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Journal of Physics Conference Series

Discord effects of inter-cluster interactions on a cluster-based Haldane state in a triangular spin tube

Takanori Sugimoto, Takami Tohyama

Published Mar 1, 2022• 1 citation
Publisher

Abstract

Abstract We have recently proposed a new concept of cluster-based Haldane states supported by an inherent chirality in a triangular spin tube with equivalent inter-cluster interactions. In this state, there appear spin-1/2 degrees of freedom consisting of a real spin and a scalar chirality as edge states. With applying a magnetic field, we can observe approximately a half of magnetization of S = 1/2 spin, i.e., a quarter spin magnetization, due to symmetrization of the real spin and the chirality. Here, we consider effects of discord between two types of inter-cluster interactions, inducing anisotropic biquadratic interactions of effective S = 1 spins. The discord brings the edge magnetization nearer to an exact value of quarter spin magnetization, whereas localization of the edge states becomes worse. These effects are also confirmed in a corresponding spin-1 model.

DOI
10.1088/1742-6596/2164/1/012029

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Since the Heisenberg spin chain can be considered the simplest realistic model of magnetism, surprise and some degree of controversy have resulted from recent work of Haldane. The prediction is that quantum spin chains with half-integer spin should all display T=0 phase behavior equivalent to that of the Bethe Ansatz integrable (solvable) spin-1/2 quantum chain. More remarkably, the class of integer spin chains is predicted to show very different phase behavior. In particular, a gap should be present in the spectrum of a Heisenberg antiferromagnetic chain. This remarkable feature is counterintuitive in terms of accepted wisdom in magnetism (spin-wave theory, spin-Peierls theory) and critical phenomena. Consequently the vertification of the prediction is of great interest. A considerable amount of numerical work has been done, involving finite-chain, finite-size scaling, variational, Monte Carlo and other calculations, which will be reviewed here. The present consensus is that the weight of numerical evidence supports the prediction, although puzzling features still remain. Adding additional interactions to the basic Heisenberg Hamiltonian such as spin (XXZ) anisotropy, single-ion anisotropy, biquadratic exchange, and an applied magnetic field, generates a rich and complicated phase diagram for chains with spin >1/2, particularly for the case of integer spin. The s=1 phase diagram seems to display critical behavior of a type not previously encountered. A theoretical appraisal of the Haldane phenomenon will include a discussion of the possible role of nonintegrability. Mention will also be made of current progress in experimental investigation of the phenomenon, including problems that might be encountered. More recent work of Affleck has greatly generalized the field-theoretic mappings which underlay the original work of Haldane. A number of interesting problems have been mapped into quantum spin chains of various types, including field theoretic phenomena and the localization problem of the quantum Hall effect.

