning range from n bgd to ∼ 1500 at the operation bandwidth, which shows a significant enhancement compared with the schemes based only on material or structural dispersions. The tuning range and also NDBP of the slow light scheme are much larger than those of the electrically tunable CPO process.
Slow light is a regime of reduced group velocity, resulting in increased photon density in optical pulses and enhanced nonlinear effects. Here, we propose the realization of slow light in the regime of strong light-matter interaction between waveguide photons and semiconductor excitons. We design a dielectric superlattice structure with a nearly-flat band characterized by low group velocity and group velocity dispersion, both required for enhancing nonlinear effects with ultrashort pulses. Furthermore, by applying this general framework to a perovskite-based structure, we demonstrate an enhancement of the single-particle phase shift by a factor of more than 20, representing a significant step toward the few-photon quantum regime. Our results provide a blueprint for accessible strong interactions in solid-state integrated optics.