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Abstract We have recently proposed a new concept of cluster-based Haldane states supported by an inherent chirality in a triangular spin tube with equivalent inter-cluster interactions. In this state, there appear spin-1/2 degrees of freedom consisting of a real spin and a scalar chirality as edge states. With applying a magnetic field, we can observe approximately a half of magnetization of S = 1/2 spin, i.e., a quarter spin magnetization, due to symmetrization of the real spin and the chirality. Here, we consider effects of discord between two types of inter-cluster interactions, inducing anisotropic biquadratic interactions of effective S = 1 spins. The discord brings the edge magnetization nearer to an exact value of quarter spin magnetization, whereas localization of the edge states becomes worse. These effects are also confirmed in a corresponding spin-1 model.
Abstract Fractionalization of quantum degrees of freedom holds the key to finding new phenomena in physics, e.g., the quark model in hadron physics and the spin-charge separation in strongly-correlated electron systems. A typical example of the fractionalization in quantum spin systems is the spin-1 Haldane state, whose intriguing characteristics are well described by fractionalized virtual spins, delivering two individual spin-1/2 degrees of freedom as edge states. Here we theoretically propose an exotic extension of the Haldane state to the pseudo spin-1 model consisting of the mixture of real spin and spin chirality, resulting in quasi-fractionalization of spin-1/2 magnetization, i.e., an approximately-1/4 spin. Existence of the edge state is confirmed both analytically and numerically in a triangular spin tube, combining a low-energy perturbation theory and variational matrix-product state method. Our study not only proposes an unconventional quantum spin object but paves a way to chop the elementary quantities further.
The authors provide a concept of the Haldane states designed in spin cluster chains, where S=1/2 spins in a cluster strongly interact with each other as compared with inter cluster interactions. As an extension of the Affleck-Kenned-Lieb-Tasaki state, the Haldane states are demonstrated in the spin cluster chains whose cluster consists of not only even but also odd number of spins. Particularly, the Haldane state in the case of an odd number of spins in a cluster is induced by the magnetic field and emerges as a magnetization plateau.
Quantum discord (QD) is a general measure of bipartite quantum correlations with a potential role in quantum information processing tasks. Spin clusters serve as ideal candidates for the implementation of some of the associated protocols. In this paper, we consider a symmetric spin trimer and a tetramer which describe a number of known molecular magnets and compute the QD in the ground and thermal states of the clusters. The variations of the QD as a function of an anisotropy parameter, magnetic field and temperature are investigated. We obtain a number of interesting results such as a finite value of the QD in the trimer ground state for which the pairwise entanglement is known to be zero, differences in the nature of some of the variations in the ferromagnetic and antiferromagnetic cases, and discontinuous jumps in the magnitude of the QD at first-order quantum phase transition points. A remarkable feature that is observed is that the QD completely vanishes only in the asymptotic limit of temperature T → ∞. We further study the dynamics of the QD and the pairwise entanglement at T = 0 under the effect of a dephasing channel describing the interaction of the reduced spin cluster state with independent local environments. The QD is found to vanish asymptotically as t → ∞. In the case of the spin trimer, the pairwise entanglement has a zero value at all times and reaches a zero value in a finite time in the case of the tetramer.
Quantum discord (QD) is a general measure of bipartite quantum correlations with a potential role in quantum information processing tasks. Spin clusters serve as ideal candidates for the implementation of some of the associated protocols. In this paper, we consider a symmetric spin trimer and a tetramer which describe a number of known molecular magnets and compute the QD in the ground and thermal states of the clusters. The variations of the QD as a function of an anisotropy parameter, magnetic field and temperature are investigated. We obtain a number of interesting results such as a finite value of the QD in the trimer ground state for which the pairwise entanglement is known to be zero, differences in the nature of some of the variations in the ferromagnetic and antiferromagnetic cases, and discontinuous jumps in the magnitude of the QD at first-order quantum phase transition points. A remarkable feature that is observed is that the QD completely vanishes only in the asymptotic limit of temperature T → ∞. We further study the dynamics of the QD and the pairwise entanglement at T = 0 under the effect of a dephasing channel describing the interaction of the reduced spin cluster state with independent local environments. The QD is found to vanish asymptotically as t → ∞. In the case of the spin trimer, the pairwise entanglement has a zero value at all times and reaches a zero value in a finite time in the case of the tetramer.
We use a combination of numerical density matrix renormalization group calculations and several analytical approaches to comprehensively study a simplified model for a spatially anisotropic spin-12\frac{1}{2}21​ triangular lattice Heisenberg antiferromagnet: the three-leg triangular spin tube (TST). The model is described by three Heisenberg chains, with exchange constant JJJ, coupled antiferromagnetically with exchange constant ${J}^{\ensuremath{'}}$ along the diagonals of the ladder system, with periodic boundary conditions in the shorter direction. Here, we determine the full phase diagram of this model as a function of both spatial anisotropy (between the isotropic and decoupled chain limits) and magnetic field. We find a rich phase diagram, which is remarkably dominated by quantum states: the phase corresponding to the classical ground state appears only in an exceedingly small region. Among the dominant phases generated by quantum effects are commensurate and incommensurate coplanar quasiordered states, which appear in the vicinity of the isotropic region for most fields, and in the high-field region for most anisotropies. The coplanar states, while not classical ground states, can at least be understood semiclassically. Even more strikingly, the largest region of phase space is occupied by a spin density wave phase, which has incommensurate collinear correlations along the field. This phase has no semiclassical analog, and may be ascribed to enhanced one-dimensional fluctuations due to frustration. Cutting across the phase diagram is a magnetization plateau, with a gap to all excitations and ``up-up-down'' spin order, with a quantized magnetization equal to 13\frac{1}{3}31​ of the saturation value. In the TST, this plateau extends almost but not quite to the decoupled chains limit. Most of the above features are expected to carry over to the two-dimensional system, which we also discuss. At low field, a dimerized phase appears, which is particular to the one-dimensional nature of the TST, and which can be understood from quantum Berry phase arguments.
Since the Heisenberg spin chain can be considered the simplest realistic model of magnetism, surprise and some degree of controversy have resulted from recent work of Haldane. The prediction is that quantum spin chains with half-integer spin should all display T=0 phase behavior equivalent to that of the Bethe Ansatz integrable (solvable) spin-1/2 quantum chain. More remarkably, the class of integer spin chains is predicted to show very different phase behavior. In particular, a gap should be present in the spectrum of a Heisenberg antiferromagnetic chain. This remarkable feature is counterintuitive in terms of accepted wisdom in magnetism (spin-wave theory, spin-Peierls theory) and critical phenomena. Consequently the vertification of the prediction is of great interest. A considerable amount of numerical work has been done, involving finite-chain, finite-size scaling, variational, Monte Carlo and other calculations, which will be reviewed here. The present consensus is that the weight of numerical evidence supports the prediction, although puzzling features still remain. Adding additional interactions to the basic Heisenberg Hamiltonian such as spin (XXZ) anisotropy, single-ion anisotropy, biquadratic exchange, and an applied magnetic field, generates a rich and complicated phase diagram for chains with spin >1/2, particularly for the case of integer spin. The s=1 phase diagram seems to display critical behavior of a type not previously encountered. A theoretical appraisal of the Haldane phenomenon will include a discussion of the possible role of nonintegrability. Mention will also be made of current progress in experimental investigation of the phenomenon, including problems that might be encountered. More recent work of Affleck has greatly generalized the field-theoretic mappings which underlay the original work of Haldane. A number of interesting problems have been mapped into quantum spin chains of various types, including field theoretic phenomena and the localization problem of the quantum Hall effect.